Ultrafast dynamics of spin and orbital correlations in quantum materials: an energy- and momentum-resolved perspective

Cao, Y.; Mazzone, D. G.; Meyers, D.; Hill, J. P.; Liu, X.; Wall, S.; Dean, M. P.  M.

doi:10.1098/rsta.2017.0480

Title: Ultrafast dynamics of spin and orbital correlations in quantum materials: an energy- and momentum-resolved perspective

Journal Article · Mon Apr 01 00:00:00 EDT 2019 · Philosophical Transactions of the Royal Society. A, Mathematical, Physical and Engineering Sciences

DOI:https://doi.org/10.1098/rsta.2017.0480· OSTI ID:1508359

Cao, Y. ^[1];

^[2]; Meyers, D. ^[3]; Hill, J. P. ^[2]; Liu, X. ^[4]; Wall, S. ^[5];

^[3]

Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics; Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
Brookhaven National Lab. (BNL), Upton, NY (United States). National Synchrotron Light Source II (NSLS-II)
Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Department
ShanghaiTech Univ., Shanghai (China). School of Physical Science and Technology
Barcelona Institute of Science and Technology (BIST), Tarragona (Spain)

Many remarkable properties of quantum materials emerge from states with intricate coupling between the charge, spin and orbital degrees of freedom. Ultrafast photo-excitations of these materials hold great promise for understanding and controlling the properties of these states. Here we introduce time-resolved resonant inelastic X-ray scattering (tr-RIXS) as a means of measuring the charge, spin and orbital excitations out of equilibrium. These excitations encode the correlations and interactions that determine the detailed properties of the states generated. After outlining the basic principles and instrumentation of tr-RIXS, we review our first observations of transient antiferromagnetic correlations in quasi two dimensions in a photo-excited Mott insulator and present possible future routes of this fast-developing technique. The increasing number of X-ray free electron laser facilities not only enables tackling long-standing fundamental scientific problems, but also promises to unleash novel inelastic X-ray scattering spectroscopies.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States); Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: Ministry of Science and Technology of the Republic of China (MOST); Swiss National Science Foundation (SNSF); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357; SC0012704

OSTI ID:: 1508359

Alternate ID(s):: OSTI ID: 1480978

Report Number(s):: BNL-209365-2018-JAAM; 147631

Journal Information:: Philosophical Transactions of the Royal Society. A, Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2145; ISSN 1364-503X

Publisher:: The Royal Society PublishingCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 15 works

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Ultrafast dynamics of spin and orbital correlations in quantum materials: An energy- and momentum-resolved perspective Supplementary material Cao, Y.; Mazzone, D. G.; Meyers, D. https://doi.org/10.6084/m9.figshare.7764209 The current record is supplemented by this text	text	January 2019
Ultrafast dynamics of spin and orbital correlations in quantum materials: An energy- and momentum-resolved perspective Supplementary material Cao, Y.; Mazzone, D. G.; Meyers, D. https://doi.org/10.6084/m9.figshare.7764209.v1 The current record is supplemented by this text	text	January 2019
Supplementary material from "Ultrafast dynamics of spin and orbital correlations in quantum materials: an energy- and momentum-resolved perspective" Cao, Y.; Mazzone, D. G.; Meyers, D. https://doi.org/10.6084/m9.figshare.c.4413392 The current record is supplemented by this collection	collection	January 2019
Supplementary material from "Ultrafast dynamics of spin and orbital correlations in quantum materials: an energy- and momentum-resolved perspective" Cao, Y.; Mazzone, D. G.; Meyers, D. https://doi.org/10.6084/m9.figshare.c.4413392.v1 The current record is supplemented by this collection	collection	January 2019

Title: Ultrafast dynamics of spin and orbital correlations in quantum materials: an energy- and momentum-resolved perspective

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