Production of extremely low volatile organic compounds from biogenic emissions: Measured yields and atmospheric implications
Abstract
Extremely low volatility organic compounds (ELVOC) are suggested to promote aerosol particle formation and cloud condensation nuclei (CCN) production in the atmosphere. We show that the capability of biogenic VOC (BVOC) to produce ELVOC depends strongly on their chemical structure and relative oxidant levels. BVOC with an endocyclic double bond, representative emissions from, e.g., boreal forests, efficiently produce ELVOC from ozonolysis. Compounds with exocyclic double bonds or acyclic compounds including isoprene, emission representative of the tropics, produce minor quantities of ELVOC, and the role of OH radical oxidation is relatively larger. Furthermore, implementing these findings into a global modeling framework shows that detailed assessment of ELVOC production pathways is crucial for understanding biogenic secondary organic aerosol and atmospheric CCN formation.
- Authors:
-
[3];
- Leibniz-Institut fur Tropospharenforschung (TROPOS), Leipzig (Germany); Univ. of Helsinki, Helsinki (Finland)
- Leibniz-Institut fur Tropospharenforschung (TROPOS), Leipzig (Germany)
- Univ. of Helsinki, Helsinki (Finland)
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Univ. of Helsinki, Helsinki (Finland); Aerodyne Research, Inc., Billerica, MA (United States)
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1221472
- Report Number(s):
- PNNL-SA-110673
Journal ID: ISSN 0027-8424
- Grant/Contract Number:
- AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Proceedings of the National Academy of Sciences of the United States of America
- Additional Journal Information:
- Journal Volume: 112; Journal Issue: 23; Journal ID: ISSN 0027-8424
- Publisher:
- National Academy of Sciences, Washington, DC (United States)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES; autoxidation; ELVOC; monoterpenes; isoprene; new particle formation
Citation Formats
Jokinen, Tuija, Berndt, Torsten, Makkonen, Risto, Kerminen, Veli-Matti, Junninen, Heikki, Paasonen, Pauli, Stratmann, Frank, Herrmann, Hartmut, Guenther, Alex B., Worsnop, Douglas R., Kulmala, Markku, Ehn, Mikael K., and Sipila, Mikko. Production of extremely low volatile organic compounds from biogenic emissions: Measured yields and atmospheric implications. United States: N. p., 2015.
Web. doi:10.1073/pnas.1423977112.
Jokinen, Tuija, Berndt, Torsten, Makkonen, Risto, Kerminen, Veli-Matti, Junninen, Heikki, Paasonen, Pauli, Stratmann, Frank, Herrmann, Hartmut, Guenther, Alex B., Worsnop, Douglas R., Kulmala, Markku, Ehn, Mikael K., & Sipila, Mikko. Production of extremely low volatile organic compounds from biogenic emissions: Measured yields and atmospheric implications. United States. https://doi.org/10.1073/pnas.1423977112
Jokinen, Tuija, Berndt, Torsten, Makkonen, Risto, Kerminen, Veli-Matti, Junninen, Heikki, Paasonen, Pauli, Stratmann, Frank, Herrmann, Hartmut, Guenther, Alex B., Worsnop, Douglas R., Kulmala, Markku, Ehn, Mikael K., and Sipila, Mikko. Tue .
"Production of extremely low volatile organic compounds from biogenic emissions: Measured yields and atmospheric implications". United States. https://doi.org/10.1073/pnas.1423977112. https://www.osti.gov/servlets/purl/1221472.
@article{osti_1221472,
title = {Production of extremely low volatile organic compounds from biogenic emissions: Measured yields and atmospheric implications},
author = {Jokinen, Tuija and Berndt, Torsten and Makkonen, Risto and Kerminen, Veli-Matti and Junninen, Heikki and Paasonen, Pauli and Stratmann, Frank and Herrmann, Hartmut and Guenther, Alex B. and Worsnop, Douglas R. and Kulmala, Markku and Ehn, Mikael K. and Sipila, Mikko},
abstractNote = {Extremely low volatility organic compounds (ELVOC) are suggested to promote aerosol particle formation and cloud condensation nuclei (CCN) production in the atmosphere. We show that the capability of biogenic VOC (BVOC) to produce ELVOC depends strongly on their chemical structure and relative oxidant levels. BVOC with an endocyclic double bond, representative emissions from, e.g., boreal forests, efficiently produce ELVOC from ozonolysis. Compounds with exocyclic double bonds or acyclic compounds including isoprene, emission representative of the tropics, produce minor quantities of ELVOC, and the role of OH radical oxidation is relatively larger. Furthermore, implementing these findings into a global modeling framework shows that detailed assessment of ELVOC production pathways is crucial for understanding biogenic secondary organic aerosol and atmospheric CCN formation.},
doi = {10.1073/pnas.1423977112},
journal = {Proceedings of the National Academy of Sciences of the United States of America},
number = 23,
volume = 112,
place = {United States},
year = {Tue May 26 00:00:00 EDT 2015},
month = {Tue May 26 00:00:00 EDT 2015}
}
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Multi-generation OH oxidation as a source for highly oxygenated organic molecules from aromatics
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Production of highly oxygenated organic molecules (HOMs) from trace contaminants during isoprene oxidation
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Evaluating the performance of five different chemical ionization techniques for detecting gaseous oxygenated organic species
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The sensitivity of benzene cluster cation chemical ionization mass spectrometry to select biogenic terpenes
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Chemistry and deposition in the Model of Atmospheric composition at Global and Regional scales using Inversion Techniques for Trace gas Emissions (MAGRITTE v1.1) – Part 1: Chemical mechanism
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