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Resonant nuclear Bragg diffraction from epitaxial sup 57 Fe sub 2 O sub 3 on natural Fe sub 2 O sub 3

Journal Article · · Journal of Applied Physics; (United States)
DOI:https://doi.org/10.1063/1.349705· OSTI ID:6188799
;  [1]
  1. Solid State Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee (USA)
We have used a {sup 57}Co Moessbauer source to measure the resonant nuclear scattering properties of epitaxial {sup 57}Fe{sub 2}O{sub 3} grown on natural Fe{sub 2}O{sub 3} substrates. Isotopically enriched {sup 57}Fe{sub 2}O{sub 3} layers were grown on {l angle}111{r angle} oriented Fe{sub 2}O{sub 3} by chemical vapor transport; Mo {ital K}{alpha} rocking curve measurements showed the mosaic spread of the epitaxial layers to be {similar to}15 arcs. The resonant nuclear scattering properties were characterized by absolute integrated intensity measurements of the (electronic and nuclear resonant) 666 reflection and the (pure nuclear resonant) 777 reflection as a function of energy near the resonance. The energy widths of the diffracted intensities were found to be {similar to}40 neV ({similar to}10{Gamma}) and the integrated intensities were found to lie between the values calculated from kinematic and dynamic diffraction theories. The results indicate that epitaxial crystals such as these can be used for resonant nuclear monochromators to obtain resonant x-ray beams from synchrotron sources.
DOE Contract Number:
AC05-84OR21400
OSTI ID:
6188799
Journal Information:
Journal of Applied Physics; (United States), Journal Name: Journal of Applied Physics; (United States) Vol. 70:12; ISSN 0021-8979; ISSN JAPIA
Country of Publication:
United States
Language:
English