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Title: Using 3D position sensitivity to reveal response non-uniformities in CdZnTe, TlBr, and CsPbBr3 detectors

Abstract

Position sensitivity enables the correction of response non-uniformities in room-temperature semiconductor detectors caused by crystal defects and other factors. It can also be used to pinpoint the exact location of crystal defects responsible for the response variations. This work describes a technique for revealing and visualizing the detector regions affecting the charge collection efficiency in CdZnTe (CZT), TlBr, and CsPbBr3 detectors configured as position-sensitive virtual Frisch-grid (VFG) devices. The technique correlates the photopeak events in energy spectra with their spatial distributions inside the detectors using the position information. By selecting the events from narrow energy intervals within a photopeak, we can visualize the detector volumes with particular charge collection efficiencies, which, in turn, correlate with the locations of electrode and crystal defects. Here, we demonstrate this technique in several examples. Columnar structures in the volume plots (position distribution maps) are consistent with signal losses near or at the anode in selected samples of CZT and TlBr. Structures exhibiting a distinct depth dependence are consistent with grain boundaries or other crystal defects.

Authors:
ORCiD logo [1];  [2];  [1]; ORCiD logo [2];  [2];  [1];  [1];  [1];  [1];  [1];  [2]; ORCiD logo [2];  [3];  [1];  [1];  [3];  [1];  [3];  [2];  [1] more »; ORCiD logo [1];  [3];  [2];  [2];  [2];  [3];  [2];  [2] « less
  1. Brookhaven National Laboratory (BNL), Upton, NY (United States)
  2. Radiation Monitoring Devices, Inc., Watertown, MA (United States)
  3. Bubble Technology Industries, Chalk River, ON (Canada)
Publication Date:
Research Org.:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE; US Department of Homeland Security (DHS)
OSTI Identifier:
2311079
Report Number(s):
BNL-225310-2024-JAAM
Journal ID: ISSN 0168-9002
Grant/Contract Number:  
SC0012704; 70RDND18C00000024
Resource Type:
Accepted Manuscript
Journal Name:
Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment
Additional Journal Information:
Journal Volume: 1057; Journal ID: ISSN 0168-9002
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL PROTECTION; room temperature semiconductor gamma-ray detectors; CdZnTe; TlBr; CsPbBr3; high granularity detectors; crystal defects; position-sensitive virtual Frisch-grid detectors

