DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Spontaneous fluctuations in a magnetic Fe/Gd skyrmion lattice

Abstract

Magnetic skyrmions are topological spin textures that exhibit classical or quantum quasi-particle behavior. A substantial amount of research has occurred in this field, both because of their unique electromagnetic properties and potential application for future nonvolatile memory storage applications, as well as fundamental questions on their topology and unique magnetic phases. Here, we investigate the fluctuation properties of a magnetic Fe/Gd skyrmion lattice, using short-pulsed xrays. We first measure spontaneous fluctuations of the skyrmion lattice phase and find an inherent, collective mode showing an underdamped oscillation with a relaxation of a couple of nanoseconds. Further observations track the response towards the continuous phase transition and a ‘critical-like’ slowing down of fluctuations is observed well before the critical point. These results suggest that the skyrmion lattice phase never fully freezes into a static crystal. This constant state of fluctuation indicates that the physics of topological magnetic phases may have more in common with high-temperature superconductors with disorder.

Authors:
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; more »; ; ; ; ; ; ; ORCiD logo « less
Publication Date:
Research Org.:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division
Contributing Org.:
U.S Office of Naval Research (provided funding but is not on your list), University of Nebraska (Nebraska EPSCoR under the FIRST Award #OIA-1557417), UC San Diego, UC Santa Cruz, Stanford University.
OSTI Identifier:
1820477
Alternate Identifier(s):
OSTI ID: 1817694
Grant/Contract Number:  
AC02-76SF00515; AC02-05-CH11231
Resource Type:
Published Article
Journal Name:
Physical Review Research
Additional Journal Information:
Journal Name: Physical Review Research Journal Volume: 3 Journal Issue: 3; Journal ID: ISSN 2643-1564
Publisher:
American Physical Society
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 77 NANOSCIENCE AND NANOTECHNOLOGY; 97 MATHEMATICS AND COMPUTING; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; 47 OTHER INSTRUMENTATION; 36 MATERIALS SCIENCE; x-rays; coherence; skyrminos; magnetism; ultrafast; resonant scattering; XPCS; XFEL; materials; condensed matter; topological phases; fluctuations

Citation Formats

Seaberg, M. H., Holladay, B., Montoya, S. A., Zheng, X. Y., Lee, J. C. T., Reid, A. H., Koralek, J. D., Shen, L., Esposito, V., Coslovich, G., Walter, P., Zohar, S., Thampy, V., Lin, M. F., Hart, P., Nakahara, K., Streubel, R., Kevan, S. D., Fischer, P., Colocho, W., Lutman, A., Decker, F. -J., Fullerton, E. E., Dunne, M., Roy, S., Sinha, S. K., and Turner, J. J. Spontaneous fluctuations in a magnetic Fe/Gd skyrmion lattice. United States: N. p., 2021. Web. doi:10.1103/PhysRevResearch.3.033249.
Seaberg, M. H., Holladay, B., Montoya, S. A., Zheng, X. Y., Lee, J. C. T., Reid, A. H., Koralek, J. D., Shen, L., Esposito, V., Coslovich, G., Walter, P., Zohar, S., Thampy, V., Lin, M. F., Hart, P., Nakahara, K., Streubel, R., Kevan, S. D., Fischer, P., Colocho, W., Lutman, A., Decker, F. -J., Fullerton, E. E., Dunne, M., Roy, S., Sinha, S. K., & Turner, J. J. Spontaneous fluctuations in a magnetic Fe/Gd skyrmion lattice. United States. https://doi.org/10.1103/PhysRevResearch.3.033249
Seaberg, M. H., Holladay, B., Montoya, S. A., Zheng, X. Y., Lee, J. C. T., Reid, A. H., Koralek, J. D., Shen, L., Esposito, V., Coslovich, G., Walter, P., Zohar, S., Thampy, V., Lin, M. F., Hart, P., Nakahara, K., Streubel, R., Kevan, S. D., Fischer, P., Colocho, W., Lutman, A., Decker, F. -J., Fullerton, E. E., Dunne, M., Roy, S., Sinha, S. K., and Turner, J. J. Wed . "Spontaneous fluctuations in a magnetic Fe/Gd skyrmion lattice". United States. https://doi.org/10.1103/PhysRevResearch.3.033249.
@article{osti_1820477,
title = {Spontaneous fluctuations in a magnetic Fe/Gd skyrmion lattice},
author = {Seaberg, M. H. and Holladay, B. and Montoya, S. A. and Zheng, X. Y. and Lee, J. C. T. and Reid, A. H. and Koralek, J. D. and Shen, L. and Esposito, V. and Coslovich, G. and Walter, P. and Zohar, S. and Thampy, V. and Lin, M. F. and Hart, P. and Nakahara, K. and Streubel, R. and Kevan, S. D. and Fischer, P. and Colocho, W. and Lutman, A. and Decker, F. -J. and Fullerton, E. E. and Dunne, M. and Roy, S. and Sinha, S. K. and Turner, J. J.},
abstractNote = {Magnetic skyrmions are topological spin textures that exhibit classical or quantum quasi-particle behavior. A substantial amount of research has occurred in this field, both because of their unique electromagnetic properties and potential application for future nonvolatile memory storage applications, as well as fundamental questions on their topology and unique magnetic phases. Here, we investigate the fluctuation properties of a magnetic Fe/Gd skyrmion lattice, using short-pulsed xrays. We first measure spontaneous fluctuations of the skyrmion lattice phase and find an inherent, collective mode showing an underdamped oscillation with a relaxation of a couple of nanoseconds. Further observations track the response towards the continuous phase transition and a ‘critical-like’ slowing down of fluctuations is observed well before the critical point. These results suggest that the skyrmion lattice phase never fully freezes into a static crystal. This constant state of fluctuation indicates that the physics of topological magnetic phases may have more in common with high-temperature superconductors with disorder.},
doi = {10.1103/PhysRevResearch.3.033249},
journal = {Physical Review Research},
number = 3,
volume = 3,
place = {United States},
year = {Wed Sep 15 00:00:00 EDT 2021},
month = {Wed Sep 15 00:00:00 EDT 2021}
}

