Thermal conductivity in self-assembled CoFe2O4/BiFeO3 vertical nanocomposite films
Abstract
The thermal conductivity of self-assembled nanocomposite oxide films consisting of cobalt ferrite (CFO) spinel pillars grown within a single-crystal bismuth ferrite (BFO) perovskite matrix is described as a function of the volume fraction of the spinel. Single phase BFO and CFO had cross-plane thermal conductivities of 1.32 W m–1 K–1 and 3.94 W m–1 K–1, respectively, and the thermal conductivity of the nanocomposites increased with the CFO volume fraction within this range. A small increase (~5%) in thermal conductivity for the pure CFO phase in the AC-demagnetized state was observed, suggesting possible magnon contributions. As a result, steady state gray-medium based variance-reduced Monte Carlo simulations show consistent trends with experimental data on the dependence of thermal conductivity with the CFO volume fraction.
- Authors:
-
[1];
[3];
- Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Shandong Univ., Qingdao (China)
- Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Solid-State Solar-Thermal Energy Conversion Center (S3TEC); Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
- OSTI Identifier:
- 1504764
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Applied Physics Letters
- Additional Journal Information:
- Journal Volume: 113; Journal Issue: 22; Journal ID: ISSN 0003-6951
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Zhang, Chen, Huberman, Samuel C., Ning, Shuai, Pelliciari, Jonathan, Duncan, Ryan A., Liao, Bolin, Ojha, Shuchi, Freeland, John W., Nelson, Keith A., Comin, Riccardo, Chen, Gang, and Ross, Caroline A. Thermal conductivity in self-assembled CoFe2O4/BiFeO3 vertical nanocomposite films. United States: N. p., 2018.
Web. doi:10.1063/1.5049176.
Zhang, Chen, Huberman, Samuel C., Ning, Shuai, Pelliciari, Jonathan, Duncan, Ryan A., Liao, Bolin, Ojha, Shuchi, Freeland, John W., Nelson, Keith A., Comin, Riccardo, Chen, Gang, & Ross, Caroline A. Thermal conductivity in self-assembled CoFe2O4/BiFeO3 vertical nanocomposite films. United States. https://doi.org/10.1063/1.5049176
Zhang, Chen, Huberman, Samuel C., Ning, Shuai, Pelliciari, Jonathan, Duncan, Ryan A., Liao, Bolin, Ojha, Shuchi, Freeland, John W., Nelson, Keith A., Comin, Riccardo, Chen, Gang, and Ross, Caroline A. Wed .
"Thermal conductivity in self-assembled CoFe2O4/BiFeO3 vertical nanocomposite films". United States. https://doi.org/10.1063/1.5049176. https://www.osti.gov/servlets/purl/1504764.
@article{osti_1504764,
title = {Thermal conductivity in self-assembled CoFe2O4/BiFeO3 vertical nanocomposite films},
author = {Zhang, Chen and Huberman, Samuel C. and Ning, Shuai and Pelliciari, Jonathan and Duncan, Ryan A. and Liao, Bolin and Ojha, Shuchi and Freeland, John W. and Nelson, Keith A. and Comin, Riccardo and Chen, Gang and Ross, Caroline A.},
abstractNote = {The thermal conductivity of self-assembled nanocomposite oxide films consisting of cobalt ferrite (CFO) spinel pillars grown within a single-crystal bismuth ferrite (BFO) perovskite matrix is described as a function of the volume fraction of the spinel. Single phase BFO and CFO had cross-plane thermal conductivities of 1.32 W m–1 K–1 and 3.94 W m–1 K–1, respectively, and the thermal conductivity of the nanocomposites increased with the CFO volume fraction within this range. A small increase (~5%) in thermal conductivity for the pure CFO phase in the AC-demagnetized state was observed, suggesting possible magnon contributions. As a result, steady state gray-medium based variance-reduced Monte Carlo simulations show consistent trends with experimental data on the dependence of thermal conductivity with the CFO volume fraction.},
doi = {10.1063/1.5049176},
journal = {Applied Physics Letters},
number = 22,
volume = 113,
place = {United States},
year = {Wed Nov 28 00:00:00 EST 2018},
month = {Wed Nov 28 00:00:00 EST 2018}
}
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