Sub-microsecond-resolved multi-speckle X-ray photon correlation spectroscopy with a pixel array detector

Zhang, Qingteng; Dufresne, Eric M.; Narayanan, Suresh; Maj, Piotr; Koziol, Anna; Szczygiel, Robert; Grybos, Pawel; Sutton, Mark; Sandy, Alec R.

doi:10.1107/S1600577518009074

Title: Sub-microsecond-resolved multi-speckle X-ray photon correlation spectroscopy with a pixel array detector

Journal Article · Thu Aug 02 00:00:00 EDT 2018 · Journal of Synchrotron Radiation (Online)

DOI:https://doi.org/10.1107/S1600577518009074· OSTI ID:1474146

^[1]; Dufresne, Eric M. ^[1]; Narayanan, Suresh ^[1]; Maj, Piotr ^[2]; Koziol, Anna ^[2]; Szczygiel, Robert ^[2]; Grybos, Pawel ^[2]; Sutton, Mark ^[3];

^[1]

Argonne National Lab. (ANL), Lemont, IL (United States)
AGH Univ. of Science and Technology, Krakow (Poland)
McGill Univ., Montreal, QC (Canada)

Small-angle X-ray photon correlation spectroscopy (XPCS) measurements spanning delay times from 826 ns to 52.8 s were performed using a photon-counting pixel array detector with a dynamic range of 0–3 (2 bits). Fine resolution and a wide dynamic range of time scales was achieved by combining two modes of operation of the detector: (i) continuous mode, where data acquisition and data readout are performed in parallel with a frame acquisition time of 19.36 µs, and (ii) burst mode, where 12 frames are acquired with frame integration times of either 2.56 µs frame^–1 or 826 ns frame^–1 followed by 3.49 ms or 1.16 ms, respectively, for readout. The applicability of the detector for performing multi-speckle XPCS was demonstrated by measuring the Brownian dynamics of 10 nm-radius gold and 57 nm-radius silica colloids in water at room temperature. In addition, the capability of the detector to faithfully record one- and two-photon counts was examined by comparing the statistical distribution of photon counts with expected probabilities from the negative binomial distribution. In conclusion, it was found that in burst mode the ratio of 2s to 1s is markedly smaller than predicted and that this is attributable to pixel-response dead-time.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC); National Science Centre (Poland)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1474146

Journal Information:: Journal of Synchrotron Radiation (Online), Vol. 25, Issue 5; ISSN 1600-5775

Publisher:: International Union of CrystallographyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 30 works

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Anisotropic and heterogeneous dynamics in an aging colloidal gel Jain, Avni; Schulz, Florian; Lokteva, Irina Deutsches Elektronen-Synchrotron, DESY, Hamburg https://doi.org/10.3204/pubdb-2020-01104	text	January 2020

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Title: Sub-microsecond-resolved multi-speckle X-ray photon correlation spectroscopy with a pixel array detector

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