Citation Formats

Bolotnikov, Aleksey E., Brown, C. A., Carini, G. A., Christian, James, Cirignano, L., Deane, C. R., Dellapenna, A., Deptuch, G., Fried, J., Herrmann, S., Kargar, A., Kim, Hadong, Koslowsky, M. R., Maj, P., Manthena, S. V., Miller, A. L., Miryala, S., Norris, A. M., Ogorodnik, Y., Pinaroli, G., Raguzin, Eric, Smith, M. B., Squillante, M. R., Squillante, M. S., Tower, J., Valente, A. J., Weststrate, E., and Shah, K. S. Using 3D position sensitivity to reveal response non-uniformities in CdZnTe, TlBr, and CsPbBr3 detectors. United States: N. p., 2023. Web. doi:10.1016/j.nima.2023.168785.
Bolotnikov, Aleksey E., Brown, C. A., Carini, G. A., Christian, James, Cirignano, L., Deane, C. R., Dellapenna, A., Deptuch, G., Fried, J., Herrmann, S., Kargar, A., Kim, Hadong, Koslowsky, M. R., Maj, P., Manthena, S. V., Miller, A. L., Miryala, S., Norris, A. M., Ogorodnik, Y., Pinaroli, G., Raguzin, Eric, Smith, M. B., Squillante, M. R., Squillante, M. S., Tower, J., Valente, A. J., Weststrate, E., & Shah, K. S. Using 3D position sensitivity to reveal response non-uniformities in CdZnTe, TlBr, and CsPbBr3 detectors. United States. https://doi.org/10.1016/j.nima.2023.168785
Bolotnikov, Aleksey E., Brown, C. A., Carini, G. A., Christian, James, Cirignano, L., Deane, C. R., Dellapenna, A., Deptuch, G., Fried, J., Herrmann, S., Kargar, A., Kim, Hadong, Koslowsky, M. R., Maj, P., Manthena, S. V., Miller, A. L., Miryala, S., Norris, A. M., Ogorodnik, Y., Pinaroli, G., Raguzin, Eric, Smith, M. B., Squillante, M. R., Squillante, M. S., Tower, J., Valente, A. J., Weststrate, E., and Shah, K. S. Thu . "Using 3D position sensitivity to reveal response non-uniformities in CdZnTe, TlBr, and CsPbBr3 detectors". United States. https://doi.org/10.1016/j.nima.2023.168785.
@article{osti_2311079,
title = {Using 3D position sensitivity to reveal response non-uniformities in CdZnTe, TlBr, and CsPbBr3 detectors},
author = {Bolotnikov, Aleksey E. and Brown, C. A. and Carini, G. A. and Christian, James and Cirignano, L. and Deane, C. R. and Dellapenna, A. and Deptuch, G. and Fried, J. and Herrmann, S. and Kargar, A. and Kim, Hadong and Koslowsky, M. R. and Maj, P. and Manthena, S. V. and Miller, A. L. and Miryala, S. and Norris, A. M. and Ogorodnik, Y. and Pinaroli, G. and Raguzin, Eric and Smith, M. B. and Squillante, M. R. and Squillante, M. S. and Tower, J. and Valente, A. J. and Weststrate, E. and Shah, K. S.},
abstractNote = {Position sensitivity enables the correction of response non-uniformities in room-temperature semiconductor detectors caused by crystal defects and other factors. It can also be used to pinpoint the exact location of crystal defects responsible for the response variations. This work describes a technique for revealing and visualizing the detector regions affecting the charge collection efficiency in CdZnTe (CZT), TlBr, and CsPbBr3 detectors configured as position-sensitive virtual Frisch-grid (VFG) devices. The technique correlates the photopeak events in energy spectra with their spatial distributions inside the detectors using the position information. By selecting the events from narrow energy intervals within a photopeak, we can visualize the detector volumes with particular charge collection efficiencies, which, in turn, correlate with the locations of electrode and crystal defects. Here, we demonstrate this technique in several examples. Columnar structures in the volume plots (position distribution maps) are consistent with signal losses near or at the anode in selected samples of CZT and TlBr. Structures exhibiting a distinct depth dependence are consistent with grain boundaries or other crystal defects.},
doi = {10.1016/j.nima.2023.168785},
journal = {Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment},
number = ,
volume = 1057,
place = {United States},
year = {Thu Oct 12 00:00:00 EDT 2023},
month = {Thu Oct 12 00:00:00 EDT 2023}
}

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Works referenced in this record:

Developing Larger TlBr Detectors—Detector Performance
journal, June 2009

  • Kim, H.; Cirignano, L.; Churilov, A.
  • IEEE Transactions on Nuclear Science, Vol. 56, Issue 3
  • DOI: 10.1109/TNS.2009.2014756

Perovskite CsPbBr3 single crystal detector for alpha-particle spectroscopy
journal, April 2019

  • He, Yihui; Liu, Zhifu; McCall, Kyle M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 922
  • DOI: 10.1016/j.nima.2019.01.008

Thallium bromide radiation detectors
journal, January 1989

  • Shah, K. S.; Lund, J. C.; Olschner, F.
  • IEEE Transactions on Nuclear Science, Vol. 36, Issue 1
  • DOI: 10.1109/23.34434

High spectral resolution of gamma-rays at room temperature by perovskite CsPbBr3 single crystals
journal, April 2018


An array of virtual Frisch-grid CdZnTe detectors and a front-end application-specific integrated circuit for large-area position-sensitive gamma-ray cameras
journal, July 2015

  • Bolotnikov, A. E.; Ackley, K.; Camarda, G. S.
  • Review of Scientific Instruments, Vol. 86, Issue 7
  • DOI: 10.1063/1.4927455