Simulation of muonium formation in liquid hydrocarbons

Journal Article · Fri Oct 01 04:00:00 EDT 1999 · Journal of Chemical Physics

DOI:https://doi.org/10.1063/1.480074· OSTI ID:698896

Siebbeles, L D ^[1]; Pimblott, S M ^[2]; Cox, S F ^[3]

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1. IRI, Delft University of Technology, Mekelweg 15, 2629 JB Delft (The Netherlands)
2. Radiation Laboratory, University of Notre Dame, Indiana 46556-0579 (United States)
3. ISIS Facility, Rutherford Appleton Lab, Chilton, Oxfordshire, OX11 0QX (United Kingdom)

Muonium formation in liquid hexane is examined by computer simulation. In track-end competition between muonium formation and cation{endash}electron recombination, the muon is found to react with electrons from a significant part of the track end, corresponding to an energy attenuation of several tens of keV and a length of several microns. This muonium formation extends to microseconds following muon implantation. Delayed muonium formation leads to a much smaller amplitude of the muonium asymmetry than for prompt muonium formation during slowing down of the muon, and in this way may account for the missing polarization in transverse magnetic field experiments. If reaction of muons with electrons from their radiolysis tracks contributes to the experimentally observed muonium yield, the muon must thermalize between 60 and 150 nm from the last ionization of the track to reproduce the amplitudes of the muon and muonium asymmetries. For the smallest distance, 60 nm, the experimentally observed muonium asymmetry results from delayed muonium only. As the muon thermalization distance increases, prompt muonium formation also contributes, so that at 150 nm the observed asymmetry is almost entirely due to prompt muonium formation. {copyright} {ital 1999 American Institute of Physics.}

• OSTI ID: 698896
• Journal Information: Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 16 Vol. 111; ISSN JCPSA6; ISSN 0021-9606
• Country of Publication: United States
• Language: English

Related Subjects

66 PHYSICS
COMPUTERIZED SIMULATION
CYCLOHEXANE
HEXANE
HYDROCARBONS
LIQUIDS
MUONIUM
MUONS
ORGANIC COMPOUNDS
RADIOLYSIS
THERMALIZATION