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Title: Mie-type GaAs nanopillar array resonators for negative electron affinity photocathodes

Abstract

This paper presents modeling results of Mie-type GaAs nanopillar array resonant structures and the design of negative electron affinity photocathodes based on Spicer’s three-step model. For direct-bandgap GaAs with high intrinsic absorption coefficient in the 500 ∼ 850 nm spectral range, photoelectrons were found to be highly localized inside the nanopillars near the top and side surfaces where electrons can be efficiently transported and emitted into vacuum, and the light reflectance can be reduced to ∼1% level at resonance wavelengths. Predictions of spectrally resolved photoemission indicate that these nanophotonics resonators, when properly optimized, can increase the photo-electron emission quantum efficiency at resonance wavelengths to levels limited only by the surface-electron escape probability, significantly outperforming traditional flat wafer photocathodes. Ultrafast photoelectric response is also expected from these nanostructured photocathodes due to the much shorter photoelectron transport distance in nanopillars compared to flat wafers. Given these unique optoelectronic properties, GaAs nanophotonic resonance structured photocathodes represent a very promising alternative to photocathodes with flat surfaces that are widely used in many applications today.

Authors:
ORCiD logo; ; ; ; ;
Publication Date:
Research Org.:
Thomas Jefferson National Accelerator Facility (TJNAF), Newport News, VA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Nuclear Physics (NP); National Natural Science Foundation of China (NSFC)
OSTI Identifier:
1581217
Alternate Identifier(s):
OSTI ID: 1607854
Report Number(s):
JLAB-ACC-19-3144; DOE/OR/23177-4952
Journal ID: ISSN 1094-4087; OPEXFF
Grant/Contract Number:  
AC05-06OR23177; 11875012; 61204071; 61661002
Resource Type:
Published Article
Journal Name:
Optics Express
Additional Journal Information:
Journal Name: Optics Express Journal Volume: 28 Journal Issue: 2; Journal ID: ISSN 1094-4087
Publisher:
Optical Society of America
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION

Citation Formats

Peng, Xincun, Poelker, Matt, Stutzman, Marcy, Tang, Bin, Zhang, Shukui, and Zou, Jijun. Mie-type GaAs nanopillar array resonators for negative electron affinity photocathodes. United States: N. p., 2020. Web. doi:10.1364/OE.378194.
Peng, Xincun, Poelker, Matt, Stutzman, Marcy, Tang, Bin, Zhang, Shukui, & Zou, Jijun. Mie-type GaAs nanopillar array resonators for negative electron affinity photocathodes. United States. https://doi.org/10.1364/OE.378194
Peng, Xincun, Poelker, Matt, Stutzman, Marcy, Tang, Bin, Zhang, Shukui, and Zou, Jijun. Mon . "Mie-type GaAs nanopillar array resonators for negative electron affinity photocathodes". United States. https://doi.org/10.1364/OE.378194.
@article{osti_1581217,
title = {Mie-type GaAs nanopillar array resonators for negative electron affinity photocathodes},
author = {Peng, Xincun and Poelker, Matt and Stutzman, Marcy and Tang, Bin and Zhang, Shukui and Zou, Jijun},
abstractNote = {This paper presents modeling results of Mie-type GaAs nanopillar array resonant structures and the design of negative electron affinity photocathodes based on Spicer’s three-step model. For direct-bandgap GaAs with high intrinsic absorption coefficient in the 500 ∼ 850 nm spectral range, photoelectrons were found to be highly localized inside the nanopillars near the top and side surfaces where electrons can be efficiently transported and emitted into vacuum, and the light reflectance can be reduced to ∼1% level at resonance wavelengths. Predictions of spectrally resolved photoemission indicate that these nanophotonics resonators, when properly optimized, can increase the photo-electron emission quantum efficiency at resonance wavelengths to levels limited only by the surface-electron escape probability, significantly outperforming traditional flat wafer photocathodes. Ultrafast photoelectric response is also expected from these nanostructured photocathodes due to the much shorter photoelectron transport distance in nanopillars compared to flat wafers. Given these unique optoelectronic properties, GaAs nanophotonic resonance structured photocathodes represent a very promising alternative to photocathodes with flat surfaces that are widely used in many applications today.},
doi = {10.1364/OE.378194},
journal = {Optics Express},
number = 2,
volume = 28,
place = {United States},
year = {Mon Jan 06 00:00:00 EST 2020},
month = {Mon Jan 06 00:00:00 EST 2020}
}

