DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Coherent control of a single nitrogen-vacancy center spin in optically levitated nanodiamond

Abstract

Here, we report the first observation, to the best of our knowledge, of electron spin transients in single negatively charged nitrogen-vacancy (NV-) centers, contained within optically trapped nanodiamonds, in both atmospheric pressure and low vacuum. It is shown that, after an initial exposure to low vacuum, the trapped nanodiamonds remain at temperatures near room temperature even in low vacuum. Furthermore, the transverse coherence time of the NV- center spin, measured to be T2=101.4 ns, is robust over the range of trapping powers considered in this study.

Authors:
 [1]; ORCiD logo [2];  [1];  [3]
  1. Univ. of Rochester, NY (United States). Inst. of Optics; Univ. of Rochester, NY (United States). Center for Coherence and Quantum Optics
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  3. Univ. of Rochester, NY (United States). Inst. of Optics; Univ. of Rochester, NY (United States). Center for Coherence and Quantum Optics; Univ. of Rochester, NY (United States). Dept. of Physics and Astronomy; Univ. of Rochester, NY (United States). Materials Science Program
Publication Date:
Research Org.:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
US Department of the Navy, Office of Naval Research (ONR); USDOE
OSTI Identifier:
1364550
Report Number(s):
LA-UR-17-20272
Journal ID: ISSN 0740-3224
Grant/Contract Number:  
AC52-06NA25396
Resource Type:
Accepted Manuscript
Journal Name:
Journal of the Optical Society of America. Part B, Optical Physics
Additional Journal Information:
Journal Volume: 34; Journal Issue: 6; Journal ID: ISSN 0740-3224
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE

Citation Formats

Pettit, Robert M., Neukirch, Levi Patrick, Zhang, Yi, and Vamivakas, A. Nick. Coherent control of a single nitrogen-vacancy center spin in optically levitated nanodiamond. United States: N. p., 2017. Web. doi:10.1364/JOSAB.34.000C31.
Pettit, Robert M., Neukirch, Levi Patrick, Zhang, Yi, & Vamivakas, A. Nick. Coherent control of a single nitrogen-vacancy center spin in optically levitated nanodiamond. United States. https://doi.org/10.1364/JOSAB.34.000C31
Pettit, Robert M., Neukirch, Levi Patrick, Zhang, Yi, and Vamivakas, A. Nick. Fri . "Coherent control of a single nitrogen-vacancy center spin in optically levitated nanodiamond". United States. https://doi.org/10.1364/JOSAB.34.000C31. https://www.osti.gov/servlets/purl/1364550.
@article{osti_1364550,
title = {Coherent control of a single nitrogen-vacancy center spin in optically levitated nanodiamond},
author = {Pettit, Robert M. and Neukirch, Levi Patrick and Zhang, Yi and Vamivakas, A. Nick},
abstractNote = {Here, we report the first observation, to the best of our knowledge, of electron spin transients in single negatively charged nitrogen-vacancy (NV-) centers, contained within optically trapped nanodiamonds, in both atmospheric pressure and low vacuum. It is shown that, after an initial exposure to low vacuum, the trapped nanodiamonds remain at temperatures near room temperature even in low vacuum. Furthermore, the transverse coherence time of the NV- center spin, measured to be T2=101.4 ns, is robust over the range of trapping powers considered in this study.},
doi = {10.1364/JOSAB.34.000C31},
journal = {Journal of the Optical Society of America. Part B, Optical Physics},
number = 6,
volume = 34,
place = {United States},
year = {Fri May 12 00:00:00 EDT 2017},
month = {Fri May 12 00:00:00 EDT 2017}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 24 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

A quantum memory intrinsic to single nitrogen–vacancy centres in diamond
journal, June 2011

  • Fuchs, G. D.; Burkard, G.; Klimov, P. V.
  • Nature Physics, Vol. 7, Issue 10
  • DOI: 10.1038/nphys2026

Quantum register based on coupled electron spins in a room-temperature solid
journal, February 2010

  • Neumann, P.; Kolesov, R.; Naydenov, B.
  • Nature Physics, Vol. 6, Issue 4
  • DOI: 10.1038/nphys1536

Quantum entanglement between an optical photon and a solid-state spin qubit
journal, August 2010


Nanoscale Nuclear Magnetic Resonance with a Nitrogen-Vacancy Spin Sensor
journal, January 2013


Magnetometry with nitrogen-vacancy defects in diamond
journal, May 2014


Nanoscale magnetic sensing with an individual electronic spin in diamond
journal, October 2008

  • Maze, J. R.; Stanwix, P. L.; Hodges, J. S.
  • Nature, Vol. 455, Issue 7213
  • DOI: 10.1038/nature07279

Electric-field sensing using single diamond spins
journal, April 2011

  • Dolde, F.; Fedder, H.; Doherty, M. W.
  • Nature Physics, Vol. 7, Issue 6
  • DOI: 10.1038/nphys1969

Nanometre-scale thermometry in a living cell
journal, July 2013


Nanoscale Fluorescence Lifetime Imaging of an Optical Antenna with a Single Diamond NV Center
journal, July 2013

  • Beams, Ryan; Smith, Dallas; Johnson, Timothy W.
  • Nano Letters, Vol. 13, Issue 8
  • DOI: 10.1021/nl401791v

Coherent Sensing of a Mechanical Resonator with a Single-Spin Qubit
journal, February 2012

