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Evaluation of Th series disequilibrium in Western Australian monazite

Journal Article · · Health Physics; (USA)
;  [1]
  1. Curtin Univ. of Technology, Perth (Western Australia)
Estimation of inhaled radiation doses associated with mineral sands processing is commonly performed by gross alpha-counting dust collected on air filters. The technique requires knowledge of the extent of disequilibrium in Th-bearing minerals. The daughters which can be expected to give rise to disequilibrium, viz. {sup 228}Ra and {sup 220}Rn (designated thoron), were investigated in a typical Western Australia monazite. The thoron flux from a dry, infinitely thick layer of monazite was found to be 41 Bq m-2 s-1. The depth of monazite from which thoron is exhaled is limited to 40-50 mm, and within the first 10 mm is a linear function of bed thickness. The relative loss within the linear region is approximately 0.02% of the equilibrium concentration and progressively less for layers beyond 10 mm. The sample investigated gave no indication of disequilibrium involving {sup 228}Ra. The results indicate that secular equilibrium may be assumed when calculating {sup 232}Th daughter concentrations in monazite from the gross alpha activity. More extensive work on monazite samples from a number of sites will be necessary before this can be stated as a general conclusion applicable to all Western Australian monazite deposits.
OSTI ID:
6996364
Journal Information:
Health Physics; (USA), Journal Name: Health Physics; (USA) Vol. 58:2; ISSN 0017-9078; ISSN HLTPA
Country of Publication:
United States
Language:
English