A statistical correlation investigation for the role of surface spins to the spin relaxation of nitrogen vacancy centers

Journal Article · Tue Apr 15 00:00:00 EDT 2014 · AIP Advances

DOI:https://doi.org/10.1063/1.4870938· OSTI ID:22253288

Song, Xuerui; Zhang, Jian; Feng, Fupan; Wang, Junfeng; Zhang, Wenlong; Lou, Liren; Zhu, Wei; Wang, Guanzhong ^[1]

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1. Hefei National Laboratory for Physical Science at Microscale, and Department of Physics, University of Science and Technology of China, Hefei, Anhui, 230026 (China)

We investigated the influence of spins on surface of nanodiamonds (NDs) to the longitudinal relaxation time (T{sub 1}) and transverse relaxation time (T{sub 2}) of nitrogen vacancy (NV) centers in ND. A spherical model of the NDs was suggested to account for the experimental results of T{sub 1} and T{sub 2}, and the density of surface spins was roughly estimated based on the statistical analysis of experimental results of 72 NDs containing a single NV center. For NDs studied here, the T{sub 1} of NV center inside is highly dependent to the surface spins of the NDs. However, for the T{sub 2} of NV center, intrinsic contributions must be much pronounced than that by surface spins. In other words, T{sub 1} of an NV center in NDs is more sensitive to the change of the surface spin density than T{sub 2}.

• OSTI ID: 22253288
• Journal Information: AIP Advances, Vol. 4, Issue 4; Other Information: (c) 2014 Author(s); Country of input: International Atomic Energy Agency (IAEA); ISSN 2158-3226
• Country of Publication: United States
• Language: English

Related Subjects

36 MATERIALS SCIENCE
DENSITY
NITROGEN
RELAXATION TIME
SPIN
SURFACES