Giant switchable photovoltaic effect in organometal trihalide perovskite devices

Xiao, Zhengguo; Yuan, Yongbo; Shao, Yuchuan; Wang, Qi; Dong, Qingfeng; Bi, Cheng; Sharma, Pankaj; Gruverman, Alexei; Huang, Jinsong

doi:10.1038/nmat4150

Title: Giant switchable photovoltaic effect in organometal trihalide perovskite devices

Journal Article · Mon Dec 08 00:00:00 EST 2014 · Nature Materials

DOI:https://doi.org/10.1038/nmat4150· OSTI ID:1238052

Xiao, Zhengguo ^[1]; Yuan, Yongbo ^[1]; Shao, Yuchuan ^[1]; Wang, Qi ^[1]; Dong, Qingfeng ^[1]; Bi, Cheng ^[1]; Sharma, Pankaj ^[1]; Gruverman, Alexei ^[1]; Huang, Jinsong ^[1]

Univ. of Nebraska, Lincoln, NE (United States)

Organolead trihalide perovskite (OTP) materials are emerging as naturally abundant materials for low-cost, solution-processed and highly efficient solar cells. Here, we show that, in OTP-based photovoltaic devices with vertical and lateral cell configurations, the photocurrent direction can be switched repeatedly by applying a small electric field of <1 V μm^–1. The switchable photocurrent, generally observed in devices based on ferroelectric materials, reached 20.1 mA cm^–2 under one sun illumination in OTP devices with a vertical architecture, which is four orders of magnitude larger than that measured in other ferroelectric photovoltaic devices. This field-switchable photovoltaic effect can be explained by the formation of reversible p–i–n structures induced by ion drift in the perovskite layer. Furthermore, the demonstration of switchable OTP photovoltaics and electric-field-manipulated doping paves the way for innovative solar cell designs and for the exploitation of OTP materials in electrically and optically readable memristors and circuits.

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Research Organization:: Univ. of Nebraska, Lincoln, NE (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: EE0006709

OSTI ID:: 1238052

Journal Information:: Nature Materials, Vol. 14, Issue 2; ISSN 1476-1122

Publisher:: Springer Nature - Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Communicating Two States in Perovskite Revealed by Time-Resolved Photoluminescence Spectroscopy Chen, Yanwen; Wang, Tianmeng; Li, Zhipeng arXiv https://doi.org/10.48550/arxiv.1811.00704	preprint	January 2018
Modeling Thin Film Solar Cells: From Organic to Perovskite Li, Deli; Song, Lin; Chen, Yonghua Advanced Science, Vol. 7, Issue 1 https://doi.org/10.1002/advs.201901397	journal	November 2019
What Is Moving in Hybrid Halide Perovskite Solar Cells? Frost, Jarvist M.; Walsh, Aron Accounts of Chemical Research, Vol. 49, Issue 3 https://doi.org/10.1021/acs.accounts.5b00431	journal	February 2016
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Thermodynamic Origin of Photoinstability in the CH ₃ NH ₃ Pb(I _{1– x} Br _x ) ₃ Hybrid Halide Perovskite Alloy Brivio, Federico; Caetano, Clovis; Walsh, Aron The Journal of Physical Chemistry Letters, Vol. 7, Issue 6 https://doi.org/10.1021/acs.jpclett.6b00226	journal	March 2016
Photoluminescence Blinking of Single-Crystal Methylammonium Lead Iodide Perovskite Nanorods Induced by Surface Traps Yuan, Haifeng; Debroye, Elke; Caliandro, Giorgio ACS Omega, Vol. 1, Issue 1 https://doi.org/10.1021/acsomega.6b00107	journal	July 2016
Effect of Cs-Incorporated NiO_x on the Performance of Perovskite Solar Cells Kim, Hui-Seon; Seo, Ji-Youn; Xie, Haibing ACS Omega, Vol. 2, Issue 12 https://doi.org/10.1021/acsomega.7b01179	journal	December 2017
Effect of Ion Migration-Induced Electrode Degradation on the Operational Stability of Perovskite Solar Cells Rivkin, Boris; Fassl, Paul; Sun, Qing ACS Omega, Vol. 3, Issue 8 https://doi.org/10.1021/acsomega.8b01626	journal	August 2018
Solid-State Ionics of Hybrid Halide Perovskites Senocrate, Alessandro; Maier, Joachim Journal of the American Chemical Society, Vol. 141, Issue 21 https://doi.org/10.1021/jacs.8b13594	journal	April 2019
Carrier separation and transport in perovskite solar cells studied by nanometre-scale profiling of electrical potential Jiang, Chun-Sheng; Yang, Mengjin; Zhou, Yuanyuan Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms9397	journal	September 2015
Management of transition dipoles in organic hole-transporting materials under solar irradiation for perovskite solar cells Ok, Song Ah; Jo, Bonghyun; Somasundaram, Sivaraman Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-06998-1	journal	October 2018
Application of ferroelectric materials for improving output power of energy harvesters. Kim, Tae Yun; Kim, Sung Kyun; Kim, Sang-Woo Springer Science and Business Media LLC https://doi.org/10.17863/cam.34465	journalarticle	January 2018
Fast Anion-Exchange in Highly Luminescent Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, I) Georgian, Nedelcu,; Loredana, Protesescu,; Sergii, Yakunin, ETH Zurich https://doi.org/10.3929/ethz-b-000103602	text	January 2015
Ambipolar Solution-processed Hybrid Perovskite Phototransistors Li, Feng; Ma, Chun; Wang, Hong arXiv https://doi.org/10.48550/arxiv.1502.03995	text	January 2015
Evidence for ion migration in hybrid perovskite solar cells with minimal hysteresis Calado, Philip; Telford, Andrew M.; Bryant, Daniel arXiv https://doi.org/10.48550/arxiv.1606.00818	text	January 2016
Dipole-field-assisted charge extraction in metal-perovskite-metal back-contact solar cells Lin, Xiongfeng; Jumabekov, Askhat N.; Lal, Niraj N. arXiv https://doi.org/10.48550/arxiv.1705.07963	text	January 2017

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