Geometrical control of topological charge transfer in Shakti-Cairo colloidal ice
Abstract
Lattice transformations that preserve the system topology, but not its geometry, are common in condensed matter systems. However, how geometric constrains influence the topological properties of the lattices is still unclear. Here we show that a geometric transformation between two mixed coordination lattices, from Shakti to Cairo in an artificial colloidal ice, leads to a breakdown of the ice rule in all but one specific geometry. We observe a transfer of topological charge among sublattices which can be controlled in sign and intensity, vanishing at the ice-rule point. These unusual topological effects are absent in magnetic spin ices and they are due to collective, non-local geometric frustration in the particle ice. By merging numerical simulations, theory and experiments, we demonstrate how the charge transfer occurs in the Cairo geometry. The broader implication of our results is that we demonstrate how geometric constraints can control the topological properties of a mesoscopic colloidal system.
- Authors:
-
- Univ. of Barcelona (Spain)
- Univ. of Barcelona (Spain); Escuela de Ingenieria y Ciencias, Tecnologico de Monterrey, NL (Mexico)
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Laboratory Directed Research and Development (LDRD) Program
- OSTI Identifier:
- 1992278
- Report Number(s):
- LA-UR-23-20641
Journal ID: ISSN 2399-3650; TRN: US2404191
- Grant/Contract Number:
- 89233218CNA000001
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Communications Physics
- Additional Journal Information:
- Journal Volume: 6; Journal Issue: 1; Journal ID: ISSN 2399-3650
- Publisher:
- Springer Nature
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; magnetic properties; materials; structure of solids and liquids
Citation Formats
Rodríguez-Gallo, Carolina, Ortiz-Ambriz, Antonio, Nisoli, Cristiano, and Tierno, Pietro. Geometrical control of topological charge transfer in Shakti-Cairo colloidal ice. United States: N. p., 2023.
Web. doi:10.1038/s42005-023-01236-7.
Rodríguez-Gallo, Carolina, Ortiz-Ambriz, Antonio, Nisoli, Cristiano, & Tierno, Pietro. Geometrical control of topological charge transfer in Shakti-Cairo colloidal ice. United States. https://doi.org/10.1038/s42005-023-01236-7
Rodríguez-Gallo, Carolina, Ortiz-Ambriz, Antonio, Nisoli, Cristiano, and Tierno, Pietro. Tue .
"Geometrical control of topological charge transfer in Shakti-Cairo colloidal ice". United States. https://doi.org/10.1038/s42005-023-01236-7. https://www.osti.gov/servlets/purl/1992278.
@article{osti_1992278,
title = {Geometrical control of topological charge transfer in Shakti-Cairo colloidal ice},
author = {Rodríguez-Gallo, Carolina and Ortiz-Ambriz, Antonio and Nisoli, Cristiano and Tierno, Pietro},
abstractNote = {Lattice transformations that preserve the system topology, but not its geometry, are common in condensed matter systems. However, how geometric constrains influence the topological properties of the lattices is still unclear. Here we show that a geometric transformation between two mixed coordination lattices, from Shakti to Cairo in an artificial colloidal ice, leads to a breakdown of the ice rule in all but one specific geometry. We observe a transfer of topological charge among sublattices which can be controlled in sign and intensity, vanishing at the ice-rule point. These unusual topological effects are absent in magnetic spin ices and they are due to collective, non-local geometric frustration in the particle ice. By merging numerical simulations, theory and experiments, we demonstrate how the charge transfer occurs in the Cairo geometry. The broader implication of our results is that we demonstrate how geometric constraints can control the topological properties of a mesoscopic colloidal system.},
doi = {10.1038/s42005-023-01236-7},
journal = {Communications Physics},
number = 1,
volume = 6,
place = {United States},
year = {Tue May 23 00:00:00 EDT 2023},
month = {Tue May 23 00:00:00 EDT 2023}
}
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