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Evidence for structural relaxation in measurements of hydrogen diffusion in rf-sputtered boron-doped a -Si:H

Journal Article · · Physical Review, B: Condensed Matter; (USA)
 [1];  [2];  [3]
  1. Ames Laboratory-U.S. Department of Energy, Ames, IA (USA) Physics Department, Iowa State University, Ames, IA (USA)
  2. Microelectronics Research Center, Iowa State University, Ames, IA (USA)
  3. Ames Laboratory-U.S. Department of Energy and Physics Department, Iowa State University, Ames, IA (USA)

H diffusion in boron-doped rf-sputter-deposited hydrogenated amorphous Si ({ital a}-Si:H) was measured by secondary ion mass spectrometry profiles of deuterium in annealed {ital a}-Si:H/{ital a}-Si:(H,D)/{ital a}-Si:H multilayers. The exponent {alpha}=0.7{plus minus}0.1 of the diffusion constant {ital D}({ital t}) ={ital D}{sub 00}({omega}{ital t}){sup {minus}{alpha}} strongly decreases after annealing for {approximately}50 h at 180 {degree}C and {approximately}35 h at 225 {degree}C. It then increases to {approximately}0.8--1, i.e., the diffusion is nearly quenched, at longer annealing periods extending up to 1100 h. This behavior is believed to result from modifications in the microvoid system related to structural relaxation of the Si network.

DOE Contract Number:
W-7405-ENG-82
OSTI ID:
6171743
Journal Information:
Physical Review, B: Condensed Matter; (USA), Journal Name: Physical Review, B: Condensed Matter; (USA) Vol. 42:10; ISSN 0163-1829; ISSN PRBMD
Country of Publication:
United States
Language:
English