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Title: Photon energy conversion by near-zero permittivity nonlinear materials

Abstract

Efficient harmonic light generation can be achieved with ultrathin films by coupling an incident pump wave to an epsilon-near-zero (ENZ) mode of the thin film. As an example, efficient third harmonic generation from an indium tin oxide nanofilm (.lamda./42 thick) on a glass substrate for a pump wavelength of 1.4 .mu.m was demonstrated. A conversion efficiency of 3.3.times.10.sup.-6 was achieved by exploiting the field enhancement properties of the ENZ mode with an enhancement factor of 200. This nanoscale frequency conversion method is applicable to other plasmonic materials and reststrahlen materials in proximity of the longitudinal optical phonon frequencies.

Inventors:
; ;
Issue Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1414408
Patent Number(s):
9846348
Application Number:
15/040,799
Assignee:
National Technology & Engineering Solutions of Sandia, LLC (Albuquerque, NM)
Patent Classifications (CPCs):
B - PERFORMING OPERATIONS B82 - NANOTECHNOLOGY B82Y - SPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES
G - PHYSICS G02 - OPTICS G02F - DEVICES OR ARRANGEMENTS, THE OPTICAL OPERATION OF WHICH IS MODIFIED BY CHANGING THE OPTICAL PROPERTIES OF THE MEDIUM OF THE DEVICES OR ARRANGEMENTS FOR THE CONTROL OF THE INTENSITY, COLOUR, PHASE, POLARISATION OR DIRECTION OF LIGHT, e.g. SWITCHING, GATING, MODULATING OR DEMODULATING
DOE Contract Number:  
AC04-94AL85000
Resource Type:
Patent
Resource Relation:
Patent File Date: 2016 Feb 10
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 30 DIRECT ENERGY CONVERSION

Citation Formats

Luk, Ting S., Sinclair, Michael B., and Campione, Salvatore. Photon energy conversion by near-zero permittivity nonlinear materials. United States: N. p., 2017. Web.
Luk, Ting S., Sinclair, Michael B., & Campione, Salvatore. Photon energy conversion by near-zero permittivity nonlinear materials. United States.
Luk, Ting S., Sinclair, Michael B., and Campione, Salvatore. Tue . "Photon energy conversion by near-zero permittivity nonlinear materials". United States. https://www.osti.gov/servlets/purl/1414408.
@article{osti_1414408,
title = {Photon energy conversion by near-zero permittivity nonlinear materials},
author = {Luk, Ting S. and Sinclair, Michael B. and Campione, Salvatore},
abstractNote = {Efficient harmonic light generation can be achieved with ultrathin films by coupling an incident pump wave to an epsilon-near-zero (ENZ) mode of the thin film. As an example, efficient third harmonic generation from an indium tin oxide nanofilm (.lamda./42 thick) on a glass substrate for a pump wavelength of 1.4 .mu.m was demonstrated. A conversion efficiency of 3.3.times.10.sup.-6 was achieved by exploiting the field enhancement properties of the ENZ mode with an enhancement factor of 200. This nanoscale frequency conversion method is applicable to other plasmonic materials and reststrahlen materials in proximity of the longitudinal optical phonon frequencies.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = {Tue Dec 19 00:00:00 EST 2017},
month = {Tue Dec 19 00:00:00 EST 2017}
}

Works referenced in this record:

Surface plasmon polariton band gap structures
patent-application, February 2002


Apparatus and Methods for Generating Electromagnetic Radiation
patent-application, August 2016


Berreman mode and epsilon near zero mode
journal, January 2012


Directional perfect absorption using deep subwavelength low-permittivity films
journal, August 2014


Enhanced third harmonic generation from the epsilon-near-zero modes of ultrathin films
journal, April 2015