Recent advances of two-dimensional material additives in hybrid perovskite solar cells
Abstract
Perovskite solar cells (PSCs) have become one of the state-of-the-art photovoltaic technologies due to their facile solution-based fabrication processes combined with extremely high photovoltaic performance originating from excellent optoelectronic properties such as strong light absorption, high charge mobility, long free charge carrier diffusion length, and tunable direct bandgap. However, the poor intrinsic stability of hybrid perovskites under environmental stresses including light, heat, and moisture, which is often associated with high defect density in the perovskite, has limited the large-scale commercialization and deployment of PSCs. The use of process additives, which can be included in various subcomponent layers in the PSC, has been identified as one of the effective approaches that can address these issues and improve the photovoltaic performance. Among various additives that have been explored, two-dimensional (2D) materials have emerged recently due to their unique structures and properties that can enhance the photovoltaic performance and device stability by improving perovskite crystallization, defect passivation, and charge transport. In this work, we provide a review of the recent progresses in 2D material additives for improving the PSC performance based on key representative 2D material systems, including graphene and its derivatives, transitional metal dichalcogenides, and black phosphorous, providing a useful guideline formore »
- Authors:
-
- Stony Brook Univ., NY (United States)
- Stony Brook Univ., NY (United States); Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)
- Publication Date:
- Research Org.:
- Brookhaven National Laboratory (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); US Department of the Navy, Office of Naval Research (ONR)
- OSTI Identifier:
- 1969363
- Report Number(s):
- BNL-224215-2023-JAAM
Journal ID: ISSN 0957-4484
- Grant/Contract Number:
- SC0012704; N000142012858
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nanotechnology
- Additional Journal Information:
- Journal Volume: 34; Journal Issue: 17; Journal ID: ISSN 0957-4484
- Publisher:
- IOP Publishing
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY
Citation Formats
Yin, Yifan, Zhou, Yuchen, Rafailovich, Miriam H., and Nam, Chang-Yong. Recent advances of two-dimensional material additives in hybrid perovskite solar cells. United States: N. p., 2023.
Web. doi:10.1088/1361-6528/acb441.
Yin, Yifan, Zhou, Yuchen, Rafailovich, Miriam H., & Nam, Chang-Yong. Recent advances of two-dimensional material additives in hybrid perovskite solar cells. United States. https://doi.org/10.1088/1361-6528/acb441
Yin, Yifan, Zhou, Yuchen, Rafailovich, Miriam H., and Nam, Chang-Yong. Fri .
"Recent advances of two-dimensional material additives in hybrid perovskite solar cells". United States. https://doi.org/10.1088/1361-6528/acb441. https://www.osti.gov/servlets/purl/1969363.
@article{osti_1969363,
title = {Recent advances of two-dimensional material additives in hybrid perovskite solar cells},
author = {Yin, Yifan and Zhou, Yuchen and Rafailovich, Miriam H. and Nam, Chang-Yong},
abstractNote = {Perovskite solar cells (PSCs) have become one of the state-of-the-art photovoltaic technologies due to their facile solution-based fabrication processes combined with extremely high photovoltaic performance originating from excellent optoelectronic properties such as strong light absorption, high charge mobility, long free charge carrier diffusion length, and tunable direct bandgap. However, the poor intrinsic stability of hybrid perovskites under environmental stresses including light, heat, and moisture, which is often associated with high defect density in the perovskite, has limited the large-scale commercialization and deployment of PSCs. The use of process additives, which can be included in various subcomponent layers in the PSC, has been identified as one of the effective approaches that can address these issues and improve the photovoltaic performance. Among various additives that have been explored, two-dimensional (2D) materials have emerged recently due to their unique structures and properties that can enhance the photovoltaic performance and device stability by improving perovskite crystallization, defect passivation, and charge transport. In this work, we provide a review of the recent progresses in 2D material additives for improving the PSC performance based on key representative 2D material systems, including graphene and its derivatives, transitional metal dichalcogenides, and black phosphorous, providing a useful guideline for further exploiting unique nanomaterial additives for more efficient and stable PSCs in the near future.},
doi = {10.1088/1361-6528/acb441},
journal = {Nanotechnology},
number = 17,
volume = 34,
place = {United States},
year = {Fri Feb 10 00:00:00 EST 2023},
month = {Fri Feb 10 00:00:00 EST 2023}
}
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