This content will become publicly available on Wed Jul 31 00:00:00 EDT 2024
Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3
Abstract
Electric field control of topologically nontrivial magnetic textures, such as skyrmions, provides a paradigm shift for future spintronics beyond current silicon-based technology. While significant progress has been made by X-ray and neutron scattering studies, direct observation of such nanoscale spin structures and their dynamics driven by external electric fields remains a challenge to understand underlying mechanisms and harness functionalities. Here, using Lorentz transmission electron microscopy combined with in situ electric and magnetic fields at liquid helium temperatures, we report the crystallographic-orientation dependent skyrmion responses to electric fields in thin slabs of magnetoelectric Cu2OSeO3. We show electric fields not only stabilize the hexagonally packed skyrmion lattices in the entire sample in a hysteretic manner but also induce the rotation of their reciprocal vector discretely by 30°. Furthermore, the nonvolatile and energy-efficient skyrmion-lattice control by electric fields demonstrated in this work provides an important foundation for designing skyrmion-based qubits and memory devices.
- Authors:
-
- Brookhaven National Laboratory (BNL), Upton, NY (United States)
- University of New South Wales, Sydney (Australia)
- University of Auckland (New Zealand); The MacDiarmid Institute for Advanced Materials and Nanotechnology, Wellington (New Zealand)
- University of Groningen (The Netherlands)
- Publication Date:
- Research Org.:
- Brookhaven National Laboratory (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)
- OSTI Identifier:
- 2005142
- Report Number(s):
- BNL-224817-2023-JAAM
Journal ID: ISSN 1530-6984; TRN: US2405756
- Grant/Contract Number:
- SC0012704
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nano Letters
- Additional Journal Information:
- Journal Volume: 23; Journal Issue: 15; Journal ID: ISSN 1530-6984
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; skyrmions; magnetoelectric coupling; electric field control of magnetism; topological spin structures; electric fields; lattices; magnetic properties; quantum mechanics; transmission electron microscopy
Citation Formats
Han, Myung-Geun, Camino, Fernando, Vorobyev, Pavel A., Garlow, Joseph, Rov, Rosanna, Söhnel, Tilo, Seidel, Jan, Mostovoy, Maxim, Tretiakov, Oleg A., and Zhu, Yimei. Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3. United States: N. p., 2023.
Web. doi:10.1021/acs.nanolett.3c02034.
Han, Myung-Geun, Camino, Fernando, Vorobyev, Pavel A., Garlow, Joseph, Rov, Rosanna, Söhnel, Tilo, Seidel, Jan, Mostovoy, Maxim, Tretiakov, Oleg A., & Zhu, Yimei. Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3. United States. https://doi.org/10.1021/acs.nanolett.3c02034
Han, Myung-Geun, Camino, Fernando, Vorobyev, Pavel A., Garlow, Joseph, Rov, Rosanna, Söhnel, Tilo, Seidel, Jan, Mostovoy, Maxim, Tretiakov, Oleg A., and Zhu, Yimei. Mon .
"Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3". United States. https://doi.org/10.1021/acs.nanolett.3c02034.
@article{osti_2005142,
title = {Hysteretic Responses of Skyrmion Lattices to Electric Fields in Magnetoelectric Cu2OSeO3},
author = {Han, Myung-Geun and Camino, Fernando and Vorobyev, Pavel A. and Garlow, Joseph and Rov, Rosanna and Söhnel, Tilo and Seidel, Jan and Mostovoy, Maxim and Tretiakov, Oleg A. and Zhu, Yimei},
abstractNote = {Electric field control of topologically nontrivial magnetic textures, such as skyrmions, provides a paradigm shift for future spintronics beyond current silicon-based technology. While significant progress has been made by X-ray and neutron scattering studies, direct observation of such nanoscale spin structures and their dynamics driven by external electric fields remains a challenge to understand underlying mechanisms and harness functionalities. Here, using Lorentz transmission electron microscopy combined with in situ electric and magnetic fields at liquid helium temperatures, we report the crystallographic-orientation dependent skyrmion responses to electric fields in thin slabs of magnetoelectric Cu2OSeO3. We show electric fields not only stabilize the hexagonally packed skyrmion lattices in the entire sample in a hysteretic manner but also induce the rotation of their reciprocal vector discretely by 30°. Furthermore, the nonvolatile and energy-efficient skyrmion-lattice control by electric fields demonstrated in this work provides an important foundation for designing skyrmion-based qubits and memory devices.},
doi = {10.1021/acs.nanolett.3c02034},
journal = {Nano Letters},
number = 15,
volume = 23,
place = {United States},
year = {Mon Jul 31 00:00:00 EDT 2023},
month = {Mon Jul 31 00:00:00 EDT 2023}
}
Works referenced in this record:
Electric field control of magnetism
journal, July 2021
- Ramesh, Ramamoorthy; Manipatruni, Sasikanth
- Proceedings of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 477, Issue 2251
Edge-mediated skyrmion chain and its collective dynamics in a confined geometry
journal, October 2015
- Du, Haifeng; Che, Renchao; Kong, Lingyao
- Nature Communications, Vol. 6, Issue 1
Magnetic Skyrmion Materials
journal, November 2020
- Tokura, Yoshinori; Kanazawa, Naoya
- Chemical Reviews, Vol. 121, Issue 5
In Situ Electric Field Skyrmion Creation in Magnetoelectric Cu 2 OSeO 3
journal, July 2018
- Huang, Ping; Cantoni, Marco; Kruchkov, Alex
- Nano Letters, Vol. 18, Issue 8
Large anisotropic deformation of skyrmions in strained crystal
journal, June 2015
- Shibata, K.; Iwasaki, J.; Kanazawa, N.
