Rational Design of a Dual-Function Hybrid Cathode Substrate for Lithium-Sulfur Batteries
Abstract
Abstract A unique 3D hybrid sponge with chemically coupled nickel disulfide‐reduced graphene oxide (NiS 2 ‐RGO) framework is rationally developed as an effective polysulfide reservoir through a biomolecule‐assisted self‐assembly synthesis. An optimized amount of NiS 2 (≈18 wt%) with porous nanoflower‐like morphology is uniformly in situ grown on the RGO substrate, providing abundant active sites to adsorb and localize polysulfides. The improved polysulfide adsorptivity from sulfiphilic NiS 2 is confirmed by experimental data and first‐principle calculations. Moreover, due to the chemical coupling between NiS 2 and RGO formed during the in situ synthesis, the conductive RGO substrate offers a 3D electron pathway to facilitate charge transfer toward the NiS 2 ‐polysulfide adsorption interface, triggering a fast redox kinetics of polysulfide conversion and excellent rate performance (C/20–4C). Therefore, the self‐assembled hybrid structure simultaneously promotes static polysulfide‐trapping capability and dynamic polysulfide‐conversion reversibility. As a result, the 3D porous sponge enables a high sulfur content (75 wt%) and a remarkably high sulfur loading (up to 21 mg cm −2 ) and areal capacity (up to 16 mAh cm −2 ), exceeding most of the reported values in the literature involving either RGO or metal sulfides/other metal compounds (sulfur content of <60 wt% andmore »
- Publication Date:
- Research Org.:
- Univ. of Texas, Austin, TX (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE)
- OSTI Identifier:
- 1487463
- Alternate Identifier(s):
- OSTI ID: 1456284
- Grant/Contract Number:
- EE0007218; DE‐EE0007218
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Energy Materials
- Additional Journal Information:
- Journal Volume: 8; Journal Issue: 24; Journal ID: ISSN 1614-6832
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 25 ENERGY STORAGE; electrochemical performance; high‐loading cathodes; lithium–sulfur batteries; porous nanoflower‐like NiS2; reduced graphene oxide substrate
Citation Formats
Luo, Liu, Chung, Sheng -Heng, and Manthiram, Arumugam. Rational Design of a Dual-Function Hybrid Cathode Substrate for Lithium-Sulfur Batteries. United States: N. p., 2018.
Web. doi:10.1002/aenm.201801014.
Luo, Liu, Chung, Sheng -Heng, & Manthiram, Arumugam. Rational Design of a Dual-Function Hybrid Cathode Substrate for Lithium-Sulfur Batteries. United States. https://doi.org/10.1002/aenm.201801014
Luo, Liu, Chung, Sheng -Heng, and Manthiram, Arumugam. Thu .
"Rational Design of a Dual-Function Hybrid Cathode Substrate for Lithium-Sulfur Batteries". United States. https://doi.org/10.1002/aenm.201801014. https://www.osti.gov/servlets/purl/1487463.
@article{osti_1487463,
title = {Rational Design of a Dual-Function Hybrid Cathode Substrate for Lithium-Sulfur Batteries},
author = {Luo, Liu and Chung, Sheng -Heng and Manthiram, Arumugam},
abstractNote = {Abstract A unique 3D hybrid sponge with chemically coupled nickel disulfide‐reduced graphene oxide (NiS 2 ‐RGO) framework is rationally developed as an effective polysulfide reservoir through a biomolecule‐assisted self‐assembly synthesis. An optimized amount of NiS 2 (≈18 wt%) with porous nanoflower‐like morphology is uniformly in situ grown on the RGO substrate, providing abundant active sites to adsorb and localize polysulfides. The improved polysulfide adsorptivity from sulfiphilic NiS 2 is confirmed by experimental data and first‐principle calculations. Moreover, due to the chemical coupling between NiS 2 and RGO formed during the in situ synthesis, the conductive RGO substrate offers a 3D electron pathway to facilitate charge transfer toward the NiS 2 ‐polysulfide adsorption interface, triggering a fast redox kinetics of polysulfide conversion and excellent rate performance (C/20–4C). Therefore, the self‐assembled hybrid structure simultaneously promotes static polysulfide‐trapping capability and dynamic polysulfide‐conversion reversibility. As a result, the 3D porous sponge enables a high sulfur content (75 wt%) and a remarkably high sulfur loading (up to 21 mg cm −2 ) and areal capacity (up to 16 mAh cm −2 ), exceeding most of the reported values in the literature involving either RGO or metal sulfides/other metal compounds (sulfur content of <60 wt% and sulfur loading of <3 mg cm −2 ).},
doi = {10.1002/aenm.201801014},
journal = {Advanced Energy Materials},
number = 24,
volume = 8,
place = {United States},
year = {Thu Jun 21 00:00:00 EDT 2018},
month = {Thu Jun 21 00:00:00 EDT 2018}
}
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Figures / Tables:
Scheme 1: (a) Synthesis procedure of the hybrid NiS2-RGO sponge. (b) Illustration of the advantage of the hybrid NiS2-RGO sponge for static polysulfide-trapping and dynamic polysulfide-conversion capability.
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