High mobility in a van der Waals layered antiferromagnetic metal

Lei, Shiming; Lin, Jingjing; Jia, Yanyu; Gray, Mason; Topp, Andreas; Farahi, Gelareh; Klemenz, Sebastian; Gao, Tong; Rodolakis, Fanny; McChesney, Jessica L.; Ast, Christian R.; Yazdani, Ali; Burch, Kenneth S.; Wu, Sanfeng; Ong, Nai Phuan; Schoop, Leslie M.

doi:10.1126/sciadv.aay6407

Title: High mobility in a van der Waals layered antiferromagnetic metal

Journal Article · Fri Feb 07 00:00:00 EST 2020 · Science Advances

DOI:https://doi.org/10.1126/sciadv.aay6407· OSTI ID:1839265

^[1];

^[2]; Topp, Andreas ^[3]; Farahi, Gelareh ^[1]; Klemenz, Sebastian ^[1];

^[1];

^[4]; McChesney, Jessica L. ^[4]; Ast, Christian R. ^[3];

^[1];

^[2]; Wu, Sanfeng ^[1];

^[1];

^[1]

Princeton Univ., NJ (United States)
Boston College, Boston, MA (United States)
Max-Planck-Inst. für Festkörperforschung, Stuttgart (Germany)
Argonne National Lab. (ANL), Argonne, IL (United States)

Van der Waals (vdW) materials with magnetic order have been heavily pursued for fundamental physics as well as for device design. Despite the rapid advances, so far, they are mainly insulating or semiconducting, and none of them has a high electronic mobility—a property that is rare in layered vdW materials in general. The realization of a high-mobility vdW material that also exhibits magnetic order would open the possibility for novel magnetic twistronic or spintronic devices. Here, we report very high carrier mobility in the layered vdW antiferromagnet GdTe₃. The electron mobility is beyond 60,000 cm²V^–1s^–1, which is the highest among all known layered magnetic materials, to the best of our knowledge. Among all known vdW materials, the mobility of bulk GdTe₃is comparable to that of black phosphorus. By mechanical exfoliation, we further demonstrate that GdTe₃can be exfoliated to ultrathin flakes of three monolayers.

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Research Organization:: Princeton Univ., NJ (United States); Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; National Science Foundation (NSF); ExxonMobil Research and Engineering Company

Grant/Contract Number:: FG02-07ER46419; AC02-06CH11357; DMR-1904442; DMR-0703406; DMR-1420541; ARO W911NF-12-1-0461; SC0017863; DMR-1709987; DMR-142054

OSTI ID:: 1839265

Alternate ID(s):: OSTI ID: 1599045

Journal Information:: Science Advances, Vol. 6, Issue 6; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 59 works

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