- Nature Nanotechnology, Vol. 10, Issue 7
Manipulation of Nanoscale Domain Switching Using an Electron Beam with Omnidirectional Electric Field Distribution
journal, July 2016
- Chen, Zibin; Wang, Xiaolin; Ringer, Simon P.
- Physical Review Letters, Vol. 117, Issue 2
Advances in magnetoelectric multiferroics
journal, February 2019
- Spaldin, N. A.; Ramesh, R.
- Nature Materials, Vol. 18, Issue 3
Manipulation of the Dzyaloshinskii–Moriya Interaction in Co/Pt Multilayers with Strain
journal, April 2020
- Gusev, N. S.; Sadovnikov, A. V.; Nikitov, S. A.
- Physical Review Letters, Vol. 124, Issue 15
Unwinding of a Skyrmion Lattice by Magnetic Monopoles
journal, May 2013
- Milde, P.; Kohler, D.; Seidel, J.
- Science, Vol. 340, Issue 6136
Directional electric-field induced transformation from skyrmion lattice to distinct helices in multiferroic
Cu 2 OSeO 3
journal, May 2017
- Okamura, Y.; Yamasaki, Y.; Morikawa, D.
- Physical Review B, Vol. 95, Issue 18
Observation of the Magnetic Skyrmion Lattice in a MnSi Nanowire by Lorentz TEM
journal, July 2013
- Yu, Xiuzhen; DeGrave, John P.; Hara, Yuka
- Nano Letters, Vol. 13, Issue 8
Magnetoelectric nature of skyrmions in a chiral magnetic insulator Cu OSeO
journal, August 2012
- Seki, S.; Ishiwata, S.; Tokura, Y.
- Physical Review B, Vol. 86, Issue 6
Manipulation of skyrmion motion by magnetic field gradients
journal, May 2018
- Zhang, S. L.; Wang, W. W.; Burn, D. M.
- Nature Communications, Vol. 9, Issue 1
Vital role of magnetocrystalline anisotropy in cubic chiral skyrmion hosts
journal, July 2021
- Preißinger, M.; Karube, K.; Ehlers, D.
- npj Quantum Materials, Vol. 6, Issue 1
Electric field control of the skyrmion lattice in Cu 2 OSeO 3
journal, October 2012
- White, J. S.; Levatić, I.; Omrani, A. A.
- Journal of Physics: Condensed Matter, Vol. 24, Issue 43
Electron-beam-induced ferroelectric domain behavior in the transmission electron microscope: Toward deterministic domain patterning
journal, November 2016
- Hart, James L.; Liu, Shi; Lang, Andrew C.
- Physical Review B, Vol. 94, Issue 17
Scaling, rotation, and channeling behavior of helical and skyrmion spin textures in thin films of Te-doped Cu 2 OSeO 3
journal, March 2020
- Han, M. -G.; Garlow, J. A.; Kharkov, Y.
- Science Advances, Vol. 6, Issue 13
Thermally driven ratchet motion of a skyrmion microcrystal and topological magnon Hall effect
journal, January 2014
- Mochizuki, M.; Yu, X. Z.; Seki, S.
- Nature Materials, Vol. 13, Issue 3
Magnetoelectric effects in the skyrmion host material Cu2OSeO3
journal, October 2015
- Ruff, E.; Lunkenheimer, P.; Loidl, A.
- Scientific Reports, Vol. 5, Issue 1
The 2020 skyrmionics roadmap
journal, June 2020
- Back, C.; Cros, V.; Ebert, H.
- Journal of Physics D: Applied Physics, Vol. 53, Issue 36
Multiferroics: a magnetic twist for ferroelectricity
journal, January 2007
- Cheong, Sang-Wook; Mostovoy, Maxim
- Nature Materials, Vol. 6, Issue 1
Topological properties and dynamics of magnetic skyrmions
journal, December 2013
- Nagaosa, Naoto; Tokura, Yoshinori
- Nature Nanotechnology, Vol. 8, Issue 12
Observation of Skyrmions in a Multiferroic Material
journal, April 2012
- Seki, S.; Yu, X. Z.; Ishiwata, S.
- Science, Vol. 336, Issue 6078
Zigzag domains caused by strain-induced anisotropy of the Dzyaloshinskii-Moriya interaction
journal, January 2022
- Sapozhnikov, M. V.; Gorev, R. V.; Skorokhodov, E. V.
- Physical Review B, Vol. 105, Issue 2
Strong Dzyaloshinskii-Moriya Interaction and Origin of Ferroelectricity in
journal, September 2012
- Yang, J. H.; Li, Z. L.; Lu, X. Z.
- Physical Review Letters, Vol. 109, Issue 10
Stabilization of magnetic skyrmions by uniaxial tensile strain
journal, December 2017
- Seki, S.; Okamura, Y.; Shibata, K.
- Physical Review B, Vol. 96, Issue 22
New magnetic phase of the chiral skyrmion material Cu 2 OSeO 3
journal, September 2018
- Qian, Fengjiao; Bannenberg, Lars J.; Wilhelm, Heribert
- Science Advances, Vol. 4, Issue 9
Skyrmion Qubits: A New Class of Quantum Logic Elements Based on Nanoscale Magnetization
journal, August 2021
- Psaroudaki, Christina; Panagopoulos, Christos
- Physical Review Letters, Vol. 127, Issue 6
Electric-Field-Induced Skyrmion Distortion and Giant Lattice Rotation in the Magnetoelectric Insulator
journal, September 2014
- White, J. S.; Prša, K.; Huang, P.
- Physical Review Letters, Vol. 113, Issue 10