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Title: Topological spin memory of antiferromagnetically coupled skyrmion pairs in Co/Gd/Pt multilayers

Abstract

Antiferromagnetically (AFM) coupled skyrmions offer potential advantages for spintronic devices, including reduced dipolar fields that may enable smaller skyrmion sizes and a reduction of the skyrmion Hall effect. However, the topological stability of AFM-coupled skyrmions subjected to dramatic spin deformation through low-temperature cycling has not been investigated. We report the discovery of a topological spin memory effect for AFM-coupled skyrmion pairs in [Co/Gd/Pt](10) multilayered films. Photoemission electron microscopy imaging shows that bubble skyrmions in the multilayer that are stable at room temperature evolve into complex in-plane spin textures as the temperature is lowered and reform completely when the sample is warmed back up. Simulations demonstrate that Dzyaloshinskii-Moriya interactions play a key role in this spin memory effect, and furthermore reveal that the topological charge is preserved throughout the dramatic spin texture rearrangement and recovery. These results highlight a key aspect of topological protection-the preservation of the topological properties under continuous deformation-and also provide a promising avenue for information encryption and recovery.

Authors:
ORCiD logo [1];  [2];  [2];  [2]; ORCiD logo [1];  [3]; ORCiD logo [4];  [5]; ORCiD logo [6];  [7];  [7];  [5]; ORCiD logo [5]; ORCiD logo [5]; ORCiD logo [8]; ORCiD logo [2]; ORCiD logo [1]
  1. Bryn Mawr College, PA (United States)
  2. Colorado State University, Fort Collins, CO (United States)
  3. Bryn Mawr College, PA (United States); Colorado State University, Fort Collins, CO (United States)
  4. Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
  5. Argonne National Laboratory (ANL), Argonne, IL (United States)
  6. Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS); University of California, Los Angeles, CA (United States)
  7. Argonne National Laboratory (ANL), Argonne, IL (United States). Advanced Photon Source (APS)
  8. Argonne National Laboratory (ANL), Argonne, IL (United States); University of Illinois at Urbana-Champaign, IL (United States)
Publication Date:
Research Org.:
Argonne National Laboratory (ANL), Argonne, IL (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE); National Science Foundation (NSF)
OSTI Identifier:
1909622
Grant/Contract Number:  
AC02-06CH11357; AC02-05CH11231; DMR 1708790; DMR 1709525
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review Materials
Additional Journal Information:
Journal Volume: 6; Journal Issue: 8; Journal ID: ISSN 2475-9953
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Dzyaloshinskii-Moriya interaction; skyrmions; spin texture; synthetic antiferromagnetic multilayers; micromagnetic modeling; x-ray magnetic circular dichroism; x-ray photoemission electron microscopy

Citation Formats

Wang, Xiao, Stuart, Alexandra R., Swyt, Mitchell S., Flores, Carla M. Quispe, Clark, Andy T., Fiagbenu, Adzo, Chopdekar, Rajesh V., Lapa, Pavel N., Xiao, Zhuyun, Keavney, Dava, Rosenberg, Richard, Vogel, Michael, Pearson, John E., Velthuis, Suzanne G. E. te, Hoffmann, Axel, Buchanan, Kristen S., and Cheng, Xuemei M. Topological spin memory of antiferromagnetically coupled skyrmion pairs in Co/Gd/Pt multilayers. United States: N. p., 2022. Web. doi:10.1103/physrevmaterials.6.084412.
Wang, Xiao, Stuart, Alexandra R., Swyt, Mitchell S., Flores, Carla M. Quispe, Clark, Andy T., Fiagbenu, Adzo, Chopdekar, Rajesh V., Lapa, Pavel N., Xiao, Zhuyun, Keavney, Dava, Rosenberg, Richard, Vogel, Michael, Pearson, John E., Velthuis, Suzanne G. E. te, Hoffmann, Axel, Buchanan, Kristen S., & Cheng, Xuemei M. Topological spin memory of antiferromagnetically coupled skyrmion pairs in Co/Gd/Pt multilayers. United States. https://doi.org/10.1103/physrevmaterials.6.084412
Wang, Xiao, Stuart, Alexandra R., Swyt, Mitchell S., Flores, Carla M. Quispe, Clark, Andy T., Fiagbenu, Adzo, Chopdekar, Rajesh V., Lapa, Pavel N., Xiao, Zhuyun, Keavney, Dava, Rosenberg, Richard, Vogel, Michael, Pearson, John E., Velthuis, Suzanne G. E. te, Hoffmann, Axel, Buchanan, Kristen S., and Cheng, Xuemei M. Tue . "Topological spin memory of antiferromagnetically coupled skyrmion pairs in Co/Gd/Pt multilayers". United States. https://doi.org/10.1103/physrevmaterials.6.084412. https://www.osti.gov/servlets/purl/1909622.
@article{osti_1909622,
title = {Topological spin memory of antiferromagnetically coupled skyrmion pairs in Co/Gd/Pt multilayers},
author = {Wang, Xiao and Stuart, Alexandra R. and Swyt, Mitchell S. and Flores, Carla M. Quispe and Clark, Andy T. and Fiagbenu, Adzo and Chopdekar, Rajesh V. and Lapa, Pavel N. and Xiao, Zhuyun and Keavney, Dava and Rosenberg, Richard and Vogel, Michael and Pearson, John E. and Velthuis, Suzanne G. E. te and Hoffmann, Axel and Buchanan, Kristen S. and Cheng, Xuemei M.},
abstractNote = {Antiferromagnetically (AFM) coupled skyrmions offer potential advantages for spintronic devices, including reduced dipolar fields that may enable smaller skyrmion sizes and a reduction of the skyrmion Hall effect. However, the topological stability of AFM-coupled skyrmions subjected to dramatic spin deformation through low-temperature cycling has not been investigated. We report the discovery of a topological spin memory effect for AFM-coupled skyrmion pairs in [Co/Gd/Pt](10) multilayered films. Photoemission electron microscopy imaging shows that bubble skyrmions in the multilayer that are stable at room temperature evolve into complex in-plane spin textures as the temperature is lowered and reform completely when the sample is warmed back up. Simulations demonstrate that Dzyaloshinskii-Moriya interactions play a key role in this spin memory effect, and furthermore reveal that the topological charge is preserved throughout the dramatic spin texture rearrangement and recovery. These results highlight a key aspect of topological protection-the preservation of the topological properties under continuous deformation-and also provide a promising avenue for information encryption and recovery.},
doi = {10.1103/physrevmaterials.6.084412},
journal = {Physical Review Materials},
number = 8,
volume = 6,
place = {United States},
year = {Tue Aug 30 00:00:00 EDT 2022},
month = {Tue Aug 30 00:00:00 EDT 2022}
}