Journal Article:
Free Publicly Available Full Text
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https://doi.org/10.1364/OE.378194

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Cited by: 12 works
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Works referenced in this record:

High voltage studies of inverted-geometry ceramic insulators for a 350 kV DC polarized electron gun
journal, February 2016

  • Hernandez-Garcia, C.; Poelker, M.; Hansknecht, J.
  • IEEE Transactions on Dielectrics and Electrical Insulation, Vol. 23, Issue 1
  • DOI: 10.1109/TDEI.2015.005126

Ultrabright and Ultrafast III–V Semiconductor Photocathodes
journal, March 2014


Patterned negative electron affinity photocathodes for maskless electron beam lithography
journal, November 1998

  • Schneider, J. E.
  • Journal of Vacuum Science & Technology B: Microelectronics and Nanometer Structures, Vol. 16, Issue 6
  • DOI: 10.1116/1.590349

Effect of crystal quality on performance of spin-polarized photocathode
journal, November 2014

  • Jin, Xiuguang; Ozdol, Burak; Yamamoto, Masahiro
  • Applied Physics Letters, Vol. 105, Issue 20
  • DOI: 10.1063/1.4902337

GaAs nanopillar-array solar cells employing in situ surface passivation
journal, February 2013

  • Mariani, Giacomo; Scofield, Adam C.; Hung, Chung-Hong
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms2509

Image intensification
journal, March 2010


Single-nanowire solar cells beyond the Shockley–Queisser limit
journal, March 2013

  • Krogstrup, Peter; Jørgensen, Henrik Ingerslev; Heiss, Martin
  • Nature Photonics, Vol. 7, Issue 4
  • DOI: 10.1038/nphoton.2013.32

Direct-Bandgap Epitaxial Core–Multishell Nanopillar Photovoltaics Featuring Subwavelength Optical Concentrators
journal, March 2013

  • Mariani, Giacomo; Zhou, Zhengliu; Scofield, Adam
  • Nano Letters, Vol. 13, Issue 4
  • DOI: 10.1021/nl400083g

Negative affinity 3–5 photocathodes: Their physics and technology
journal, February 1977


Empirical low-field mobility model for III–V compounds applicable in device simulation codes
journal, March 2000

  • Sotoodeh, M.; Khalid, A. H.; Rezazadeh, A. A.
  • Journal of Applied Physics, Vol. 87, Issue 6
  • DOI: 10.1063/1.372274

Semiconductor Nanowire Optical Antenna Solar Absorbers
journal, February 2010

  • Cao, Linyou; Fan, Pengyu; Vasudev, Alok P.
  • Nano Letters, Vol. 10, Issue 2
  • DOI: 10.1021/nl9036627

On optical properties of GaAs and GaAs/AlGaAs core-shell periodic nanowire arrays
journal, March 2011

  • Gu, Zongquan; Prete, Paola; Lovergine, Nicola
  • Journal of Applied Physics, Vol. 109, Issue 6
  • DOI: 10.1063/1.3555096

Broadband omnidirectional antireflection coating based on subwavelength surface Mie resonators
journal, January 2012

  • Spinelli, P.; Verschuuren, M. A.; Polman, A.
  • Nature Communications, Vol. 3, Issue 1
  • DOI: 10.1038/ncomms1691

Enhanced external quantum efficiency in rectangular single nanowire solar cells
journal, January 2013

  • Li, Xiaofeng; Zhan, Yaohui
  • Applied Physics Letters, Vol. 102, Issue 2
  • DOI: 10.1063/1.4775578

First Lasing of the CAEP THz FEL facility Driven by a Superconducting Accelerator
journal, September 2018


Optically resonant dielectric nanostructures
journal, November 2016

  • Kuznetsov, Arseniy I.; Miroshnichenko, Andrey E.; Brongersma, Mark L.
  • Science, Vol. 354, Issue 6314
  • DOI: 10.1126/science.aag2472

Meta-Optics with Mie Resonances
journal, January 2017


Analysis of quantum efficiency improvement in spin-polarized photocathode
journal, October 2016

  • Jin, Xiuguang; Ohki, Shunsuke; Ishikawa, Tomoki
  • Journal of Applied Physics, Vol. 120, Issue 16
  • DOI: 10.1063/1.4965723

