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U.S. Department of Energy
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A study of some wastewater contaminants

Technical Report ·
OSTI ID:6203140

Coal conversion processes (liquefaction and gasification) always generate process wastewaters containing relatively high concentrations of toxic phenolic organic compounds, ammonia, cyanide, hydrogen sulfide, as well as, certain toxic heavy metals. Studies in our laboratory show that these metal ions react with the phenolic compounds to form complex ions and coordination compounds. The interaction of iron(III), copper(II), zinc(II), cobalt(II) dichromate ion, and dioxouranium(VI) ion with our model reagent 2-hydroxymethyl- 6(2{prime}-hydrozymethyl-5{prime}- hydrozy-4{prime} pyrone-6{prime}) pyranyl(3,2-b) pyran-4,8-dione has been studied. The formation constants and coordination numbers for most of these ions have been determined using the polarography. Polarographic studies carried out on Zn{sup +2}, Co{sup +2}, and Cr{sub 2}O{sub 7}{sup =} under the conditions used in this study were not completely reproducible. These studies, in aqueous media, suggest that there is a substantial and material need to study the extent of transport of metal complexes across the aqueous organic interface in the liquid-liquid extraction of coal-conversion process wastewaters.

Research Organization:
Texas Southern Univ., Houston, TX (USA). Dept. of Chemistry
Sponsoring Organization:
DOE/FE
DOE Contract Number:
FG22-85PC80541
OSTI ID:
6203140
Report Number(s):
DOE/PC/80541-T13; ON: DE89004334
Country of Publication:
United States
Language:
English

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