DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Uncertainty quantification for optical model parameters

Abstract

Background: Although uncertainty quantification has been making its way into nuclear theory, these methods have yet to be explored in the context of reaction theory. For example, it is well known that different parameterizations of the optical potential can result in different cross sections, but these differences have not been systematically studied and quantified. Purpose: The purpose of this work is to investigate the uncertainties in nuclear reactions that result from fitting a given model to elastic-scattering data, as well as to study how these uncertainties propagate to the inelastic and transfer channels. Method: We use statistical methods to determine a best fit and create corresponding 95% confidence bands. A simple model of the process is fit to elastic-scattering data and used to predict either inelastic or transfer cross sections. In this initial work, we assume that our model is correct, and the only uncertainties come from the variation of the fit parameters. Results: We study a number of reactions involving neutron and deuteron projectiles with energies in the range of 5-25 MeV/u, on targets with mass A = 12-208. We investigate the correlations between the parameters in the fit. The case of deuterons on C-12 is discussed in detail:more » the elastic-scattering fit and the prediction of C-12(d, p) C-13 transfer angular distributions, using both uncorrelated and correlated. 2 minimization functions. The general features for all cases are compiled in a systematic manner to identify trends. Conclusions: Our work shows that, in many cases, the correlated chi(2) functions (in comparison to the uncorrelated chi(2) functions) provide a more natural parameterization of the process. These correlated functions do, however, produce broader confidence bands. Further optimization may require improvement in the models themselves and/or more information included in the fit.« less

Authors:
 [1];  [1];  [2];  [2]
  1. Michigan State Univ., East Lansing, MI (United States). National Superconducting Cyclotron Lab. Dept. of Physics and Astronomy
  2. Argonne National Lab. (ANL), Argonne, IL (United States). Mathematics and Computer Science Division
Publication Date:
Research Org.:
Argonne National Laboratory (ANL), Argonne, IL (United States); Michigan State Univ., East Lansing, MI (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA), Office of Defense Programs (DP); USDOE Office of Science (SC), Advanced Scientific Computing Research (ASCR); National Science Foundation (NSF)
OSTI Identifier:
1357088
Alternate Identifier(s):
OSTI ID: 1344597; OSTI ID: 1368560
Grant/Contract Number:  
NA0002135; FG52-08NA28552; AC02-06CH11357; PHY-1403906; PHY-1520929
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review C
Additional Journal Information:
Journal Volume: 95; Journal Issue: 2; Journal ID: ISSN 2469-9985
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS; uncertainty quantification; elastic scattering; inelastic scattering; transfer reactions; direct reaction theory

Citation Formats

Lovell, A. E., Nunes, F. M., Sarich, J., and Wild, S. M. Uncertainty quantification for optical model parameters. United States: N. p., 2017. Web. doi:10.1103/PhysRevC.95.024611.
Lovell, A. E., Nunes, F. M., Sarich, J., & Wild, S. M. Uncertainty quantification for optical model parameters. United States. https://doi.org/10.1103/PhysRevC.95.024611
Lovell, A. E., Nunes, F. M., Sarich, J., and Wild, S. M. Tue . "Uncertainty quantification for optical model parameters". United States. https://doi.org/10.1103/PhysRevC.95.024611. https://www.osti.gov/servlets/purl/1357088.
@article{osti_1357088,
title = {Uncertainty quantification for optical model parameters},
author = {Lovell, A. E. and Nunes, F. M. and Sarich, J. and Wild, S. M.},
abstractNote = {Background: Although uncertainty quantification has been making its way into nuclear theory, these methods have yet to be explored in the context of reaction theory. For example, it is well known that different parameterizations of the optical potential can result in different cross sections, but these differences have not been systematically studied and quantified. Purpose: The purpose of this work is to investigate the uncertainties in nuclear reactions that result from fitting a given model to elastic-scattering data, as well as to study how these uncertainties propagate to the inelastic and transfer channels. Method: We use statistical methods to determine a best fit and create corresponding 95% confidence bands. A simple model of the process is fit to elastic-scattering data and used to predict either inelastic or transfer cross sections. In this initial work, we assume that our model is correct, and the only uncertainties come from the variation of the fit parameters. Results: We study a number of reactions involving neutron and deuteron projectiles with energies in the range of 5-25 MeV/u, on targets with mass A = 12-208. We investigate the correlations between the parameters in the fit. The case of deuterons on C-12 is discussed in detail: the elastic-scattering fit and the prediction of C-12(d, p) C-13 transfer angular distributions, using both uncorrelated and correlated. 2 minimization functions. The general features for all cases are compiled in a systematic manner to identify trends. Conclusions: Our work shows that, in many cases, the correlated chi(2) functions (in comparison to the uncorrelated chi(2) functions) provide a more natural parameterization of the process. These correlated functions do, however, produce broader confidence bands. Further optimization may require improvement in the models themselves and/or more information included in the fit.},
doi = {10.1103/PhysRevC.95.024611},
journal = {Physical Review C},
number = 2,
volume = 95,
place = {United States},
year = {Tue Feb 21 00:00:00 EST 2017},
month = {Tue Feb 21 00:00:00 EST 2017}
}

