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Title: Optical-Resonance-Enhanced Photoemission from Nanostructured GaAs Photocathodes

Abstract

A negative electron affinity photocathode based on GaAs nanopillar-array (NPA) Mie-type resonators is demonstrated and significant quantum efficiency enhancement is observed. Nanophotonic resonance assisted photoelectron emission into vacuum is investigated, indicating an enhanced density of optical states due to increased light concentration and increased electron emission area. For visible wavelengths, the Mie resonances in GaAs NPA reduce light reflectivity to less than 6% compared to a typical value >35% and result in maximum quantum efficiency 3.5 times greater than a GaAs wafer photocathode without the NPA structure. In conclusion, comprehensive simulations and experimental studies are presented.

Authors:
ORCiD logo [1];  [2];  [2];  [3];  [4];  [4];  [2];  [4];  [5]
  1. East China Univ. of Technology, Nanchang (China). Engineering Research Center of New Energy Technology of Jiangxi Province; Thomas Jefferson National Accelerator Facility (TJNAF), Newport News, VA (United States)
  2. East China Univ. of Technology, Nanchang (China). Engineering Research Center of New Energy Technology of Jiangxi Province
  3. College of William and Mary, Williamsburg, VA (United States)
  4. Thomas Jefferson National Accelerator Facility (TJNAF), Newport News, VA (United States)
  5. East China Univ. of Technology, Nanchang (China). Engineering Research Center of New Energy Technology of Jiangxi Province; Thomas Jefferson National Accelerator Facility (TJNAF), Newport News, VA (United States); College of William and Mary, Williamsburg, VA (United States)
Publication Date:
Research Org.:
Thomas Jefferson National Accelerator Facility (TJNAF), Newport News, VA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1577074
Report Number(s):
JLAB-ACC-19-3042; DOE/OR/23177-4781
Journal ID: ISSN 2331-7019; PRAHB2; TRN: US2102131
Grant/Contract Number:  
11875012; 61204071; 61661002
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review Applied
Additional Journal Information:
Journal Volume: 12; Journal Issue: 6; Journal ID: ISSN 2331-7019
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS

Citation Formats

Peng, Xincun, Wang, Zhidong, Liu, Yun, Manos, Dennis M., Poelker, Matt, Stutzman, Marcy, Tang, Bin, Zhang, Shukui, and Zou, Jijun. Optical-Resonance-Enhanced Photoemission from Nanostructured GaAs Photocathodes. United States: N. p., 2019. Web. doi:10.1103/PhysRevApplied.12.064002.
Peng, Xincun, Wang, Zhidong, Liu, Yun, Manos, Dennis M., Poelker, Matt, Stutzman, Marcy, Tang, Bin, Zhang, Shukui, & Zou, Jijun. Optical-Resonance-Enhanced Photoemission from Nanostructured GaAs Photocathodes. United States. https://doi.org/10.1103/PhysRevApplied.12.064002
Peng, Xincun, Wang, Zhidong, Liu, Yun, Manos, Dennis M., Poelker, Matt, Stutzman, Marcy, Tang, Bin, Zhang, Shukui, and Zou, Jijun. Mon . "Optical-Resonance-Enhanced Photoemission from Nanostructured GaAs Photocathodes". United States. https://doi.org/10.1103/PhysRevApplied.12.064002. https://www.osti.gov/servlets/purl/1577074.
@article{osti_1577074,
title = {Optical-Resonance-Enhanced Photoemission from Nanostructured GaAs Photocathodes},
author = {Peng, Xincun and Wang, Zhidong and Liu, Yun and Manos, Dennis M. and Poelker, Matt and Stutzman, Marcy and Tang, Bin and Zhang, Shukui and Zou, Jijun},
abstractNote = {A negative electron affinity photocathode based on GaAs nanopillar-array (NPA) Mie-type resonators is demonstrated and significant quantum efficiency enhancement is observed. Nanophotonic resonance assisted photoelectron emission into vacuum is investigated, indicating an enhanced density of optical states due to increased light concentration and increased electron emission area. For visible wavelengths, the Mie resonances in GaAs NPA reduce light reflectivity to less than 6% compared to a typical value >35% and result in maximum quantum efficiency 3.5 times greater than a GaAs wafer photocathode without the NPA structure. In conclusion, comprehensive simulations and experimental studies are presented.},
doi = {10.1103/PhysRevApplied.12.064002},
journal = {Physical Review Applied},
number = 6,
volume = 12,
place = {United States},
year = {Mon Dec 02 00:00:00 EST 2019},
month = {Mon Dec 02 00:00:00 EST 2019}
}

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Works referenced in this record:

Ultrabright and Ultrafast III–V Semiconductor Photocathodes
journal, March 2014


Patterned negative electron affinity photocathodes for maskless electron beam lithography
journal, November 1998

  • Schneider, J. E.
  • Journal of Vacuum Science & Technology B: Microelectronics and Nanometer Structures, Vol. 16, Issue 6
  • DOI: 10.1116/1.590349

Effect of crystal quality on performance of spin-polarized photocathode
journal, November 2014

  • Jin, Xiuguang; Ozdol, Burak; Yamamoto, Masahiro
  • Applied Physics Letters, Vol. 105, Issue 20
  • DOI: 10.1063/1.4902337

Resolution characteristics of graded doping and graded composition transmission-mode AlGaAs/GaAs photocathodes
journal, January 2015

  • Deng, Wenjuan; Zou, Jijun; Peng, Xincun
  • Applied Optics, Vol. 54, Issue 6
  • DOI: 10.1364/AO.54.001414

Single-nanowire solar cells beyond the Shockley–Queisser limit
journal, March 2013

