A dual-chamber method for quantifying the effects of atmospheric perturbations on secondary organic aerosol formation from biomass burning emissions: Investigation of Biomass Burning SOA
Abstract
Biomass burning (BB) is a major source of atmospheric pollutants. Field and laboratory studies indicate that secondary organic aerosol (SOA) formation from BB emissions is highly variable. We investigated sources of this variability using a novel dual-smog-chamber method that directly compares the SOA formation from the same BB emissions under two different atmospheric conditions. During each experiment, we filled two identical Teflon smog chambers simultaneously with BB emissions from the same fire. We then perturbed the smoke with UV lights, UV lights plus nitrous acid (HONO), or dark ozone in one or both chambers. These perturbations caused SOA formation in nearly every experiment with an average organic aerosol (OA) mass enhancement ratio of 1.78 ± 0.91 (mean ± 1σ). However, the effects of the perturbations were highly variable ranging with OA mass enhancement ratios ranging from 0.7 (30% loss of OA mass) to 4.4 across the set of perturbation experiments. There was no apparent relationship between OA enhancement and perturbation type, fuel type, and modified combustion efficiency. To better isolate the effects of different perturbations, we report dual-chamber enhancement (DUCE), which is the quantity of the effects of a perturbation relative to a reference condition. DUCE values were also highlymore »
- Authors:
-
- Carnegie Mellon Univ., Pittsburgh, PA (United States)
- Univ. of Montana, Missoula, MT (United States)
- National Oceanic and Atmospheric Administration (NOAA), Boulder, CO (United States). Earth System Research Lab.
- Univ. of California, Irvine, CA (United States)
- Publication Date:
- Research Org.:
- Carnegie Mellon Univ., Pittsburgh, PA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1532986
- Grant/Contract Number:
- SC0007075
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Geophysical Research: Atmospheres
- Additional Journal Information:
- Journal Volume: 122; Journal Issue: 11; Journal ID: ISSN 2169-897X
- Publisher:
- American Geophysical Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES; Meteorology & Atmospheric Sciences
Citation Formats
Tkacik, Daniel S., Robinson, Ellis S., Ahern, Adam, Saleh, Rawad, Stockwell, Chelsea, Veres, Patrick, Simpson, Isobel J., Meinardi, Simone, Blake, Donald R., Yokelson, Robert J., Presto, Albert A., Sullivan, Ryan C., Donahue, Neil M., and Robinson, Allen L. A dual-chamber method for quantifying the effects of atmospheric perturbations on secondary organic aerosol formation from biomass burning emissions: Investigation of Biomass Burning SOA. United States: N. p., 2017.
Web. doi:10.1002/2016jd025784.
Tkacik, Daniel S., Robinson, Ellis S., Ahern, Adam, Saleh, Rawad, Stockwell, Chelsea, Veres, Patrick, Simpson, Isobel J., Meinardi, Simone, Blake, Donald R., Yokelson, Robert J., Presto, Albert A., Sullivan, Ryan C., Donahue, Neil M., & Robinson, Allen L. A dual-chamber method for quantifying the effects of atmospheric perturbations on secondary organic aerosol formation from biomass burning emissions: Investigation of Biomass Burning SOA. United States. https://doi.org/10.1002/2016jd025784
Tkacik, Daniel S., Robinson, Ellis S., Ahern, Adam, Saleh, Rawad, Stockwell, Chelsea, Veres, Patrick, Simpson, Isobel J., Meinardi, Simone, Blake, Donald R., Yokelson, Robert J., Presto, Albert A., Sullivan, Ryan C., Donahue, Neil M., and Robinson, Allen L. Wed .
"A dual-chamber method for quantifying the effects of atmospheric perturbations on secondary organic aerosol formation from biomass burning emissions: Investigation of Biomass Burning SOA". United States. https://doi.org/10.1002/2016jd025784. https://www.osti.gov/servlets/purl/1532986.
@article{osti_1532986,
title = {A dual-chamber method for quantifying the effects of atmospheric perturbations on secondary organic aerosol formation from biomass burning emissions: Investigation of Biomass Burning SOA},
author = {Tkacik, Daniel S. and Robinson, Ellis S. and Ahern, Adam and Saleh, Rawad and Stockwell, Chelsea and Veres, Patrick and Simpson, Isobel J. and Meinardi, Simone and Blake, Donald R. and Yokelson, Robert J. and Presto, Albert A. and Sullivan, Ryan C. and Donahue, Neil M. and Robinson, Allen L.},
abstractNote = {Biomass burning (BB) is a major source of atmospheric pollutants. Field and laboratory studies indicate that secondary organic aerosol (SOA) formation from BB emissions is highly variable. We investigated sources of this variability using a novel dual-smog-chamber method that directly compares the SOA formation from the same BB emissions under two different atmospheric conditions. During each experiment, we filled two identical Teflon smog chambers simultaneously with BB emissions from the same fire. We then perturbed the smoke with UV lights, UV lights plus nitrous acid (HONO), or dark ozone in one or both chambers. These perturbations caused SOA formation in nearly every experiment with an average organic aerosol (OA) mass enhancement ratio of 1.78 ± 0.91 (mean ± 1σ). However, the effects of the perturbations were highly variable ranging with OA mass enhancement ratios ranging from 0.7 (30% loss of OA mass) to 4.4 across the set of perturbation experiments. There was no apparent relationship between OA enhancement and perturbation type, fuel type, and modified combustion efficiency. To better isolate the effects of different perturbations, we report dual-chamber enhancement (DUCE), which is the quantity of the effects of a perturbation relative to a reference condition. DUCE values were also highly variable, even for the same perturbation and fuel type. Gas measurements indicate substantial burn-to-burn variability in the magnitude and composition of SOA precursor emissions, even in repeated burns of the same fuel under nominally identical conditions. Therefore, the effects of different atmospheric perturbations on SOA formation from BB emissions appear to be less important than burn-to-burn variability.},
doi = {10.1002/2016jd025784},
journal = {Journal of Geophysical Research: Atmospheres},
number = 11,
volume = 122,
place = {United States},
year = {Wed May 03 00:00:00 EDT 2017},
month = {Wed May 03 00:00:00 EDT 2017}
}
Web of Science
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Secondary Organic Aerosol Formation from Acetylene (C 2 H 2 ): seed effect on SOA yields due to organic photochemistry in the aerosol aqueous phase
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Emissions from biomass burning in the Yucatan
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Coupling field and laboratory measurements to estimate the emission factors of identified and unidentified trace gases for prescribed fires
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Absorptivity of brown carbon in fresh and photo-chemically aged biomass-burning emissions
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Ozone photochemistry in boreal biomass burning plumes
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The formation, properties and impact of secondary organic aerosol: current and emerging issues
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Secondary organic aerosol formation from photooxidation of naphthalene and alkylnaphthalenes: implications for oxidation of intermediate volatility organic compounds (IVOCs)
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