Works referenced in this record:

Current-driven dynamics and inhibition of the skyrmion Hall effect of ferrimagnetic skyrmions in GdFeCo films
journal, March 2018


Direct Demonstration of Topological Stability of Magnetic Skyrmions via Topology Manipulation
journal, March 2020


Controlling Dzyaloshinskii-Moriya Interaction via Chirality Dependent Atomic-Layer Stacking, Insulator Capping and Electric Field
journal, August 2018


Evolution of topological skyrmions across the spin reorientation transition in Pt/Co/Ta multilayers
journal, May 2018


A thermodynamic theory of “weak” ferromagnetism of antiferromagnetics
journal, January 1958


Experimental Confirmation of the X-Ray Magnetic Circular Dichroism Sum Rules for Iron and Cobalt
journal, July 1995


Evolution of Zero-Field Ferrimagnetic Domains and Skyrmions in Exchange-Coupled Pt/CoGd/Pt Confined Nanostructures: Implications for Antiferromagnetic Devices
journal, November 2019

  • Brandão, J.; Dugato, D. A.; Puydinger dos Santos, M. V.
  • ACS Applied Nano Materials, Vol. 2, Issue 12
  • DOI: 10.1021/acsanm.9b01593

Room-temperature chiral magnetic skyrmions in ultrathin magnetic nanostructures
journal, January 2016

  • Boulle, Olivier; Vogel, Jan; Yang, Hongxin
  • Nature Nanotechnology, Vol. 11, Issue 5
  • DOI: 10.1038/nnano.2015.315

Antiferromagnetic spintronics
journal, February 2018


Path to collapse for an isolated Néel skyrmion
journal, June 2016


Anatomy of Dzyaloshinskii-Moriya Interaction at Co / Pt Interfaces
journal, December 2015


The design and verification of MuMax3
journal, October 2014

  • Vansteenkiste, Arne; Leliaert, Jonathan; Dvornik, Mykola
  • AIP Advances, Vol. 4, Issue 10
  • DOI: 10.1063/1.4899186

Magnetic bilayer-skyrmions without skyrmion Hall effect
journal, January 2016

  • Zhang, Xichao; Zhou, Yan; Ezawa, Motohiko
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms10293

Studies of nanomagnetism using synchrotron-based x-ray photoemission electron microscopy (X-PEEM)
journal, January 2012


Linear relation between Heisenberg exchange and interfacial Dzyaloshinskii–Moriya interaction in metal films
journal, August 2015

  • Nembach, Hans T.; Shaw, Justin M.; Weiler, Mathias
  • Nature Physics, Vol. 11, Issue 10
  • DOI: 10.1038/nphys3418

Very large domain wall velocities in Pt/Co/GdOx and Pt/Co/Gd trilayers with Dzyaloshinskii-Moriya interaction
journal, March 2016