Journal Article:

Citation Metrics:
Cited by: 25 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Uncertainty quantification and propagation in nuclear density functional theory
journal, December 2015


The calculation of neutron cross-sections from optical potentials
journal, June 1964


Error analysis in nuclear density functional theory
journal, February 2015

  • Schunck, Nicolas; McDonnell, Jordan D.; Sarich, Jason
  • Journal of Physics G: Nuclear and Particle Physics, Vol. 42, Issue 3
  • DOI: 10.1088/0954-3899/42/3/034024

Elastic scattering of 9–13 MeV vector polarized deuterons
journal, November 1974


Neutron scattering from 12 C between 15.6 and 17.3 MeV
journal, June 1993

  • Chen, Z. M.; Baird, K.; Howell, C. R.
  • Journal of Physics G: Nuclear and Particle Physics, Vol. 19, Issue 6
  • DOI: 10.1088/0954-3899/19/6/008

Erratum to “Bayesian methods for parameter estimation in effective field theories” [Ann. Phys. 324 (2009) 682–708]
journal, September 2009


Vector analysing power and cross section for 90Zr(, p)91Zr at 11 and 12 MeV
journal, May 1973


Nucleon-Nucleus Optical-Model Parameters, A > 40 , E < 50 MeV
journal, June 1969


Local phenomenological nucleon-nucleon potentials
journal, December 1968


Adiabatic approximation versus exact Faddeev method for ( d , p ) and ( p , d ) reactions
journal, September 2011


Bayesian Monte Carlo Method for Nuclear Data Evaluation
journal, January 2015


Collective doorway configurations in Ca 49 through neutron scattering on Ca 48
journal, June 1990


Scattering and pick-up reactions with deuterons on Be, B, C, N and O at 11.8 MeV
journal, September 1967


Energy dependence of the deformed optical potential for neutron scattering from 54 , 56 Fe and 58 , 60 Ni up to 80 MeV
journal, November 1988


Comparing nonperturbative models of the breakup of neutron-halo nuclei
journal, April 2012


Bayesian parameter estimation for effective field theories
journal, May 2016

  • Wesolowski, S.; Klco, N.; Furnstahl, R. J.
  • Journal of Physics G: Nuclear and Particle Physics, Vol. 43, Issue 7
  • DOI: 10.1088/0954-3899/43/7/074001

Uncertainty quantification of effective nuclear interactions
journal, May 2016

  • Pérez, R. Navarro; Amaro, J. E.; Arriola, E. Ruiz
  • International Journal of Modern Physics E, Vol. 25, Issue 05
  • DOI: 10.1142/S0218301316410093

Deuteron global optical model potential for energies up to 200 MeV
journal, October 2006


Three-body description of direct nuclear reactions: Comparison with the continuum discretized coupled channels method
journal, December 2007


Improved description of Ar 34 , 36 , 46 ( p , d ) transfer reactions
journal, March 2011


Applying Bayesian parameter estimation to relativistic heavy-ion collisions: Simultaneous characterization of the initial state and quark-gluon plasma medium
journal, August 2016


Study of the ( d ,   p ) Reaction in the 1 p Shell
journal, December 1967


Systematic uncertainties in direct reaction theories
journal, February 2015


Are coupled channel effects important for the asymptotic normalization coefficient method?
journal, November 2001


Statistics of Measuring Neutron star Radii: Assessing a Frequentist and a Bayesian Approach
journal, September 2015


Excitation of low-lying collective states in Ca 40 and Pb 208 by inelastic neutron scattering
journal, October 1977


Coupling and higher-order effects in the C 12 ( d , p ) C 13 and C 13 ( p , d ) C 12 reactions
journal, July 2005


Analysis of a low-energy correction to the eikonal approximation
journal, September 2014


Effective field theory for nuclear vibrations with quantified uncertainties
journal, December 2015


Uncertainty Analysis and Order-by-Order Optimization of Chiral Nuclear Interactions
journal, February 2016


Quantifying truncation errors in effective field theory
journal, August 2015


Role of core excitation in ( d , p ) transfer reactions
journal, October 2016


Uncertainty Quantification for Nuclear Density Functional Theory and Information Content of New Measurements
journal, March 2015


Neutron scattering from 208Pb
journal, February 1978


Calculation and Evaluation of Cross Sections and Kerma Factors for Neutrons up to 100 MeV on Carbon
journal, May 1996

  • Chadwick, M. B.; Cox, L. J.; Young, P. G.
  • Nuclear Science and Engineering, Vol. 123, Issue 1
  • DOI: 10.13182/NSE96-A24210