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High resolution Raman spectroscopy of complexes and clusters in molecular beams

Technical Report ·
DOI:https://doi.org/10.2172/6090820· OSTI ID:6090820

The DOE-sponsored project in this laboratory has two facets. The first is the development of methods of nonlinear Raman spectroscopy for application in studies of sparse samples. The second is the application of such methods to structural and dynamical studies of species in supersonic molecular beams. The progress we have made in both of these areas is described in this paper. The report is divided into five remaining sections. The first pertains to theoretical and experimental developments in Fourier transform stimulated emission spectroscopy and Fourier transform hole-burning spectroscopy. The second deals with progress in the development of ionization-detected stimulated Raman spectroscopies (IDSRS). The third describes results from the application of IDSRS methods to studies of jet-cooled benzene clusters. The fourth describes IDSRS results from studies of hydrogen-bonded complexes containing phenols. The fifth relates to studies of carbazole-(Ar){sub n} clusters.

Research Organization:
California Univ., Los Angeles, CA (United States)
Sponsoring Organization:
DOE; USDOE, Washington, DC (United States)
DOE Contract Number:
FG03-89ER14066
OSTI ID:
6090820
Report Number(s):
DOE/ER/14066-3; ON: DE92004206
Country of Publication:
United States
Language:
English

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Related Subjects

661220 -- Particle Beam Production & Handling
664200* -- Spectra of Atoms & Molecules & their Interactions with Photons-- (1992-)
71 CLASSICAL AND QUANTUM MECHANICS
GENERAL PHYSICS
74 ATOMIC AND MOLECULAR PHYSICS
AROMATICS
AZAARENES
AZOLES
BEAMS
BENZENE
CARBAZOLES
CLUSTER BEAMS
DOCUMENT TYPES
ENERGY LEVELS
FOURIER TRANSFORM SPECTROMETERS
FREQUENCY DEPENDENCE
HETEROCYCLIC COMPOUNDS
HYDROCARBONS
HYDROXY COMPOUNDS
IONIZATION
LASER SPECTROSCOPY
MEASURING INSTRUMENTS
MOLECULAR BEAMS
ORGANIC COMPOUNDS
ORGANIC NITROGEN COMPOUNDS
PHENOLS
PROGRESS REPORT
RAMAN SPECTROSCOPY
SPECTROMETERS
SPECTROSCOPY
Ta
Targets-- (1992-)