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Degradation of discontinuous gold films under MeV heavy-ion bombardment

Journal Article · · J. Appl. Phys.; (United States)
DOI:https://doi.org/10.1063/1.324487· OSTI ID:6627961
Thin discontinuous gold films evaporated onto 150--230-A-thick C substrates were irradiated with perpendicularly impinging MeV N, O, F, Cl, and Br ions up to fluences of 5 x 10/sup 15/ ions/cm/sup 2/ and fluxes up to 8 x 10/sup 11/ ions/cm/sup 2/ sec. Surprisingly rapid degradation of the gold films was found; in some cases, up to 2000 gold atoms per impinging ion were removed, as measured by Rutherford scattering. The degradation was also investigated by transmission-electron microscopy. The angular distribution of the ejected gold atoms was indicated by a simple collector experiment and found incompatible with chunk emission. The degradation is concluded to be caused by the same ionization mechanism as that occurring when fission fragments form tracks in discontinuous metal films. During irradiation, the remaining part of the film is found to be stabilized against further degradation by ionization-induced cracking of hydrocarbons.
Research Organization:
Institute of Physics, University of Aarhus, DK-8000 Aarhus C, Denmark
OSTI ID:
6627961
Journal Information:
J. Appl. Phys.; (United States), Journal Name: J. Appl. Phys.; (United States) Vol. 49:11; ISSN JAPIA
Country of Publication:
United States
Language:
English