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Possible viscosity effects in neutron-induced fission of /sup 232/Th and /sup 238/U. [Yields]

Conference ·
OSTI ID:6247473
Fission yields induced in the /sup 238/U(n,f) and /sup 232/Th(n,f) reactions were determined as a function of incident neutron energy (E/sub n/). The ratio of /sup 115/Cd-to-/sup 140/Ba yields as a function of E/sub n/ is analyzed by means of the equation Y/sub 1//Y/sub 2/ = exp(2(a/sub 1/(E/sub n/+E/sub 1/)/sup 1/2/ -2(a/sub 2/(E/sub n/+E/sub 2/)/sup 1/2/) to give values of a/sub i/, the level density parameter, and E/sub i/, the excitation energy for E/sub n/=0. The energies E/sub i/ are interpreted on the basis of the liquid drop model with shell and pairing corrections. Values are deduced for the energy dissipated by viscosity effects in the descent from the saddle point to the point where masses are fixed in the fissioning nucleus. These values are 1.7 MeV for /sup 232/Th(n,f) and 4.8 MeV for /sup 238/U(n,f). These values are consistent with the experimental observation that anti ..nu../sub p/ is approx. 0.6 neutron greater for /sup 239/U fission than for /sup 233/Th fission and that strong odd--even (nucleon pairing) effects are found in the fragment total kinetic energy distribution for /sup 230/Th fission but not for /sup 234/U fission. The low dissipation energy values together with the low values of pre-scission kinetic energy deduced by Guet, et al., (Nucl. Phys. A134 (1971)1) indicate a shorter path from the saddle point of the fissioning nucleus to scission than is generally assumed in theoretical calculations. 31 references.
Research Organization:
Argonne National Lab., IL (USA)
DOE Contract Number:
W-31109-ENG-38
OSTI ID:
6247473
Report Number(s):
CONF-790507-7
Country of Publication:
United States
Language:
English

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