Works referenced in this record:

Probing complex materials with coherent soft X-rays
journal, May 2008


Linac Coherent Light Source soft x-ray materials science instrument optical design and monochromator commissioning
journal, September 2011

  • Heimann, Philip; Krupin, Oleg; Schlotter, William F.
  • Review of Scientific Instruments, Vol. 82, Issue 9
  • DOI: 10.1063/1.3633947

Observation of Magnetic Excitations of Skyrmion Crystal in a Helimagnetic Insulator Cu 2 OSeO 3
journal, July 2012


Linac Coherent Light Source: The first five years
journal, March 2016


Imprinting a Focused X-Ray Laser Beam to Measure Its Full Spatial Characteristics
journal, July 2015


The Soft X-ray Research instrument at the Linac Coherent Light Source
journal, April 2015

  • Dakovski, Georgi L.; Heimann, Philip; Holmes, Michael
  • Journal of Synchrotron Radiation, Vol. 22, Issue 3
  • DOI: 10.1107/S160057751500301X

Specific Heat of the Skyrmion Lattice Phase and Field-Induced Tricritical Point in MnSi
journal, April 2013


First lasing and operation of an ångstrom-wavelength free-electron laser
journal, August 2010


Skyrmion Lattice in a Chiral Magnet
journal, February 2009


Skyrmion fluctuations at a first-order phase transition boundary
journal, May 2020

  • Esposito, V.; Zheng, X. Y.; Seaberg, M. H.
  • Applied Physics Letters, Vol. 116, Issue 18
  • DOI: 10.1063/5.0004879

Spin waves in a skyrmion crystal
journal, December 2011


Topology-Dependent Brownian Gyromotion of a Single Skyrmion
journal, July 2020


Trochoidal motion and pair generation in skyrmion and antiskyrmion dynamics under spin–orbit torques
journal, August 2018


Comparing different approaches to characterization of focused X-ray laser beams
journal, March 2011

  • Chalupsky, J.; Bohacek, P.; Hajkova, V.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 631, Issue 1
  • DOI: 10.1016/j.nima.2010.12.040

