Studies of ground-state dynamics in isolated species by ionization-detected stimulated Raman techniques
- Univ. of California, Los Angeles (United States)
First, the author aims to develop methods of nonlinear Raman spectroscopy for application in studies of sparse samples. Second, the author wishes to apply such methods to structural and dynamical studies of species (molecules, complexes, and clusters) in supersonic molecular beams. In the past year, the author has made progress in several areas. The first pertains to the application of mass-selective ionization-detected stimulated Raman spectroscopies (IDSRS) to the size-specific vibrational spectroscopy of solute-solvent{sub n} clusters. The second involves the application of IDSRS methods to studies of jet-cooled benzene clusters. The third pertains to the use of IDSRS methods in the study of intermolecular vibrational transitions in van der Waals complexes.
- Research Organization:
- Brookhaven National Lab., Upton, NY (United States)
- OSTI ID:
- 139872
- Report Number(s):
- BNL--48923; CONF-9306172--; ON: DE93015758
- Country of Publication:
- United States
- Language:
- English
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