High-efficiency solution-processed perovskite solar cells with millimeter-scale grains

Nie, W.; Tsai, H.; Asadpour, R.; Blancon, J. -C.; Neukirch, A. J.; Gupta, G.; Crochet, J. J.; Chhowalla, M.; Tretiak, S.; Alam, M. A.; Wang, H. -L.; Mohite, A. D.

doi:10.1126/science.aaa0472

Title: High-efficiency solution-processed perovskite solar cells with millimeter-scale grains

Journal Article · Fri Jan 30 00:00:00 EST 2015 · Science

DOI:https://doi.org/10.1126/science.aaa0472· OSTI ID:1579878

Nie, W. ^[1]; Tsai, H. ^[1]; Asadpour, R. ^[2]; Blancon, J. -C. ^[1]; Neukirch, A. J. ^[1]; Gupta, G. ^[1]; Crochet, J. J. ^[1]; Chhowalla, M. ^[3]; Tretiak, S. ^[1]; Alam, M. A. ^[2]; Wang, H. -L. ^[1]; Mohite, A. D. ^[1]

Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Purdue Univ., West Lafayette, IN (United States)
Rutgers Univ., Piscataway, NJ (United States)

Currently, state-of-the-art photovoltaics use high-purity, large-area, wafer-scale single-crystalline semiconductors grown by sophisticated, high-temperature crystal growth processes. We show a solution-based hot-casting technique to grow continuous, pinhole-free thin films of organometallic perovskites with millimeter-scale crystalline grains. We fabricated planar solar cells with efficiencies approaching 18%, with little cell-to-cell variability. The devices show hysteresis-free photovoltaic response, which had been a fundamental bottleneck for the stable operation of perovskite devices. Characterization and modeling attribute the improved performance to reduced bulk defects and improved charge carrier mobility in large-grain devices. We anticipate that this technique will lead the field toward synthesis of wafer-scale crystalline perovskites, necessary for the fabrication of high-efficiency solar cells, and will be applicable to several other material systems plagued by polydispersity, defects, and grain boundary recombination in solution-processed thin films.

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Research Organization:: Stanford Univ., CA (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office

Grant/Contract Number:: EE0004946

OSTI ID:: 1579878

Journal Information:: Science, Vol. 347, Issue 6221; ISSN 0036-8075

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 2700 works

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