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Title: Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3

Abstract

Electric field control of topologically nontrivial magnetic textures, such as skyrmions, provides a paradigm shift for future spintronics beyond current silicon-based technology. While significant progress has been made by X-ray and neutron scattering studies, direct observation of such nanoscale spin structures and their dynamics driven by external electric fields remains a challenge to understand underlying mechanisms and harness functionalities. Here, using Lorentz transmission electron microscopy combined with in situ electric and magnetic fields at liquid helium temperatures, we report the crystallographic-orientation dependent skyrmion responses to electric fields in thin slabs of magnetoelectric Cu2OSeO3. We show electric fields not only stabilize the hexagonally packed skyrmion lattices in the entire sample in a hysteretic manner but also induce the rotation of their reciprocal vector discretely by 30°. Furthermore, the nonvolatile and energy-efficient skyrmion-lattice control by electric fields demonstrated in this work provides an important foundation for designing skyrmion-based qubits and memory devices.

Authors:
ORCiD logo [1];  [1];  [2];  [1];  [3]; ORCiD logo [3]; ORCiD logo [2];  [4]; ORCiD logo [2]; ORCiD logo [1]
  1. Brookhaven National Laboratory (BNL), Upton, NY (United States)
  2. University of New South Wales, Sydney (Australia)
  3. University of Auckland (New Zealand); The MacDiarmid Institute for Advanced Materials and Nanotechnology, Wellington (New Zealand)
  4. University of Groningen (The Netherlands)
Publication Date:
Research Org.:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)
OSTI Identifier:
2005142
Report Number(s):
BNL-224817-2023-JAAM
Journal ID: ISSN 1530-6984; TRN: US2405756
Grant/Contract Number:  
SC0012704
Resource Type:
Accepted Manuscript
Journal Name:
Nano Letters
Additional Journal Information:
Journal Volume: 23; Journal Issue: 15; Journal ID: ISSN 1530-6984
Publisher:
American Chemical Society
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; skyrmions; magnetoelectric coupling; electric field control of magnetism; topological spin structures; electric fields; lattices; magnetic properties; quantum mechanics; transmission electron microscopy

Citation Formats

Han, Myung-Geun, Camino, Fernando, Vorobyev, Pavel A., Garlow, Joseph, Rov, Rosanna, Söhnel, Tilo, Seidel, Jan, Mostovoy, Maxim, Tretiakov, Oleg A., and Zhu, Yimei. Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3. United States: N. p., 2023. Web. doi:10.1021/acs.nanolett.3c02034.
Han, Myung-Geun, Camino, Fernando, Vorobyev, Pavel A., Garlow, Joseph, Rov, Rosanna, Söhnel, Tilo, Seidel, Jan, Mostovoy, Maxim, Tretiakov, Oleg A., & Zhu, Yimei. Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3. United States. https://doi.org/10.1021/acs.nanolett.3c02034
Han, Myung-Geun, Camino, Fernando, Vorobyev, Pavel A., Garlow, Joseph, Rov, Rosanna, Söhnel, Tilo, Seidel, Jan, Mostovoy, Maxim, Tretiakov, Oleg A., and Zhu, Yimei. Mon . "Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3". United States. https://doi.org/10.1021/acs.nanolett.3c02034.
@article{osti_2005142,
title = {Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3},
author = {Han, Myung-Geun and Camino, Fernando and Vorobyev, Pavel A. and Garlow, Joseph and Rov, Rosanna and Söhnel, Tilo and Seidel, Jan and Mostovoy, Maxim and Tretiakov, Oleg A. and Zhu, Yimei},
abstractNote = {Electric field control of topologically nontrivial magnetic textures, such as skyrmions, provides a paradigm shift for future spintronics beyond current silicon-based technology. While significant progress has been made by X-ray and neutron scattering studies, direct observation of such nanoscale spin structures and their dynamics driven by external electric fields remains a challenge to understand underlying mechanisms and harness functionalities. Here, using Lorentz transmission electron microscopy combined with in situ electric and magnetic fields at liquid helium temperatures, we report the crystallographic-orientation dependent skyrmion responses to electric fields in thin slabs of magnetoelectric Cu2OSeO3. We show electric fields not only stabilize the hexagonally packed skyrmion lattices in the entire sample in a hysteretic manner but also induce the rotation of their reciprocal vector discretely by 30°. Furthermore, the nonvolatile and energy-efficient skyrmion-lattice control by electric fields demonstrated in this work provides an important foundation for designing skyrmion-based qubits and memory devices.},
doi = {10.1021/acs.nanolett.3c02034},
journal = {Nano Letters},
number = 15,
volume = 23,
place = {United States},
year = {Mon Jul 31 00:00:00 EDT 2023},
month = {Mon Jul 31 00:00:00 EDT 2023}
}

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