Improved activation technique for preparing high-efficiency GaAs photocathodes
journal, January 2017

  • Zhang, Yijun; Qian, Yunsheng; Feng, Cheng
  • Optical Materials Express, Vol. 7, Issue 9
  • DOI: 10.1364/OME.7.003456

Theoretical analysis and modeling of light trapping in high efficicency GaAs nanowire array solar cells
journal, October 2011

  • Wen, Long; Zhao, Zhifei; Li, Xinhua
  • Applied Physics Letters, Vol. 99, Issue 14
  • DOI: 10.1063/1.3647847

Maximum intensity, transmission limited cold electron beams from GaAs photocathode in the eV and sub-eV kinetic energy range
journal, March 2014

  • Shornikov, A.; Orlov, D. A.; Krantz, C.
  • Physical Review Special Topics - Accelerators and Beams, Vol. 17, Issue 4
  • DOI: 10.1103/PhysRevSTAB.17.042802

Variation of quantum-yield curves for GaAs photocathodes under illumination
journal, February 2007

  • Zou, Jijun; Chang, Benkang; Chen, Huailin
  • Journal of Applied Physics, Vol. 101, Issue 3
  • DOI: 10.1063/1.2435075

Photoemission from advanced heterostructured Al_xGa_1-xAs/GaAs photocathodes under multilevel built-in electric field
journal, January 2015

  • Feng, Cheng; Zhang, Yijun; Qian, Yunsheng
  • Optics Express, Vol. 23, Issue 15
  • DOI: 10.1364/OE.23.019478

All-dielectric metamaterials
journal, January 2016


Production of Highly Polarized Positrons Using Polarized Electrons at MeV Energies
journal, May 2016


Functional Meta-Optics and Nanophotonics Governed by Mie Resonances
journal, October 2017


Spectral sensitivity of graded composition AlGaAs/GaAs nanowire photodetectors
journal, November 2016


Photoemission characteristics of graded band-gap AlGaAs/GaAs wire photocathode
journal, May 2016


Absorption and Scattering of Light by Small Particles
book, April 1998


Improved quantum efficiency and stability of GaAs photocathode using favorable illumination during activation
journal, July 2019


Designing dielectric resonators on substrates: Combining magnetic and electric resonances
journal, January 2013


Efficient tool flow for 3D photovoltaic modelling
journal, August 2015


NEA photocathode for SEM application
journal, June 2003


Light-trapping in photon enhanced thermionic emitters
journal, January 2015

  • Buencuerpo, Jerónimo; Llorens, José M.; Zilio, Pierfrancesco
  • Optics Express, Vol. 23, Issue 19
  • DOI: 10.1364/OE.23.0A1220

Effects of ion bombardment on bulk GaAs photocathodes with different surface-cleavage planes
journal, October 2016


Negative electron affinity GaAs wire-array photocathodes
journal, January 2016


Monte Carlo charge transport and photoemission from negative electron affinity GaAs photocathodes
journal, March 2013

  • Karkare, Siddharth; Dimitrov, Dimitre; Schaff, William
  • Journal of Applied Physics, Vol. 113, Issue 10
  • DOI: 10.1063/1.4794822

MCP detector development for UV space missions
journal, March 2018

  • Conti, Lauro; Barnstedt, Jürgen; Hanke, Lars
  • Astrophysics and Space Science, Vol. 363, Issue 4
  • DOI: 10.1007/s10509-018-3283-4

High-quantum-efficiency ultraviolet solar-blind AlGaN photocathode detector with a sharp spectral sensitivity threshold at 300  nm
journal, January 2018

  • Tang, Guanghua; Yan, Feng; Chen, Xinlong
  • Applied Optics, Vol. 57, Issue 27
  • DOI: 10.1364/AO.57.008060

Photocathodes for High Brightness Photo Injectors
journal, January 2015


Record-level quantum efficiency from a high polarization strained GaAs/GaAsP superlattice photocathode with distributed Bragg reflector
journal, December 2016

  • Liu, Wei; Chen, Yiqiao; Lu, Wentao
  • Applied Physics Letters, Vol. 109, Issue 25
  • DOI: 10.1063/1.4972180

Broadband Quantum Efficiency Enhancement in High Index Nanowire Resonators
journal, April 2015