Dynamics and inertia of skyrmionic spin structures
journal, February 2015

  • Büttner, Felix; Moutafis, C.; Schneider, M.
  • Nature Physics, Vol. 11, Issue 3
  • DOI: 10.1038/nphys3234

The soft x-ray instrument for materials studies at the linac coherent light source x-ray free-electron laser
journal, April 2012

  • Schlotter, W. F.; Turner, J. J.; Rowen, M.
  • Review of Scientific Instruments, Vol. 83, Issue 4
  • DOI: 10.1063/1.3698294

Magnetic Materials: Chiral Spin Textures in Amorphous Iron–Germanium Thick Films (Adv. Mater. 8/2021)
journal, February 2021

  • Streubel, Robert; Bouma, D. Simca; Bruni, Frank
  • Advanced Materials, Vol. 33, Issue 8
  • DOI: 10.1002/adma.202170061

Microwave magnetoelectric effect via skyrmion resonance modes in a helimagnetic multiferroic
journal, August 2013

  • Okamura, Y.; Kagawa, F.; Mochizuki, M.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3391

One-Dimensional Anomalous Diffusion of Gold Nanoparticles in a Polymer Melt
journal, March 2019


Spin-Wave Modes and Their Intense Excitation Effects in Skyrmion Crystals
journal, January 2012


Magnetic skyrmions: advances in physics and potential applications
journal, June 2017


Spin-orbit torque-driven skyrmion dynamics revealed by time-resolved X-ray microscopy
journal, May 2017

  • Woo, Seonghoon; Song, Kyung Mee; Han, Hee-Sung
  • Nature Communications, Vol. 8, Issue 1
  • DOI: 10.1038/ncomms15573

Dynamics of Skyrmion Crystals in Metallic Thin Films
journal, September 2011


Topological properties and dynamics of magnetic skyrmions
journal, December 2013


Pulse energy measurement at the SXR instrument
journal, April 2015

  • Moeller, Stefan; Brown, Garth; Dakovski, Georgi
  • Journal of Synchrotron Radiation, Vol. 22, Issue 3
  • DOI: 10.1107/S1600577515006098

Synthesizing skyrmion bound pairs in Fe-Gd thin films
journal, July 2016

  • Lee, J. C. T.; Chess, J. J.; Montoya, S. A.
  • Applied Physics Letters, Vol. 109, Issue 2
  • DOI: 10.1063/1.4955462

Scaling of domain cascades in stripe and skyrmion phases
journal, April 2019


Resonant properties of dipole skyrmions in amorphous Fe/Gd multilayers
journal, June 2017


A snapshot review—Fluctuations in quantum materials: from skyrmions to superconductivity
journal, April 2021


High Contrast X-ray Speckle from Atomic-Scale Order in Liquids and Glasses
journal, November 2012


An introduction to the Ginzburg–Landau theory of phase transitions and nonequilibrium patterns
journal, April 2015


Blowing magnetic skyrmion bubbles
journal, June 2015


Measuring temporal speckle correlations at ultrafast x-ray sources
journal, December 2008


Absolute pulse energy measurements of soft x-rays at the Linac Coherent Light Source
journal, January 2014

  • Tiedtke, K.; Sorokin, A. A.; Jastrow, U.
  • Optics Express, Vol. 22, Issue 18
  • DOI: 10.1364/OE.22.021214

Biskyrmion states and their current-driven motion in a layered manganite
journal, January 2014

  • Yu, X. Z.; Tokunaga, Y.; Kaneko, Y.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4198

Do Images of Biskyrmions Show Type‐II Bubbles?
journal, February 2019

  • Loudon, James C.; Twitchett‐Harrison, Alison C.; Cortés‐Ortuño, David
  • Advanced Materials, Vol. 31, Issue 16
  • DOI: 10.1002/adma.201806598

Tailoring magnetic energies to form dipole skyrmions and skyrmion lattices
journal, January 2017


Large-format, high-speed, X-ray pnCCDs combined with electron and ion imaging spectrometers in a multipurpose chamber for experiments at 4th generation light sources
journal, March 2010

  • Strüder, Lothar; Epp, Sascha; Rolles, Daniel
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 614, Issue 3
  • DOI: 10.1016/j.nima.2009.12.053