Emergent behavior of LaNiO3 in short-periodic nickelate superlattices
Abstract
Heterostructure engineering provides an efficient way to obtain several emergent phases of LaNiO3, as demonstrated in recent works. In this work, a new class of short periodic superlattices, consisting of LaNiO3 and EuNiO3 have been grown by pulsed laser interval deposition to investigate the effect of structural symmetry mismatch on the electronic and magnetic behaviors. Using synchrotron based soft and hard x-ray resonant scattering experiments, we have found that these heterostructures undergo simultaneous electronic and magnetic transitions. Most importantly, LaNiO3 within these artificial structures exhibits a new antiferromagnetic, charge ordered insulating phase, which may be a potential candidate to achieve high temperature superconductivity.
- Authors:
-
- Indian Inst. of Science, Bengaluru (India)
- Oklahoma State Univ., Stillwater, OK (United States)
- Rutgers Univ., Piscataway, NJ (United States)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
- Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; Gordon and Betty Moore Foundation (GBMF); DST Nano Mission, India; Infosys Foundation, Bangalore
- OSTI Identifier:
- 1775375
- Alternate Identifier(s):
- OSTI ID: 1616034
- Grant/Contract Number:
- AC02-06CH11357; AC02-05CH11231; DST/NM/NS/2018/246; ECR/2018/001512; GBMF4534.
- Resource Type:
- Accepted Manuscript
- Journal Name:
- APL Materials
- Additional Journal Information:
- Journal Volume: 8; Journal Issue: 4; Journal ID: ISSN 2166-532X
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; nickelate; charge order; magnetism; superlattice; thin film
Citation Formats
Patel, Ranjan Kumar, Meyers, D., Liu, Xiaoran, Mandal, Prithwijit, Kareev, M., Shafer, P., Kim, J. -W., Ryan, P. J., Middey, S., and Chakhalian, J. Emergent behavior of LaNiO3 in short-periodic nickelate superlattices. United States: N. p., 2020.
Web. doi:10.1063/5.0004530.
Patel, Ranjan Kumar, Meyers, D., Liu, Xiaoran, Mandal, Prithwijit, Kareev, M., Shafer, P., Kim, J. -W., Ryan, P. J., Middey, S., & Chakhalian, J. Emergent behavior of LaNiO3 in short-periodic nickelate superlattices. United States. https://doi.org/10.1063/5.0004530
Patel, Ranjan Kumar, Meyers, D., Liu, Xiaoran, Mandal, Prithwijit, Kareev, M., Shafer, P., Kim, J. -W., Ryan, P. J., Middey, S., and Chakhalian, J. Fri .
"Emergent behavior of LaNiO3 in short-periodic nickelate superlattices". United States. https://doi.org/10.1063/5.0004530. https://www.osti.gov/servlets/purl/1775375.
@article{osti_1775375,
title = {Emergent behavior of LaNiO3 in short-periodic nickelate superlattices},
author = {Patel, Ranjan Kumar and Meyers, D. and Liu, Xiaoran and Mandal, Prithwijit and Kareev, M. and Shafer, P. and Kim, J. -W. and Ryan, P. J. and Middey, S. and Chakhalian, J.},
abstractNote = {Heterostructure engineering provides an efficient way to obtain several emergent phases of LaNiO3, as demonstrated in recent works. In this work, a new class of short periodic superlattices, consisting of LaNiO3 and EuNiO3 have been grown by pulsed laser interval deposition to investigate the effect of structural symmetry mismatch on the electronic and magnetic behaviors. Using synchrotron based soft and hard x-ray resonant scattering experiments, we have found that these heterostructures undergo simultaneous electronic and magnetic transitions. Most importantly, LaNiO3 within these artificial structures exhibits a new antiferromagnetic, charge ordered insulating phase, which may be a potential candidate to achieve high temperature superconductivity.},
doi = {10.1063/5.0004530},
journal = {APL Materials},
number = 4,
volume = 8,
place = {United States},
year = {Fri Apr 17 00:00:00 EDT 2020},
month = {Fri Apr 17 00:00:00 EDT 2020}
}
Web of Science
Works referenced in this record:
Dimensionality Control of Electronic Phase Transitions in Nickel-Oxide Superlattices
journal, May 2011
- Boris, A. V.; Matiks, Y.; Benckiser, E.
- Science, Vol. 332, Issue 6032
Phase engineering of rare earth nickelates by digital synthesis
journal, August 2018
- Middey, S.; Meyers, D.; Kumar Patel, Ranjan
- Applied Physics Letters, Vol. 113, Issue 8
Pure electronic metal-insulator transition at the interface of complex oxides
journal, June 2016
- Meyers, D.; Liu, Jian; Freeland, J. W.
- Scientific Reports, Vol. 6, Issue 1
Physics of Ultrathin Films and Heterostructures of Rare-Earth Nickelates
journal, July 2016
- Middey, S.; Chakhalian, J.; Mahadevan, P.
