Ice rule fragility via topological charge transfer in artificial colloidal ice

Libál, András; Lee, Dong Yun; Ortiz-Ambriz, Antonio; Reichhardt, Charles; Reichhardt, Cynthia J.  O.; Tierno, Pietro; Nisoli, Cristiano

doi:10.1038/s41467-018-06631-1

Title: Ice rule fragility via topological charge transfer in artificial colloidal ice

Journal Article · 08 October 2018 · Nature Communications

DOI: https://doi.org/10.1038/s41467-018-06631-1 · OSTI ID:1479943

Libál, András ^[1]; Lee, Dong Yun ^[2];

^[2]; Reichhardt, Charles ^[3]; Reichhardt, Cynthia J. O. ^[3];

^[2];

^[3]

Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Babeş-Bolyai University, Cluj (Romania)
Universitat de Barcelona (Spain)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Artificial particle ices are model systems of constrained, interacting particles. They have been introduced theoretically to study ice-manifolds emergent from frustration, along with domain wall and grain boundary dynamics, doping, pinning-depinning, controlled transport of topological defects, avalanches, and memory effects. Recently such particle-based ices have been experimentally realized with vortices in nano-patterned superconductors or gravitationally trapped colloids. Here we demonstrate that, although these ices are generally considered equivalent to magnetic spin ices, they can access a novel spectrum of phenomenologies that are inaccessible to the latter. With experiments, theory and simulations we demonstrate that in mixed coordination geometries, entropy-driven negative monopoles spontaneously appear at a density determined by the vertex-mixture ratio. Unlike its spin-based analogue, the colloidal system displays a “fragile ice” manifold, where local energetics oppose the ice rule, which is instead enforced through conservation of the global topological charge. The fragile colloidal ice, stabilized by topology, can be spontaneously broken by topological charge transfer.

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Research Organization:: Los Alamos National Laboratory (LANL)

Sponsoring Organization:: Laboratory Directed Research and Development (LDRD); USDOE

Grant/Contract Number:: AC52-06NA25396

OSTI ID:: 1479943

Report Number(s):: LA-UR-18-29641

Journal Information:: Nature Communications, Journal Name: Nature Communications Journal Issue: 1 Vol. 9; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Dimer Covering and Percolation Frustration Haji-Akbari, Amir; Haji-Akbari, Nasim; Ziff, Robert M. arXiv https://doi.org/10.48550/arxiv.1507.04411	text	January 2015
Realizing Colloidal Artificial Ice on Arrays of Optical Traps Libal, A.; Reichhardt, C.; Reichhardt, C. J. Olson arXiv https://doi.org/10.48550/arxiv.cond-mat/0603265	text	January 2006

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Competing orders in colloidal kagome ice: Importance of the in-trap motion of the particles Le Cunuder, Anne; Frérot, Irénée; Ortiz-Ambriz, Antonio Physical Review B, Vol. 99, Issue 14 https://doi.org/10.1103/physrevb.99.140405	journal	April 2019
Colloquium : Ice rule and emergent frustration in particle ice and beyond Ortiz-Ambriz, Antonio; Nisoli, Cristiano; Reichhardt, Charles Reviews of Modern Physics, Vol. 91, Issue 4 https://doi.org/10.1103/revmodphys.91.041003	journal	December 2019

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