DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Single-mode porous silicon waveguide interferometers with unity confinement factors for ultra-sensitive surface adlayer sensing

Abstract

Guided wave-optics has emerged as a promising platform for label free biosensing. However, device sensitivity toward surface-bound small molecules is directly limited by the evanescent interaction and low confinement factor with the active sensing region. Here, we report a mesoporous silicon waveguide design and inverse fabrication technique that resolves the evanescent field interaction limitation while achieving maximal transverse confinement factors and preserving single-mode operation. The waveguide sensors are characterized in a Fabry-Perot interferometer configuration and the ultra-high sensitivity to small molecule adlayers is demonstrated. We also identify dispersion to be a promising degree of freedom for exceeding the sensitivity limits predicted by the conventional non-dispersive effective medium theory.

Authors:
ORCiD logo [1];  [1]; ORCiD logo [2];  [1]
  1. Clemson Univ., SC (United States)
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Publication Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1546510
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Optics Express
Additional Journal Information:
Journal Volume: 27; Journal Issue: 16; Journal ID: ISSN 1094-4087
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION

Citation Formats

Talukdar, Tahmid, Allen, Gabrielle, Kravchenko, Ivan I., and Ryckman, Judson. Single-mode porous silicon waveguide interferometers with unity confinement factors for ultra-sensitive surface adlayer sensing. United States: N. p., 2019. Web. doi:10.1364/OE.27.022485.
Talukdar, Tahmid, Allen, Gabrielle, Kravchenko, Ivan I., & Ryckman, Judson. Single-mode porous silicon waveguide interferometers with unity confinement factors for ultra-sensitive surface adlayer sensing. United States. https://doi.org/10.1364/OE.27.022485
Talukdar, Tahmid, Allen, Gabrielle, Kravchenko, Ivan I., and Ryckman, Judson. Tue . "Single-mode porous silicon waveguide interferometers with unity confinement factors for ultra-sensitive surface adlayer sensing". United States. https://doi.org/10.1364/OE.27.022485. https://www.osti.gov/servlets/purl/1546510.
@article{osti_1546510,
title = {Single-mode porous silicon waveguide interferometers with unity confinement factors for ultra-sensitive surface adlayer sensing},
author = {Talukdar, Tahmid and Allen, Gabrielle and Kravchenko, Ivan I. and Ryckman, Judson},
abstractNote = {Guided wave-optics has emerged as a promising platform for label free biosensing. However, device sensitivity toward surface-bound small molecules is directly limited by the evanescent interaction and low confinement factor with the active sensing region. Here, we report a mesoporous silicon waveguide design and inverse fabrication technique that resolves the evanescent field interaction limitation while achieving maximal transverse confinement factors and preserving single-mode operation. The waveguide sensors are characterized in a Fabry-Perot interferometer configuration and the ultra-high sensitivity to small molecule adlayers is demonstrated. We also identify dispersion to be a promising degree of freedom for exceeding the sensitivity limits predicted by the conventional non-dispersive effective medium theory.},
doi = {10.1364/OE.27.022485},
journal = {Optics Express},
number = 16,
volume = 27,
place = {United States},
year = {Tue Jul 23 00:00:00 EDT 2019},
month = {Tue Jul 23 00:00:00 EDT 2019}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 14 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Sensors and Biosensors for the Determination of Small Molecule Biological Toxins
journal, September 2008


Label-Free Biosensor Imaging on Photonic Crystal Surfaces
journal, August 2015


Optimized sensitivity of Silicon-on-Insulator (SOI) strip waveguide resonator sensor
journal, January 2017

  • TalebiFard, Sahba; Schmidt, Shon; Shi, Wei
  • Biomedical Optics Express, Vol. 8, Issue 2
  • DOI: 10.1364/BOE.8.000500

Label-Free Biosensor Arrays Based on Silicon Ring Resonators and High-Speed Optical Scanning Instrumentation
journal, January 2010

  • Iqbal, Muzammil; Gleeson, Martin A.; Spaugh, Bradley
  • IEEE Journal of Selected Topics in Quantum Electronics, Vol. 16, Issue 3
  • DOI: 10.1109/JSTQE.2009.2032510

TiO 2 Nanophotonic Sensors for Efficient Integrated Evanescent Raman Spectroscopy
journal, July 2016


Mid-infrared plasmonic biosensing with graphene
journal, July 2015


Optical Microcavity: Sensing down to Single Molecules and Atoms
journal, February 2011

  • Yoshie, Tomoyuki; Tang, Lingling; Su, Shu-Yu
  • Sensors, Vol. 11, Issue 2
  • DOI: 10.3390/s110201972

Optical Refractive Index Sensors with Plasmonic and Photonic Structures: Promising and Inconvenient Truth
journal, February 2019


Liquid Core ARROW Waveguides: A Promising Photonic Structure for Integrated Optofluidic Microsensors
journal, March 2016

  • Testa, Genni; Persichetti, Gianluca; Bernini, Romeo
  • Micromachines, Vol. 7, Issue 3
  • DOI: 10.3390/mi7030047

Characterization of sensing capability of optofluidic ring resonator biosensors
journal, July 2010

  • Li, Hao; Fan, Xudong
  • Applied Physics Letters, Vol. 97, Issue 1
  • DOI: 10.1063/1.3462296

Nanoscale porous silicon waveguide for label-free DNA sensing
journal, May 2008


Surface sensing with integrated optical waveguides: a design guideline
journal, January 2018

  • Milvich, Johannes; Kohler, Daria; Freude, Wolfgang
  • Optics Express, Vol. 26, Issue 16
  • DOI: 10.1364/OE.26.019885

Porous silicon ring resonator for compact, high sensitivity biosensing applications
journal, January 2015

