High resolution Raman spectroscopy of complexes and clusters in molecular beams. Performance report

Technical Report · Tue Jan 01 04:00:00 EST 1991

DOI:https://doi.org/10.2172/10108029· OSTI ID:10108029

Felker, P M

The DOE-sponsored project in this laboratory has two facets. The first is the development of methods of nonlinear Raman spectroscopy for application in studies of sparse samples. The second is the application of such methods to structural and dynamical studies of species in supersonic molecular beams. The progress we have made in both of these areas is described in this paper. The report is divided into five remaining sections. The first pertains to theoretical and experimental developments in Fourier transform stimulated emission spectroscopy and Fourier transform hole-burning spectroscopy. The second deals with progress in the development of ionization-detected stimulated Raman spectroscopies (IDSRS). The third describes results from the application of IDSRS methods to studies of jet-cooled benzene clusters. The fourth describes IDSRS results from studies of hydrogen-bonded complexes containing phenols. The fifth relates to studies of carbazole-(Ar){sub n} clusters.

• Research Organization: California Univ., Los Angeles, CA (United States)
• Sponsoring Organization: USDOE, Washington, DC (United States)
• DOE Contract Number: FG03-89ER14066
• OSTI ID: 10108029
• Report Number(s): DOE/ER/14066--3; ON: DE92004206
• Country of Publication: United States
• Language: English

Related Subjects

661220
664200
71 CLASSICAL AND QUANTUM MECHANICS
GENERAL PHYSICS
74 ATOMIC AND MOLECULAR PHYSICS
BENZENE
CARBAZOLES
CLUSTER BEAMS
ENERGY LEVELS
FOURIER TRANSFORM SPECTROMETERS
FREQUENCY DEPENDENCE
IONIZATION
MOLECULAR BEAMS
PARTICLE BEAM PRODUCTION AND HANDLING
PHENOLS
PROGRESS REPORT
RAMAN SPECTROSCOPY
SPECTRA OF ATOMS AND MOLECULES AND THEIR INTERACTIONS WITH PHOTONS
TARGETS