- Annual Review of Materials Research, Vol. 46, Issue 1
Structural, magnetic and electronic properties of perovskites (R = rare earth)
journal, February 1997
- Medarde, María Luisa
- Journal of Physics: Condensed Matter, Vol. 9, Issue 8
Heterointerface engineered electronic and magnetic phases of NdNiO3 thin films
journal, November 2013
- Liu, Jian; Kargarian, Mehdi; Kareev, Mikhail
- Nature Communications, Vol. 4, Issue 1
Engineered Mott ground state in a LaTiO3+δ/LaNiO3 heterostructure
journal, January 2016
- Cao, Yanwei; Liu, Xiaoran; Kareev, M.
- Nature Communications, Vol. 7, Issue 1
Dependence of negative differential resistance on electronic phase separation in unpatterned manganite films
journal, February 2012
- Ding, J. F.; Jin, K. X.; Zhang, Z.
- Applied Physics Letters, Vol. 100, Issue 6
Metal-Insulator Transition in Ultrathin Films
journal, June 2011
- Scherwitzl, R.; Gariglio, S.; Gabay, M.
- Physical Review Letters, Vol. 106, Issue 24
Atomic-scale control of competing electronic phases in ultrathin LaNiO3
journal, April 2014
- King, P. D. C.; Wei, H. I.; Nie, Y. F.
- Nature Nanotechnology, Vol. 9, Issue 6
Tuning bad metal and non-Fermi liquid behavior in a Mott material: Rare-earth nickelate thin films
journal, November 2015
- Mikheev, Evgeny; Hauser, Adam J.; Himmetoglu, Burak
- Science Advances, Vol. 1, Issue 10
Evolution of electronic structure across the rare-earth RNiO3 series
journal, April 2016
- Freeland, John W.; van Veenendaal, Michel; Chakhalian, Jak
- Journal of Electron Spectroscopy and Related Phenomena, Vol. 208
Charge Disproportionation in Perovskites: Simultaneous Metal-Insulator and Structural Transition in
journal, May 1999
- Alonso, J. A.; García-Muñoz, J. L.; Fernández-Díaz, M. T.
- Physical Review Letters, Vol. 82, Issue 19
Unconventional ferromagnetism in epitaxial (111)
journal, September 2018
- Asaba, Tomoya; Xiang, Ziji; Kim, T. H.
- Physical Review B, Vol. 98, Issue 12
Electronic transitions in strained SmNiO 3 thin films
journal, November 2014
- Catalano, S.; Gibert, M.; Bisogni, V.
- APL Materials, Vol. 2, Issue 11
Orbital control in strained ultra-thin LaNiO 3 /LaAlO 3 superlattices
journal, November 2011
- Freeland, J. W.; Liu, Jian; Kareev, M.
- EPL (Europhysics Letters), Vol. 96, Issue 5
Anisotropic Imprint of Amorphization and Phase Separation in Manganite Thin Films via Laser Interference Irradiation
journal, September 2014
- Ding, Junfeng; Lin, Zhipeng; Wu, Jianchun
- Small, Vol. 11, Issue 5
Direct Mapping of Phase Separation across the Metal–Insulator Transition of NdNiO 3
journal, March 2018
- Preziosi, Daniele; Lopez-Mir, Laura; Li, Xiaoyan
- Nano Letters, Vol. 18, Issue 4
Mott Transition and Magnetism in Rare Earth Nickelates and its Fingerprint on the X-ray Scattering
journal, September 2017
- Haule, Kristjan; Pascut, Gheorghe L.
- Scientific Reports, Vol. 7, Issue 1
Rare-earth nickelates R NiO 3 : thin films and heterostructures
journal, February 2018
- Catalano, S.; Gibert, M.; Fowlie, J.
- Reports on Progress in Physics, Vol. 81, Issue 4
Progress in perovskite nickelate research
journal, July 2008
- Catalan, G.
- Phase Transitions, Vol. 81, Issue 7-8
Strain-Enhanced Charge Transfer and Magnetism at a Manganite/Nickelate Interface
journal, August 2018
- Xu, Zedong; Hu, Songbai; Wu, Rui
- ACS Applied Materials & Interfaces, Vol. 10, Issue 36
Superconductivity in an infinite-layer nickelate
journal, August 2019
- Li, Danfeng; Lee, Kyuho; Wang, Bai Yang
- Nature, Vol. 572, Issue 7771
Quantum confinement of Mott electrons in ultrathin LaNiO /LaAlO superlattices
journal, April 2011
- Liu, Jian; Okamoto, S.; van Veenendaal, M.
- Physical Review B, Vol. 83, Issue 16
Complex magnetic order in nickelate slabs
journal, July 2018
- Hepting, M.; Green, R. J.; Zhong, Z.
- Nature Physics, Vol. 14, Issue 11