Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Electron Paramagnetic Resonance Study of Pr

Journal Article · · Journal of Solid State Chemistry

Electron paramagnetic resonance (EPR) spectra of tetravalent praseodymium ions doped in the cubic perovskite compound BaHfO{sub 3} have been measured at 4.2 K. A very large hyperfine interaction with the {sup 141}Pr nucleus was observed in the spectrum of Pr{sup 4+}/ BaHfO{sub 3}. The results were analyzed based on the weak field approximation, and the g value (|g|=0.619) and a hyperfine coupling constant (A=0.0589 cm{sup {minus}1}) were obtained. The measured g value is much smaller than |-10/7|, which indicates that the crystal field effect on the behavior of a 4f electron is large. These g and A values were compared with the EPR results for other f{sup 1} ions in an octahedral crystal field.

Research Organization:
Division of Chemistry, Graduate School of Science, Hokkaido University, Sapporo (JP)
Sponsoring Organization:
Ministry of Education, Science, Sports, and Culture of Japan (MONBUSHO) (US)
OSTI ID:
784347
Journal Information:
Journal of Solid State Chemistry, Journal Name: Journal of Solid State Chemistry Journal Issue: 1 Vol. 156; ISSN 0022-4596
Country of Publication:
United States
Language:
English

Similar Records

Electron paramagnetic resonance spectra of Pr{sup 4+} in BaCeO{sub 3}, BaZrO{sub 3}, BaSnO{sub 3}, and their solid solutions
Journal Article · Thu Feb 29 23:00:00 EST 1996 · Journal of Solid State Chemistry · OSTI ID:269890

Electron paramagnetic resonance spectra of Pr{sup 4+} ions doped in Sr{sub 2}SnO{sub 4} and Ba{sub 2}SnO{sub 4}
Journal Article · Thu May 01 00:00:00 EDT 1997 · Journal of Solid State Chemistry · OSTI ID:577476

Electron paramagnetic resonance spectrum of Pr{sup 4+} in BaCeO{sub 3}
Journal Article · Thu Sep 01 00:00:00 EDT 1994 · Journal of Solid State Chemistry · OSTI ID:518199