Photoionization of metastable heliumlike ions: Precision study of intermediate doubly excited states
Abstract
In a joint experimental and theoretical endeavor, photoionization of metastable C4+(1s2s3S1) ions via intermediate levels with hollow, double-K-vacancy configurations 2s2p, 2s3p, 2p3s, 2p3d, 2s4p, 2p4s, and 2p4d has been investigated. High-resolution photon-ion merged-beams measurements were carried out with the resolving power reaching up to 25 800 which is sufficient to separate the leading fine-structure components of the 2s2p 3P term. Many-body perturbation theory was employed to determine level-to-level cross sections for K-shell excitation with subsequent autoionization. The resonance energies were calculated with inclusion of electron correlation and radiative contributions. Their uncertainties are estimated to be below ±1 meV. Detailed balance confirms the present photoionization cross-section results by comparison with previous dielectronic-recombination measurements. Finally, the high accuracy of the theoretical transition energies together with the present experimental results qualify photoabsorption resonances in heliumlike ions as new, greatly improved energy-reference standards at synchrotron radiation facilities.
- Authors:
-
- Justus-Liebig-Univ., Giessen (Germany)
- Alba Nova Univ. Center, Stockholm (Sweden)
- Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
- GSI Helmholtzzentrum fur Schwerionenforschung, Darmstadt (Germany); Columbia Univ., New York, NY (United States)
- Sorbonne Univ., Paris (France)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
- Univ. Hamburg (Germany)
- Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Helmholtz-Zentrum, Berlin (Germany)
- Justus-Liebig-Univ., Giessen (Germany); Max-Planck-Inst. fur Kernphysik, Heidelberg (Germany)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); Bundesministerium fur Bildung und Forschung; European Union (EU); Helmholtz Association; Swedish Research Council (SRC)
- OSTI Identifier:
- 1604650
- Grant/Contract Number:
- AC02-05CH11231; 05K10RG1; 05K10GUB; 05K16RG1; 05K16GUV; 654220; EMMI HA-216; 2016-03789
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review A
- Additional Journal Information:
- Journal Volume: 98; Journal Issue: 3; Journal ID: ISSN 2469-9926
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 74 ATOMIC AND MOLECULAR PHYSICS; atomic & molecular structure; autoionization & Auger processes; electronic structure of atoms & molecules; electronic transitions; relativistic & quantum electrodynamic effects in atoms, molecules, & ions; single- and few-photon ionization & excitation
Citation Formats
Müller, A., Lindroth, E., Bari, S., Borovik, A., Hillenbrand, P. -M., Holste, K., Indelicato, P., Kilcoyne, A. L. D., Klumpp, S., Martins, M., Viefhaus, J., Wilhelm, P., and Schippers, S. Photoionization of metastable heliumlike C4+(1s2sS13) ions: Precision study of intermediate doubly excited states. United States: N. p., 2018.
Web. doi:10.1103/PhysRevA.98.033416.
Müller, A., Lindroth, E., Bari, S., Borovik, A., Hillenbrand, P. -M., Holste, K., Indelicato, P., Kilcoyne, A. L. D., Klumpp, S., Martins, M., Viefhaus, J., Wilhelm, P., & Schippers, S. Photoionization of metastable heliumlike C4+(1s2sS13) ions: Precision study of intermediate doubly excited states. United States. https://doi.org/10.1103/PhysRevA.98.033416
Müller, A., Lindroth, E., Bari, S., Borovik, A., Hillenbrand, P. -M., Holste, K., Indelicato, P., Kilcoyne, A. L. D., Klumpp, S., Martins, M., Viefhaus, J., Wilhelm, P., and Schippers, S. Tue .
"Photoionization of metastable heliumlike C4+(1s2sS13) ions: Precision study of intermediate doubly excited states". United States. https://doi.org/10.1103/PhysRevA.98.033416. https://www.osti.gov/servlets/purl/1604650.
@article{osti_1604650,
title = {Photoionization of metastable heliumlike C4+(1s2sS13) ions: Precision study of intermediate doubly excited states},
author = {Müller, A. and Lindroth, E. and Bari, S. and Borovik, A. and Hillenbrand, P. -M. and Holste, K. and Indelicato, P. and Kilcoyne, A. L. D. and Klumpp, S. and Martins, M. and Viefhaus, J. and Wilhelm, P. and Schippers, S.},
abstractNote = {In a joint experimental and theoretical endeavor, photoionization of metastable C4+(1s2s3S1) ions via intermediate levels with hollow, double-K-vacancy configurations 2s2p, 2s3p, 2p3s, 2p3d, 2s4p, 2p4s, and 2p4d has been investigated. High-resolution photon-ion merged-beams measurements were carried out with the resolving power reaching up to 25 800 which is sufficient to separate the leading fine-structure components of the 2s2p 3P term. Many-body perturbation theory was employed to determine level-to-level cross sections for K-shell excitation with subsequent autoionization. The resonance energies were calculated with inclusion of electron correlation and radiative contributions. Their uncertainties are estimated to be below ±1 meV. Detailed balance confirms the present photoionization cross-section results by comparison with previous dielectronic-recombination measurements. Finally, the high accuracy of the theoretical transition energies together with the present experimental results qualify photoabsorption resonances in heliumlike ions as new, greatly improved energy-reference standards at synchrotron radiation facilities.},
doi = {10.1103/PhysRevA.98.033416},
journal = {Physical Review A},
number = 3,
volume = 98,
place = {United States},
year = {Tue Sep 25 00:00:00 EDT 2018},
month = {Tue Sep 25 00:00:00 EDT 2018}
}
Web of Science
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Works referencing / citing this record:
The photon‐ion merged‐beams experiment PIPE at PETRA III—The first five years
text, January 2020
- Schippers, Stefan; Buhr, Ticia; Borovik, Alexander
- GSI Helmholtzzentrum fuer Schwerionenforschung, GSI, Darmstadt
The photon‐ion merged‐beams experiment PIPE at PETRA III—The first five years
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Photoionization and photofragmentation of singly charged positive and negative endohedral fullerene ions
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Photoionization and photofragmentation of singly charged positive and negative Sc$_3$N@C$_{80}$ endohedral fullerene ions
text, January 2019
- Mueller, Alfred; Martins, M.; Kilcoyne, A. L. D.
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
The photon‐ion merged‐beams experiment PIPE at PETRA III—The first five years
text, January 2019
- Schippers, Stefan; Buhr, Ticia; Borovik, Alexander
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Multiple Photodetachment of Carbon Anions via Single and Double Core-Hole Creation
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- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Complex scaled relativistic configuration-interaction study of the $LL$ resonances in helium-like ions: from Boron to Argon
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