  • Krogstrup, Peter; Jørgensen, Henrik Ingerslev; Heiss, Martin
  • Nature Photonics, Vol. 7, Issue 4
  • DOI: 10.1038/nphoton.2013.32

Negative affinity 3–5 photocathodes: Their physics and technology
journal, February 1977


NEA surface activation of GaAs photocathode with different gases
journal, October 2017


Semiconductor Nanowire Optical Antenna Solar Absorbers
journal, February 2010

  • Cao, Linyou; Fan, Pengyu; Vasudev, Alok P.
  • Nano Letters, Vol. 10, Issue 2
  • DOI: 10.1021/nl9036627

Optimization of substrate conformal imprint lithography (SCIL) and etching for nanostructure
journal, April 2015

  • Geng, Zhaoxin; Guo, Xiangbin; Kan, Qiang
  • AIP Advances, Vol. 5, Issue 4
  • DOI: 10.1063/1.4904061

Plasmoelectric potentials in metal nanostructures
journal, October 2014


Silicon Mie resonators for highly directional light emission from monolayer MoS2
journal, April 2018


Optically resonant dielectric nanostructures
journal, November 2016

  • Kuznetsov, Arseniy I.; Miroshnichenko, Andrey E.; Brongersma, Mark L.
  • Science, Vol. 354, Issue 6314
  • DOI: 10.1126/science.aag2472

Analysis of quantum efficiency improvement in spin-polarized photocathode
journal, October 2016

  • Jin, Xiuguang; Ohki, Shunsuke; Ishikawa, Tomoki
  • Journal of Applied Physics, Vol. 120, Issue 16
  • DOI: 10.1063/1.4965723

First Lasing of the CAEP THz FEL facility Driven by a Superconducting Accelerator
journal, September 2018


Improved activation technique for preparing high-efficiency GaAs photocathodes
journal, January 2017

  • Zhang, Yijun; Qian, Yunsheng; Feng, Cheng
  • Optical Materials Express, Vol. 7, Issue 9
  • DOI: 10.1364/OME.7.003456

Theoretical analysis and modeling of light trapping in high efficicency GaAs nanowire array solar cells
journal, October 2011

  • Wen, Long; Zhao, Zhifei; Li, Xinhua
  • Applied Physics Letters, Vol. 99, Issue 14
  • DOI: 10.1063/1.3647847

Charge and fluence lifetime measurements of a dc high voltage GaAs photogun at high average current
journal, April 2011

  • Grames, J.; Suleiman, R.; Adderley, P. A.
  • Physical Review Special Topics - Accelerators and Beams, Vol. 14, Issue 4
  • DOI: 10.1103/PhysRevSTAB.14.043501

Energy distributions of electrons emitted from reflection-mode Cs-covered GaAs photocathodes
journal, January 2012

  • Zou, Jijun; Zhang, Yijun; Peng, Xincun
  • Applied Optics, Vol. 51, Issue 31
  • DOI: 10.1364/AO.51.007662

Rugged spin-polarized electron sources based on negative electron affinity GaAs photocathode with robust Cs 2 Te coating
journal, April 2018

  • Bae, Jai Kwan; Cultrera, Luca; DiGiacomo, Philip
  • Applied Physics Letters, Vol. 112, Issue 15
  • DOI: 10.1063/1.5026701

Variation of quantum-yield curves for GaAs photocathodes under illumination
journal, February 2007

  • Zou, Jijun; Chang, Benkang; Chen, Huailin
  • Journal of Applied Physics, Vol. 101, Issue 3
  • DOI: 10.1063/1.2435075

All-dielectric metamaterials
journal, January 2016


Production of Highly Polarized Positrons Using Polarized Electrons at MeV Energies
journal, May 2016


Spectral sensitivity of graded composition AlGaAs/GaAs nanowire photodetectors
journal, November 2016


The surface activation layer of GaAs negative electron affinity photocathode activated by Cs, Li, and NF3
journal, October 2009

  • Sun, Y.; Kirby, R. E.; Maruyama, T.
  • Applied Physics Letters, Vol. 95, Issue 17
  • DOI: 10.1063/1.3257730

Designing dielectric resonators on substrates: Combining magnetic and electric resonances
journal, January 2013


Effects of ion bombardment on bulk GaAs photocathodes with different surface-cleavage planes
journal, October 2016


Observation and measurement of temperature rise and distribution on GaAs photo-cathode wafer with a 532nm drive laser and a thermal imaging camera
journal, March 2011

  • Zhang, S.; Benson, S. V.; H-Garcia, C.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 631, Issue 1
  • DOI: 10.1016/j.nima.2010.12.132

Negative electron affinity GaAs wire-array photocathodes
journal, January 2016


High-quantum-efficiency ultraviolet solar-blind AlGaN photocathode detector with a sharp spectral sensitivity threshold at 300  nm
journal, January 2018

  • Tang, Guanghua; Yan, Feng; Chen, Xinlong
  • Applied Optics, Vol. 57, Issue 27
  • DOI: 10.1364/AO.57.008060

Evolution of surface potential barrier for negative-electron-affinity GaAs photocathodes
journal, January 2009

  • Zou, Jijun; Chang, Benkang; Yang, Zhi
  • Journal of Applied Physics, Vol. 105, Issue 1
  • DOI: 10.1063/1.3063686

Record-level quantum efficiency from a high polarization strained GaAs/GaAsP superlattice photocathode with distributed Bragg reflector
journal, December 2016

  • Liu, Wei; Chen, Yiqiao; Lu, Wentao
  • Applied Physics Letters, Vol. 109, Issue 25
  • DOI: 10.1063/1.4972180

Broadband Quantum Efficiency Enhancement in High Index Nanowire Resonators
journal, April 2015


Single nanowire solar cells beyond the Shockley-Queisser limit
text, January 2013