  • Kolkowitz, S.; Bleszynski Jayich, A. C.; Unterreithmeier, Q. P.
  • Science, Vol. 335, Issue 6076
  • DOI: 10.1126/science.1216821

A single nitrogen-vacancy defect coupled to a nanomechanical oscillator
journal, September 2011

  • Arcizet, O.; Jacques, V.; Siria, A.
  • Nature Physics, Vol. 7, Issue 11
  • DOI: 10.1038/nphys2070

Matter-Wave Interferometry of a Levitated Thermal Nano-Oscillator Induced and Probed by a Spin
journal, October 2013


Large quantum superpositions of a levitated nanodiamond through spin-optomechanical coupling
journal, September 2013


Large Quantum Superpositions and Interference of Massive Nanometer-Sized Objects
journal, July 2011


Testing quantum gravity by nanodiamond interferometry with nitrogen-vacancy centers
journal, September 2014


Single and two-mode mechanical squeezing of an optically levitated nanodiamond via dressed-state coherence
journal, October 2016


Room-temperature ultrasensitive mass spectrometer via dynamical decoupling
journal, October 2014


Multi-dimensional single-spin nano-optomechanics with a levitated nanodiamond
journal, September 2015

  • Neukirch, Levi P.; von Haartman, Eva; Rosenholm, Jessica M.
  • Nature Photonics, Vol. 9, Issue 10
  • DOI: 10.1038/nphoton.2015.162

Electron spin control of optically levitated nanodiamonds in vacuum
journal, July 2016

  • Hoang, Thai M.; Ahn, Jonghoon; Bang, Jaehoon
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms12250

Electron spin resonance from NV centers in diamonds levitating in an ion trap
journal, March 2017


Nanoscale temperature measurements using non-equilibrium Brownian dynamics of a levitated nanosphere
journal, May 2014


Measurement of the Instantaneous Velocity of a Brownian Particle
journal, May 2010


Subkelvin Parametric Feedback Cooling of a Laser-Trapped Nanoparticle
journal, September 2012


Millikelvin cooling of an optically trapped microsphere in vacuum
journal, March 2011

  • Li, Tongcang; Kheifets, Simon; Raizen, Mark G.
  • Nature Physics, Vol. 7, Issue 7
  • DOI: 10.1038/nphys1952

Torsional Optomechanics of a Levitated Nonspherical Nanoparticle
journal, September 2016


Burning and graphitization of optically levitated nanodiamonds in vacuum
journal, February 2016

  • Rahman, A. T. M. A.; Frangeskou, A. C.; Kim, M. S.
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep21633

Surface Structure of Aerobically Oxidized Diamond Nanocrystals
journal, November 2014

  • Wolcott, Abraham; Schiros, Theanne; Trusheim, Matthew E.
  • The Journal of Physical Chemistry C, Vol. 118, Issue 46
  • DOI: 10.1021/jp506992c

Electronic Properties and Metrology Applications of the Diamond NV Center under Pressure
journal, January 2014


Observation of nitrogen vacancy photoluminescence from an optically levitated nanodiamond
journal, January 2013

  • Neukirch, Levi P.; Gieseler, Jan; Quidant, Romain
  • Optics Letters, Vol. 38, Issue 16
  • DOI: 10.1364/OL.38.002976

Ultralong spin coherence time in isotopically engineered diamond
journal, April 2009

  • Balasubramanian, Gopalakrishnan; Neumann, Philipp; Twitchen, Daniel
  • Nature Materials, Vol. 8, Issue 5
  • DOI: 10.1038/nmat2420

Dynamical decoupling of a single-electron spin at room temperature
journal, February 2011


Optical and Spin Coherence Properties of Nitrogen-Vacancy Centers Placed in a 100 nm Thick Isotopically Purified Diamond Layer
journal, January 2012

  • Ishikawa, Toyofumi; Fu, Kai-Mei C.; Santori, Charles
  • Nano Letters, Vol. 12, Issue 4
  • DOI: 10.1021/nl300350r

Works referencing / citing this record:

An optical tweezer phonon laser
journal, April 2019


Magneto-mechanical trapping of micro-diamonds at low pressures
journal, February 2019

  • O'Brien, M. C.; Dunn, S.; Downes, J. E.
  • Applied Physics Letters, Vol. 114, Issue 5
  • DOI: 10.1063/1.5066065

Optomechanics with levitated particles
journal, January 2020

  • Millen, James; Monteiro, Tania S.; Pettit, Robert
  • Reports on Progress in Physics, Vol. 83, Issue 2
  • DOI: 10.1088/1361-6633/ab6100

Pure nanodiamonds for levitated optomechanics in vacuum
journal, April 2018

  • Frangeskou, A. C.; Rahman, A. T. M. A.; Gines, L.
  • New Journal of Physics, Vol. 20, Issue 4
  • DOI: 10.1088/1367-2630/aab700

Ramsey Interferences and Spin Echoes from Electron Spins Inside a Levitating Macroscopic Particle
journal, July 2018


Laser-induced heating in a high-density ensemble of nitrogen-vacancy centers in diamond and its effects on quantum sensing
journal, January 2019

  • Duan, Dewen; Kavatamane, Vinaya Kumar; Arumugam, Sri Ranjini
  • Optics Letters, Vol. 44, Issue 11
  • DOI: 10.1364/ol.44.002851