Transport of anthropogenic and biomass burning aerosols from Europe to the Arctic during spring 2008
Abstract
During the POLARCAT-France airborne campaign in April 2008, pollution originating from anthropogenic and biomass burning emissions was measured in the European Arctic. We compare these aircraft measurements with simulations using the WRF-Chem model to investigate model representation of aerosols transported from Europe to the Arctic. Modeled PM2.5 is evaluated using European Monitoring and Evaluation Programme (EMEP) measurements in source regions and POLARCAT aircraft measurements in the Scandinavian Arctic. Total PM2.5 agrees well with the measurements, although the model overestimates nitrate and underestimates organic carbon in source regions. Using WRF-Chem in combination with the Lagrangian model FLEXPART-WRF, we find that during the campaign the research aircraft sampled two different types of European plumes: mixed anthropogenic and fire plumes from eastern Europe and Russia transported below 2 km, and anthropogenic plumes from central Europe uplifted by warm conveyor belt circulations to 5–6 km. Both modeled plume types had undergone significant wet scavenging (> 50% PM10) during transport. Modeled aerosol vertical distributions and optical properties below the aircraft are evaluated in the Arctic using airborne lidar measurements. Model results show that the pollution event transported aerosols into the Arctic (> 66.6° N) for a 4-day period. During this 4-day period, biomass burning emissionsmore »
- Authors:
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1182901
- Report Number(s):
- PNNL-SA-109564
Journal ID: ISSN 1680-7324; KP1701000
- Grant/Contract Number:
- AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Atmospheric Chemistry and Physics (Online)
- Additional Journal Information:
- Journal Name: Atmospheric Chemistry and Physics (Online); Journal Volume: 15; Journal Issue: 7; Journal ID: ISSN 1680-7324
- Publisher:
- European Geosciences Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES
Citation Formats
Marelle, L., Raut, Jean-Christophe, Thomas, J. L., Law, K. S., Quennehen, Boris, Ancellet, G., Pelon, J., Schwarzenboeck, A., and Fast, Jerome D. Transport of anthropogenic and biomass burning aerosols from Europe to the Arctic during spring 2008. United States: N. p., 2015.
Web. doi:10.5194/acp-15-3831-2015.
Marelle, L., Raut, Jean-Christophe, Thomas, J. L., Law, K. S., Quennehen, Boris, Ancellet, G., Pelon, J., Schwarzenboeck, A., & Fast, Jerome D. Transport of anthropogenic and biomass burning aerosols from Europe to the Arctic during spring 2008. United States. https://doi.org/10.5194/acp-15-3831-2015
Marelle, L., Raut, Jean-Christophe, Thomas, J. L., Law, K. S., Quennehen, Boris, Ancellet, G., Pelon, J., Schwarzenboeck, A., and Fast, Jerome D. Fri .
"Transport of anthropogenic and biomass burning aerosols from Europe to the Arctic during spring 2008". United States. https://doi.org/10.5194/acp-15-3831-2015. https://www.osti.gov/servlets/purl/1182901.
@article{osti_1182901,
title = {Transport of anthropogenic and biomass burning aerosols from Europe to the Arctic during spring 2008},
author = {Marelle, L. and Raut, Jean-Christophe and Thomas, J. L. and Law, K. S. and Quennehen, Boris and Ancellet, G. and Pelon, J. and Schwarzenboeck, A. and Fast, Jerome D.},
abstractNote = {During the POLARCAT-France airborne campaign in April 2008, pollution originating from anthropogenic and biomass burning emissions was measured in the European Arctic. We compare these aircraft measurements with simulations using the WRF-Chem model to investigate model representation of aerosols transported from Europe to the Arctic. Modeled PM2.5 is evaluated using European Monitoring and Evaluation Programme (EMEP) measurements in source regions and POLARCAT aircraft measurements in the Scandinavian Arctic. Total PM2.5 agrees well with the measurements, although the model overestimates nitrate and underestimates organic carbon in source regions. Using WRF-Chem in combination with the Lagrangian model FLEXPART-WRF, we find that during the campaign the research aircraft sampled two different types of European plumes: mixed anthropogenic and fire plumes from eastern Europe and Russia transported below 2 km, and anthropogenic plumes from central Europe uplifted by warm conveyor belt circulations to 5–6 km. Both modeled plume types had undergone significant wet scavenging (> 50% PM10) during transport. Modeled aerosol vertical distributions and optical properties below the aircraft are evaluated in the Arctic using airborne lidar measurements. Model results show that the pollution event transported aerosols into the Arctic (> 66.6° N) for a 4-day period. During this 4-day period, biomass burning emissions have the strongest influence on concentrations between 2.5 and 3 km altitudes, while European anthropogenic emissions influence aerosols at both lower (~ 1.5 km) and higher altitudes (~ 4.5 km). As a proportion of PM2.5, modeled black carbon and SO4= concentrations are more enhanced near the surface in anthropogenic plumes. The European plumes sampled during the POLARCAT-France campaign were transported over the region of springtime snow cover in northern Scandinavia, where they had a significant local atmospheric warming effect. We find that, during this transport event, the average modeled top-of-atmosphere (TOA) shortwave direct and semi-direct radiative effect (DSRE) north of 60° N over snow and ice-covered surfaces reaches +0.58 W m−2, peaking at +3.3 W m−2 at noon over Scandinavia and Finland.},
doi = {10.5194/acp-15-3831-2015},
journal = {Atmospheric Chemistry and Physics (Online)},
number = 7,
volume = 15,
place = {United States},
year = {Fri Apr 10 00:00:00 EDT 2015},
month = {Fri Apr 10 00:00:00 EDT 2015}
}
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