Magnetic anisotropy in Gd/(FeCo) and Gd/Fe multilayers for high density magneto-optical recording
journal, April 1999

  • Stavrou, E.; Röll, K.
  • Journal of Applied Physics, Vol. 85, Issue 8
  • DOI: 10.1063/1.370008

Observation of room-temperature magnetic skyrmions and their current-driven dynamics in ultrathin metallic ferromagnets
journal, February 2016

  • Woo, Seonghoon; Litzius, Kai; Krüger, Benjamin
  • Nature Materials, Vol. 15, Issue 5
  • DOI: 10.1038/nmat4593

Electron-yield saturation effects in L -edge x-ray magnetic circular dichroism spectra of Fe, Co, and Ni
journal, March 1999


On the induced cobalt moments in (GdxY1−x)Co3 compounds
journal, February 1981


Generation and Hall effect of skyrmions enabled using nonmagnetic point contacts
journal, November 2019


X-ray circular dichroism and local magnetic fields
journal, February 1993


Tailoring Curie temperature and magnetic anisotropy in ultrathin Pt/Co/Pt films
journal, May 2016

  • Parakkat, Vineeth Mohanan; Ganesh, K. R.; Anil Kumar, P. S.
  • AIP Advances, Vol. 6, Issue 5
  • DOI: 10.1063/1.4944343

Exchange coupling torque in ferrimagnetic Co/Gd bilayer maximized near angular momentum compensation temperature
journal, November 2018


Magnetic and structural properties of Co/Pt multilayers
journal, February 1991


Indirect exchange for rare earths in metals
journal, May 1972


Inverted and biased loops in amorphous Gd-Co films
journal, September 1977


Fast current-driven domain walls and small skyrmions in a compensated ferrimagnet
journal, September 2018


Interfacial Dzyaloshinskii-Moriya interaction in perpendicularly magnetized Pt/Co/AlO x ultrathin films measured by Brillouin light spectroscopy
journal, May 2015


Skyrmion–Anti-Skyrmion Pair Creation by in-Plane Currents
journal, June 2017


Anisotropic Superexchange Interaction and Weak Ferromagnetism
journal, October 1960


Room-Temperature Current-Induced Generation and Motion of sub-100 nm Skyrmions
journal, March 2017


Experimental Evidence of Chiral Ferrimagnetism in Amorphous GdCo Films
journal, May 2018

  • Streubel, Robert; Lambert, Charles-Henri; Kent, Noah
  • Advanced Materials, Vol. 30, Issue 27
  • DOI: 10.1002/adma.201800199

Spin-wave propagation in the presence of interfacial Dzyaloshinskii-Moriya interaction
journal, November 2013


Room-temperature stabilization of antiferromagnetic skyrmions in synthetic antiferromagnets
journal, September 2019


The probing depth of total electron yield in the sub-keV range: TEY-XAS and X-PEEM
journal, July 2003


Fabrication of Ferrimagnetic Co/Gd/Pt Multilayers with Structural Inversion Symmetry Breaking
journal, January 2020

  • Nishimura, T.; Haruta, M.; Kim, D. -H.
  • Journal of the Magnetics Society of Japan, Vol. 44, Issue 1
  • DOI: 10.3379/msjmag.2001R002

X-ray spectro-microscopy of complex materials and surfaces
journal, July 2000

  • Stohr, J.; Anders, S.
  • IBM Journal of Research and Development, Vol. 44, Issue 4
  • DOI: 10.1147/rd.444.0535

X-ray circular dichroism as a probe of orbital magnetization
journal, March 1992


Blowing magnetic skyrmion bubbles
journal, June 2015


Formation and current-induced motion of synthetic antiferromagnetic skyrmion bubbles
journal, November 2019


Magnetic anisotropy and spin reorientation effects in Gd/Fe and Gd/(FeCo) multilayers for high density magneto-optical recording
journal, May 2000

  • Stavrou, E.; Sbiaa, R.; Suzuki, T.
  • Journal of Applied Physics, Vol. 87, Issue 9
  • DOI: 10.1063/1.372879

Direct observation of the skyrmion Hall effect
journal, September 2016

  • Jiang, Wanjun; Zhang, Xichao; Yu, Guoqiang
  • Nature Physics, Vol. 13, Issue 2
  • DOI: 10.1038/nphys3883

Experimental study of spin-wave dispersion in Py/Pt film structures in the presence of an interface Dzyaloshinskii-Moriya interaction
journal, June 2015


Static and Dynamical Properties of Antiferromagnetic Skyrmions in the Presence of Applied Current and Temperature
journal, April 2016


Topological charge analysis of ultrafast single skyrmion creation
journal, May 2016


Realization of ground-state artificial skyrmion lattices at room temperature
journal, October 2015

  • Gilbert, Dustin A.; Maranville, Brian B.; Balk, Andrew L.
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms9462