Continuous Flow Processing of ZIF-8 Membranes on Polymeric Porous Hollow Fiber Supports for CO2 Capture
Abstract
We have utilized an environmentally friendly synthesis approach for the accelerated growth of a selective inorganic membrane on a polymeric hollow fiber support for postcombustion carbon capture. Specifically, continuous defect-free ZIF-8 thin films were grown and anchored using continuous flow synthesis on the outer surface of porous supports using water as solvent. These membranes demonstrated CO2 permeance of 22 GPU and the highest reported CO2/N2 selectivity of 52 for a continuous flow synthesized ZIF-8 membrane.
- Authors:
-
- National Energy Technology Lab. (NETL), Pittsburgh, PA (United States); Oak Ridge Inst. for Science and Education (ORISE), Pittsburgh, PA (United States)
- National Energy Technology Lab. (NETL), Pittsburgh, PA (United States); Oak Ridge Inst. for Science and Education (ORISE), Pittsburgh, PA (United States)
- National Energy Technology Lab. (NETL), Pittsburgh, PA (United States); AECOM Pittsburgh, PA (United States)
- National Energy Technology Lab. (NETL), Pittsburgh, PA (United States)
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Center for Gas Separations Relevant to Clean Energy Technologies (CGS)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Fossil Energy (FE)
- OSTI Identifier:
- 1388091
- Grant/Contract Number:
- SC0001015
- Resource Type:
- Accepted Manuscript
- Journal Name:
- ACS Applied Materials and Interfaces
- Additional Journal Information:
- Journal Volume: 9; Journal Issue: 7; Related Information: CGS partners with University of California, Berkeley; University of California, Davis; Lawrence Berkeley National Laboratory; University of Minnesota; National Energy Technology Laboratory; Texas A&M University; Journal ID: ISSN 1944-8244
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; membrane; carbon capture; materials and chemistry by design; synthesis (novel materials); synthesis (self-assembly); synthesis (scalable processing)
Citation Formats
Marti, Anne M., Wickramanayake, Wasala, Dahe, Ganpat, Sekizkardes, Ali, Bank, Tracy L., Hopkinson, David P., and Venna, Surendar R. Continuous Flow Processing of ZIF-8 Membranes on Polymeric Porous Hollow Fiber Supports for CO2 Capture. United States: N. p., 2017.
Web. doi:10.1021/acsami.6b16297.
Marti, Anne M., Wickramanayake, Wasala, Dahe, Ganpat, Sekizkardes, Ali, Bank, Tracy L., Hopkinson, David P., & Venna, Surendar R. Continuous Flow Processing of ZIF-8 Membranes on Polymeric Porous Hollow Fiber Supports for CO2 Capture. United States. https://doi.org/10.1021/acsami.6b16297
Marti, Anne M., Wickramanayake, Wasala, Dahe, Ganpat, Sekizkardes, Ali, Bank, Tracy L., Hopkinson, David P., and Venna, Surendar R. Thu .
"Continuous Flow Processing of ZIF-8 Membranes on Polymeric Porous Hollow Fiber Supports for CO2 Capture". United States. https://doi.org/10.1021/acsami.6b16297. https://www.osti.gov/servlets/purl/1388091.
@article{osti_1388091,
title = {Continuous Flow Processing of ZIF-8 Membranes on Polymeric Porous Hollow Fiber Supports for CO2 Capture},
author = {Marti, Anne M. and Wickramanayake, Wasala and Dahe, Ganpat and Sekizkardes, Ali and Bank, Tracy L. and Hopkinson, David P. and Venna, Surendar R.},
abstractNote = {We have utilized an environmentally friendly synthesis approach for the accelerated growth of a selective inorganic membrane on a polymeric hollow fiber support for postcombustion carbon capture. Specifically, continuous defect-free ZIF-8 thin films were grown and anchored using continuous flow synthesis on the outer surface of porous supports using water as solvent. These membranes demonstrated CO2 permeance of 22 GPU and the highest reported CO2/N2 selectivity of 52 for a continuous flow synthesized ZIF-8 membrane.},
doi = {10.1021/acsami.6b16297},
journal = {ACS Applied Materials and Interfaces},
number = 7,
volume = 9,
place = {United States},
year = {Thu Feb 09 00:00:00 EST 2017},
month = {Thu Feb 09 00:00:00 EST 2017}
}
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