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Muonium atoms and intraspur processes in water

Journal Article · · J. Chem. Phys.; (United States)
DOI:https://doi.org/10.1063/1.437275· OSTI ID:6079721
Since muonium atoms come into existence as a result of stopping energetic positive muons, it has been suggested that intraspur reactions (primarily with thermalized electrons or OH radicals, in water) are responsible for: (i) muonium formation, (ii) direct generation of a fraction of the muons in diamagnetic molecules, and (iii) the ''missing'' muon polarization. These postulates are examined in detail by adding scavengers which can preclude intraspur reactions without reacting with muonium. The results show convincingly that intraspur processes are insignificant in (i) and (ii). Furthermore, they could only be important in (iii) if a spin-exchange process occurred with a frequency which was much greater than the ordinary diffusion-limited encounter frequency. Rather than this ''spur model'', the data obtained are consistent with the ''hot model'', whereby hot muonium atoms form beyond the spurs of the muon track.
Research Organization:
TRIUMF and Department of Chemistry, University of British Columbia, Vancouver, British Columbia V6T 1WS, Canada
OSTI ID:
6079721
Journal Information:
J. Chem. Phys.; (United States), Journal Name: J. Chem. Phys.; (United States) Vol. 70:10; ISSN JCPSA
Country of Publication:
United States
Language:
English

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