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Title: Re Doping in 2D Transition Metal Dichalcogenides as a New Route to Tailor Structural Phases and Induced Magnetism

Abstract

Alloying in 2D results in the development of new, diverse, and versatile systems with prospects in bandgap engineering, catalysis, and energy storage. Tailoring structural phase transitions using alloying is a novel idea with implications in designing all 2D device architecture as the structural phases in 2D materials such as transition metal dichalcogenides are correlated with electronic phases. In this paper, this study develops a new growth strategy employing chemical vapor deposition to grow monolayer 2D alloys of Re-doped MoSe2 with show composition tunable structural phase variations. The compositions where the phase transition is observed agree well with the theoretical predictions for these 2D systems. Finally, it is also shown that in addition to the predicted new electronic phases, these systems also provide opportunities to study novel phenomena such as magnetism which broadens the range of their applications.

Authors:
 [1];  [1];  [2];  [3];  [4];  [1];  [2];  [5];  [4];  [4];  [4]; ORCiD logo [1];  [1]
+ Show Author Affiliations
  1. Rice Univ., Houston, TX (United States). Materials Science and Nano Engineering
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences
  3. Univ. of Southern California, Los Angeles, CA (United States). Collaboratory for Advanced Computing and Simulations; Kumamoto Univ. (Japan). Dept. of Physics
  4. Univ. of Southern California, Los Angeles, CA (United States). Collaboratory for Advanced Computing and Simulations
  5. Kumamoto Univ. (Japan). Dept. of Physics
Publication Date:
Research Org.:
Univ. of Southern California, Los Angeles, CA (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Rice Univ., Houston, TX (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1423052
Alternate Identifier(s):
OSTI ID: 1398722
Grant/Contract Number:  
AC05-00OR22725; SC0014607
Resource Type:
Accepted Manuscript
Journal Name:
Advanced Materials
Additional Journal Information:
Journal Volume: 29; Journal Issue: 43; Journal ID: ISSN 0935-9648
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 2D materials; alloys; DFT calculations; magnetic properties; phase transition

Citation Formats

Kochat, Vidya, Apte, Amey, Hachtel, Jordan A., Kumazoe, Hiroyuki, Krishnamoorthy, Aravind, Susarla, Sandhya, Idrobo, Juan Carlos, Shimojo, Fuyuki, Vashishta, Priya, Kalia, Rajiv, Nakano, Aiichiro, Tiwary, Chandra Sekhar, and Ajayan, Pulickel M. Re Doping in 2D Transition Metal Dichalcogenides as a New Route to Tailor Structural Phases and Induced Magnetism. United States: N. p., 2017. Web. doi:10.1002/adma.201703754.
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Kochat, Vidya, Apte, Amey, Hachtel, Jordan A., Kumazoe, Hiroyuki, Krishnamoorthy, Aravind, Susarla, Sandhya, Idrobo, Juan Carlos, Shimojo, Fuyuki, Vashishta, Priya, Kalia, Rajiv, Nakano, Aiichiro, Tiwary, Chandra Sekhar, & Ajayan, Pulickel M. Re Doping in 2D Transition Metal Dichalcogenides as a New Route to Tailor Structural Phases and Induced Magnetism. United States. https://doi.org/10.1002/adma.201703754
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Kochat, Vidya, Apte, Amey, Hachtel, Jordan A., Kumazoe, Hiroyuki, Krishnamoorthy, Aravind, Susarla, Sandhya, Idrobo, Juan Carlos, Shimojo, Fuyuki, Vashishta, Priya, Kalia, Rajiv, Nakano, Aiichiro, Tiwary, Chandra Sekhar, and Ajayan, Pulickel M. Mon . "Re Doping in 2D Transition Metal Dichalcogenides as a New Route to Tailor Structural Phases and Induced Magnetism". United States. https://doi.org/10.1002/adma.201703754. https://www.osti.gov/servlets/purl/1423052.
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@article{osti_1423052,
title = {Re Doping in 2D Transition Metal Dichalcogenides as a New Route to Tailor Structural Phases and Induced Magnetism},
author = {Kochat, Vidya and Apte, Amey and Hachtel, Jordan A. and Kumazoe, Hiroyuki and Krishnamoorthy, Aravind and Susarla, Sandhya and Idrobo, Juan Carlos and Shimojo, Fuyuki and Vashishta, Priya and Kalia, Rajiv and Nakano, Aiichiro and Tiwary, Chandra Sekhar and Ajayan, Pulickel M.},
abstractNote = {Alloying in 2D results in the development of new, diverse, and versatile systems with prospects in bandgap engineering, catalysis, and energy storage. Tailoring structural phase transitions using alloying is a novel idea with implications in designing all 2D device architecture as the structural phases in 2D materials such as transition metal dichalcogenides are correlated with electronic phases. In this paper, this study develops a new growth strategy employing chemical vapor deposition to grow monolayer 2D alloys of Re-doped MoSe2 with show composition tunable structural phase variations. The compositions where the phase transition is observed agree well with the theoretical predictions for these 2D systems. Finally, it is also shown that in addition to the predicted new electronic phases, these systems also provide opportunities to study novel phenomena such as magnetism which broadens the range of their applications.},
doi = {10.1002/adma.201703754},
journal = {Advanced Materials},
number = 43,
volume = 29,
place = {United States},
year = {Mon Oct 09 00:00:00 EDT 2017},
month = {Mon Oct 09 00:00:00 EDT 2017}
}
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https://doi.org/10.1002/adma.201703754
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