Gold Nanoparticle Monolayers with Tunable Optical and Electrical Properties

Yang, Guang; Hu, Longqian; Keiper, Timothy D.; Xiong, Peng; Hallinan, Jr., Daniel T.

doi:10.1021/acs.langmuir.6b00347

Title: Gold Nanoparticle Monolayers with Tunable Optical and Electrical Properties

Journal Article · Sun Mar 27 00:00:00 EDT 2016 · Langmuir

DOI:https://doi.org/10.1021/acs.langmuir.6b00347· OSTI ID:1249258

Yang, Guang ^[1]; Hu, Longqian ^[2]; Keiper, Timothy D. ^[2]; Xiong, Peng ^[2]; Hallinan, Jr., Daniel T. ^[1]

Florida State Univ., Tallahassee, FL (United States); Florida A & M University, Tallahassee, FL (United States)
Florida State Univ., Tallahassee, FL (United States)

In this work, centimeter-scale gold nanoparticle (Au NP) monolayer films have been fabricated using a water/organic solvent self-assembly strategy. A recently developed approach, drain to deposit, is demonstrated to be most effective in transferring the Au NP films from the water/organic solvent interface to various solid substrates while maintaining their integrity. The interparticle spacing was tuned from 1.4 to 3.1 nm using alkylamine ligands of different lengths. The ordering of the films increased with increasing ligand length. The surface plasmon resonance and the in-plane electrical conductivity of the Au NP films both exhibit an exponential dependence on the interparticle spacing. These findings show great potential in scaling up the manufacturing of high-performance optical and electronic devices based on two-dimensional metallic nanoparticle superlattices.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States). Advanced Photon Source (APS)

Sponsoring Organization:: National Science Foundation (NSF); State of Florida; USDOE

Grant/Contract Number:: DMR-1308613; AC02-06CH11357

OSTI ID:: 1249258

Journal Information:: Langmuir, Vol. 32, Issue 16; ISSN 0743-7463

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: ENGLISH

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Cited by: 54 works

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