  • Rodriguez, Gilberto A.; Hu, Shuren; Weiss, Sharon M.
  • Optics Express, Vol. 23, Issue 6
  • DOI: 10.1364/OE.23.007111

Experimental study of the sensitivity of a porous silicon ring resonator sensor using continuous in-flow measurements
journal, January 2017

  • Caroselli, Raffaele; Ponce-Alcántara, Salvador; Quilez, Francisco Prats
  • Optics Express, Vol. 25, Issue 25
  • DOI: 10.1364/OE.25.031651

Optimization of porous silicon waveguide design for micro-ring resonator sensing applications
journal, June 2018


A Porous Silicon-Based Optical Interferometric Biosensor
journal, October 1997


Layer-by-layer biofunctionalization of nanostructured porous silicon for high-sensitivity and high-selectivity label-free affinity biosensing
journal, December 2018

  • Mariani, Stefano; Robbiano, Valentina; Strambini, Lucanos M.
  • Nature Communications, Vol. 9, Issue 1
  • DOI: 10.1038/s41467-018-07723-8

Photonic crystal nanobeam biosensors based on porous silicon
journal, January 2019

  • Rodriguez, Gilberto A.; Markov, Petr; Cartwright, Alyssa P.
  • Optics Express, Vol. 27, Issue 7
  • DOI: 10.1364/OE.27.009536

Direct Imprinting of Porous Substrates: A Rapid and Low-Cost Approach for Patterning Porous Nanomaterials
journal, May 2011

  • Ryckman, Judson D.; Liscidini, Marco; Sipe, J. E.
  • Nano Letters, Vol. 11, Issue 5
  • DOI: 10.1021/nl1028073

Patterned Microstructures of Porous Silicon by Dry-Removal Soft Lithography
journal, January 2003


Direct Imprinting of Porous Silicon via Metal-Assisted Chemical Etching
journal, February 2016

  • Azeredo, Bruno P.; Lin, Yu-Wei; Avagyan, Arik
  • Advanced Functional Materials, Vol. 26, Issue 17
  • DOI: 10.1002/adfm.201505153

First-principle derivation of gain in high-index-contrast waveguides
journal, January 2008

  • Robinson, Jacob T.; Preston, Kyle; Painter, Oskar
  • Optics Express, Vol. 16, Issue 21
  • DOI: 10.1364/OE.16.016659

Slow light in photonic crystal waveguides
journal, April 2007


Defect-mediated resonance shift of silicon-on-insulator racetrack resonators
journal, January 2011

  • Ackert, J. J.; Doylend, J. K.; Logan, D. F.
  • Optics Express, Vol. 19, Issue 13
  • DOI: 10.1364/OE.19.011969

Plasmonic Nanostructures for Nano-Scale Bio-Sensing
journal, November 2011

  • Chung, Taerin; Lee, Seung-Yeol; Song, Eui Young
  • Sensors, Vol. 11, Issue 11
  • DOI: 10.3390/s111110907

Resonant Mode Engineering of Photonic Crystal Sensors Clad with Ultralow Refractive Index Porous Silicon Dioxide
journal, September 2017

  • Wan, Yuhang; Krueger, Neil A.; Ocier, Christian R.
  • Advanced Optical Materials, Vol. 5, Issue 21
  • DOI: 10.1002/adom.201700605

Optical sensing by optimized silicon slot waveguides
journal, January 2007

  • Dell'Olio, Francesco; Passaro, Vittorio M.
  • Optics Express, Vol. 15, Issue 8
  • DOI: 10.1364/OE.15.004977

Porous Silicon Gradient Refractive Index Micro-Optics
journal, November 2016


Quantitative analysis of the sensitivity of porous silicon optical biosensors
journal, April 2006

  • Ouyang, Huimin; Striemer, Christopher C.; Fauchet, Philippe M.
  • Applied Physics Letters, Vol. 88, Issue 16
  • DOI: 10.1063/1.2196069

Birefringent porous silicon membranes for optical sensing
journal, January 2011

  • Álvarez, Jesús; Bettotti, Paolo; Suárez, Isaac
  • Optics Express, Vol. 19, Issue 27
  • DOI: 10.1364/OE.19.026106

Dichroic rugate filters based on birefringent porous silicon
journal, January 2008

  • Ishikura, Nobuyuki; Fujii, Minoru; Nishida, Kohei
  • Optics Express, Vol. 16, Issue 20
  • DOI: 10.1364/OE.16.015531

Porous Silicon-Based Photonic Biosensors: Current Status and Emerging Applications
journal, November 2018


Real-time monitoring of enzyme activity in a mesoporous silicon double layer
journal, February 2009

  • Orosco, Manuel M.; Pacholski, Claudia; Sailor, Michael J.
  • Nature Nanotechnology, Vol. 4, Issue 4
  • DOI: 10.1038/nnano.2009.11

Ultra-broadband dispersion engineering of nanophotonic waveguides
journal, January 2016


Controlling evanescent waves using silicon photonic all-dielectric metamaterials for dense integration
journal, May 2018


Transparent subdiffraction optics: nanoscale light confinement without metal
journal, January 2014


Biosensing Using Porous Silicon Double-Layer Interferometers:  Reflective Interferometric Fourier Transform Spectroscopy
journal, August 2005

  • Pacholski, Claudia; Sartor, Marta; Sailor, Michael J.
  • Journal of the American Chemical Society, Vol. 127, Issue 33
  • DOI: 10.1021/ja0511671

Transparent subdiffraction optics: nanoscale light confinement without metal
conference, January 2015


Surface sensing with integrated optical waveguides: a design guideline
text, January 2018

  • Milvich, Johannes; Kohler, Daria; Freude, Wolfgang
  • The Optical Society of America (OSA)
  • DOI: 10.5445/ir/1000084982