Electric-field-induced strain effects on the magnetization of a Pr0.67Sr0.33MnO3 film

Zhang, B.; Sun, C. -J.; Lu, W.; Venkatesan, T.; Han, M. -G.; Zhu, Y.; Chen, J.; Chow, G. M.

doi:10.1103/PhysRevB.91.174431

Title: Electric-field-induced strain effects on the magnetization of a Pr_0.67Sr_0.33MnO₃ film

Journal Article · Tue May 26 00:00:00 EDT 2015 · Physical Review. B, Condensed Matter and Materials Physics

DOI:https://doi.org/10.1103/PhysRevB.91.174431· OSTI ID:1226033

Zhang, B. ^[1]; Sun, C. -J. ^[2]; Lu, W. ^[1]; Venkatesan, T. ^[1]; Han, M. -G. ^[3]; Zhu, Y. ^[3]; Chen, J. ^[1]; Chow, G. M. ^[1]

National Univ. of Singapore (Singapore)
Argonne National Lab. (ANL), Argonne, IL (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States)

The electric-field control of magnetic properties of Pr_0.67Sr_0.33MnO₃ (PSMO) film on piezoelectric Pb(Mg_1/3Nb_2/3)O₃-PbTiO₃ (PMNT) substrate was investigated. The piezoelectric response of the PMNT substrate to the electric field produced strain that was coupled to the PSMO film. The in-plane compressive (tensile) strain increased (decreased) the magnetization. The change of magnetic moment was associated with the Mn ions. First principle simulations showed that the strain-induced electronic redistribution of the two e_g orbitals (3d_z² and 3d_x²_-y²) of Mn ions was responsible for the change of magnetic moment. This work demonstrates that the magnetoelectric effect in manganite/piezoelectric hetero-structures originates from the change in eg orbital occupancy of Mn ions induced by strain rather than the interfacial effect.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC00112704; AC02-06CH11357; AC02-98CH10886

OSTI ID:: 1226033

Alternate ID(s):: OSTI ID: 1182853

Report Number(s):: BNL-108282-2015-JA; R&D Project: MA015MACA; KC0201010

Journal Information:: Physical Review. B, Condensed Matter and Materials Physics, Vol. 91, Issue 17; ISSN 1098-0121

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 6 works

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