Fundamental Understanding and Material Challenges in Rechargeable Nonaqueous Li-O2 Batteries: Recent Progress and Perspective

Ma, Lu; Yu, Tongwen; Tzoganakis, Evangelos; Amine, Khalil; Wu, Tianpin; Chen, Zhongwei; Lu, Jun

doi:10.1002/aenm.201800348

Title: Fundamental Understanding and Material Challenges in Rechargeable Nonaqueous Li-O₂ Batteries: Recent Progress and Perspective

Journal Article · Tue May 29 00:00:00 EDT 2018 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.201800348· OSTI ID:1471419

Ma, Lu ^[1]; Yu, Tongwen ^[2]; Tzoganakis, Evangelos ^[2]; Amine, Khalil ^[3]; Wu, Tianpin ^[1]; Chen, Zhongwei ^[2];

^[1]

Argonne National Lab. (ANL), Lemont, IL (United States)
Univ. of Waterloo, Waterloo, ON (Canada)
Argonne National Lab. (ANL), Lemont, IL (United States); Imam Abdulrahman Bin Faisal University, Dammam (Saudi Arabia); Stanford Univ., Stanford, CA (United States)

Abstract Energy storage challenges have triggered growing interest in various battery technologies and electrocatalysis. As a particularly promising variety, the Li–O ₂ battery with an extremely high energy density is of great significance, offering tremendous opportunities to improve cell performance via understanding catalytic mechanisms and the exploration of new materials. Furthermore, focus on nonaqueous electrolyte‐based Li–O ₂ batteries has markedly intensified since there could be a higher probability of commercialization, compared to that of solid‐state or aqueous electrolytes. The recent advancements of the nonaqueous Li–O ₂ battery in terms of fundamental understanding and material challenges, including electrolyte stability, water effect, and noncarbon cathode materials are summarized in this review. Further, the current status of water impact on discharge products, possible mechanisms, and parasitic reactions in nonaqueous electrolytes are reviewed for the first time. The key challenges of noncarbon oxygen electrode materials, such as noble metals and metal oxides‐based cathodes, transition metals, transition metal compounds (carbides, oxides) based cathodes as well as noncarbon supported catalysts are discussed. This review concludes with a perspective on future research directions for nonaqueous Li–O ₂ batteries.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V); USDOE

Grant/Contract Number:: AC02-06CH11357; DE‐AC02‐06CH11357

OSTI ID:: 1471419

Alternate ID(s):: OSTI ID: 1439402

Journal Information:: Advanced Energy Materials, Vol. 8, Issue 22; ISSN 1614-6832

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 121 works

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Singlet Oxygen Generation as a Major Cause for Parasitic Reactions during Cycling of Aprotic Lithium-Oxygen Batteries Mahne, Nika; Schafzahl, Bettina; Leypold, Christian arXiv https://doi.org/10.48550/arxiv.1711.10340	text	January 2017
Cycling Li-O2 Batteries via LiOH Formation and Decomposition Liu, Tao; Leskes, Michal; Yu, Wanjing arXiv https://doi.org/10.48550/arxiv.1805.03042	preprint	January 2018

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NiCo ₂ S ₄ Nanorod Arrays Supported on Carbon Textile as a Free-Standing Electrode for Stable and Long-Life Lithium-Oxygen Batteries Hu, Anjun; Long, Jianping; Shu, Chaozhu ChemElectroChem, Vol. 6, Issue 2 https://doi.org/10.1002/celc.201801474	journal	November 2018
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Design strategies toward catalytic materials and cathode structures for emerging Li–CO ₂ batteries Hu, Anjun; Shu, Chaozhu; Xu, Chenxi Journal of Materials Chemistry A, Vol. 7, Issue 38 https://doi.org/10.1039/c9ta06506g	journal	January 2019
Novel MoSi ₂ catalysts featuring surface activation as highly efficient cathode materials for long-life Li–O ₂ batteries Dang, Congcong; Wang, Yu; He, Biao Journal of Materials Chemistry A, Vol. 8, Issue 1 https://doi.org/10.1039/c9ta10713d	journal	January 2020
Three-Dimensional Nitrogen-Doped Hollow Carbon Fiber with a Micro-Scale Diameter as a Binder-Free Oxygen Electrode for Li-O ₂ Batteries Lim, Katie Heeyum; Kweon, Heejun; Kim, Hansung Journal of The Electrochemical Society, Vol. 166, Issue 14 https://doi.org/10.1149/2.1101914jes	journal	January 2019
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Recent Progress on Catalysts for the Positive Electrode of Aprotic Lithium-Oxygen Batteries † Cai, Yichao; Hou, Yunpeng; Lu, Yong Inorganics, Vol. 7, Issue 6 https://doi.org/10.3390/inorganics7060069	journal	May 2019
Understanding the Reaction Chemistry during Charging in Aprotic Lithium–Oxygen Batteries: Existing Problems and Solutions Shu, Chaozhu; Wang, Jiazhao; Long, Jianping Advanced Materials, Vol. 31, Issue 15 https://doi.org/10.1002/adma.201804587	journal	February 2019

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