Recent Advances in Rechargeable Aluminum-Ion Batteries and Considerations for Their Future Progress

Zhang, Kaiqiang; Kirlikovali, Kent O.; Suh, Jun Min; Choi, Ji-Won; Jang, Ho Won; Varma, Rajender S.; Farha, Omar K.; Shokouhimehr, Mohammadreza

doi:10.1021/acsaem.0c00957

Title: Recent Advances in Rechargeable Aluminum-Ion Batteries and Considerations for Their Future Progress

Journal Article · Mon Jun 01 00:00:00 EDT 2020 · ACS Applied Energy Materials

DOI:https://doi.org/10.1021/acsaem.0c00957· OSTI ID:1771015

Zhang, Kaiqiang ^[1];

^[2]; Suh, Jun Min ^[3];

^[4];

^[3];

^[5];

^[2];

^[3]

Seoul National Univ. (Korea); Korea Inst. of Science and Technology (KIST), Seoul (Korea)
Northwestern Univ., Evanston, IL (United States)
Seoul National Univ. (Korea)
Korea Inst. of Science and Technology (KIST), Seoul (Korea)
Palacky Univ., Olomouc (Czech Republic)

Owing to their high theoretical capacity and reliable operational safety, nonaqueous rechargeable aluminum batteries (RABs) have emerged as a promising class of battery materials and been intensively studied in recent years; however, a lack of suitable, high-performing positive electrode materials, along with the need for air-sensitive and expensive ionic liquid electrolytes, has significantly hindered the practical use of RABs in large-scale applications. Therefore, we sought to carefully analyze positive electrode materials and the associated electrolytes that have been reported in these battery systems in order to stimulate the design of the next generation of high-performance and low-cost RABs. In this review, we have summarized the electrode materials that have been used in both nonaqueous and aqueous RAB systems and provided a rational classification based on the types of materials used and their respective structures. Additionally, we have reviewed electrolytes employed in RABs and have categorized them according to two main types of applications, either for fixed battery systems or for use in portable devices. Here, a systematic account of recent developments on RABs, with a focus on electrode materials, innovative perspectives, and impending research efforts on future RABs, has been included. Finally, a proposed liquid RAB system is discussed with the aim of solving issues regarding fast-charging and long operational lifetimes, followed by insights into solid RABs for use in both portable and multistructural RAB systems.

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Research Organization:: Univ. of Minnesota, Minneapolis, MN (United States)

Sponsoring Organization:: USDOE; US Army Research Office (ARO); Korea Institute of Science and Technology Future Resource Program

Grant/Contract Number:: SC0008688; W911NF1910340; 2E29400

OSTI ID:: 1771015

Journal Information:: ACS Applied Energy Materials, Vol. 3, Issue 7; ISSN 2574-0962

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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