Separation of radium and actinium using zirconia

Brown, M. Alex

doi:10.1016/j.apradiso.2022.110238

Separation of radium and actinium using zirconia

Journal Article · Mon Apr 11 00:00:00 EDT 2022 · Applied Radiation and Isotopes

DOI:https://doi.org/10.1016/j.apradiso.2022.110238· OSTI ID:1915449

Brown, M. Alex ^[1]

Argonne National Lab. (ANL), Argonne, IL (United States)

Herein, zirconia was investigated as a radiation-resistant support for radium and actinium aqueous ion separations. Acetate and total metal ion concentrations were experimentally evaluated as factors that could affect retention using La and Ba surrogates. Pseudo-second order rate constants were derived and the uptake of La was determined to be endothermic. Elution profiles containing Ba, La, ²²⁸Ra, ²²⁸Ac, and ²¹²Pb are presented and discussed.

View Accepted Manuscript (DOE)

Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1915449

Journal Information:: Applied Radiation and Isotopes, Journal Name: Applied Radiation and Isotopes Vol. 185; ISSN 0969-8043

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Separation of radium and actinium using zirconia

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