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Nanostructured GaN Nucleation Layer for Light-Emitting Diodes

Journal Article · · Journal of Nanoscience and Nanotechnology
 [1];  [1];  [1];  [2];  [3]
  1. North Carolina State University
  2. University of North Carolina, Chapel Hill
  3. ORNL

This paper addresses the formation of nanostructured gallium nitride nucleation (NL) or initial layer (IL), which is necessary to obtain a smooth surface morphology and reduce defects in h-GaN layers for light-emitting diodes and lasers. From detailed X-ray and HR-TEM studies, researchers determined that this layer consists of nanostructured grains with average grain size of 25 nm, which are separated by small-angle grain boundaries (with misorientation 1 ), known as subgrain boundaries. Thus NL is considered to be single-crystal layer with mosaicity of about 1 . These nc grains are mostly faulted cubic GaN (c-GaN) and a small fraction of unfaulted c-GaN. This unfaulted Zinc-blende c-GaN, which is considered a nonequilibrium phase, often appears as embedded or occluded within the faulted c-GaN. The NL layer contained in-plane tensile strain, presumably arising from defects due to island coalescence during Volmer-Weber growth. The 10L X-ray scans showed c-GaN fraction to be over 63% and the rest h-GaN. The NL layer grows epitaxially with the (0001) sapphire substrate by domain matching epitaxy, and this epitaxial relationship is remarkably maintained when c-GaN converts into h-GaN during high-temperature growth.

Research Organization:
Oak Ridge National Laboratory (ORNL)
Sponsoring Organization:
SC USDOE - Office of Science (SC)
DOE Contract Number:
AC05-00OR22725
OSTI ID:
931814
Journal Information:
Journal of Nanoscience and Nanotechnology, Journal Name: Journal of Nanoscience and Nanotechnology Journal Issue: 8 Vol. 7
Country of Publication:
United States
Language:
English

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