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Hydrogen distribution in high stability a-Si:H prepared by the hot wire technique

Book ·
OSTI ID:527675
; ;  [1];  [2]
  1. Univ. of North Carolina, Chapel Hill, NC (United States). Dept. of Physics and Astronomy
  2. National Renewable Energy Lab., Golden, CO (United States)
One of the biggest problems for the widespread use of a-Si:H based solar cells is the so-called Staebler-Wronski effect (SWE). In this work the microstructures of 2--3 hydrogen at.% hot-wire CVD a-Si:H films were characterized by {sup 1}H nuclear magnetic resonance (NMR). Significant differences were found between the hydrogen distribution in these samples and that in conventional plasma-enhanced CVD samples. Among other things, the broad resonance line in the hot-wire a-Si:H is 50 kHz wide, which is much broader than that observed 25--35 kHz in PECVD a-Si:H films. Moreover, a 0.5 kHz resonance absorption hole width due to intrinsic dipolar interactions is obtained using the hole-burning technique. Surprisingly, approximately 90% of the hydrogen atoms give rise to the 50 kHz line and only a very small percentage of the hydrogen atoms give rise to the much narrower resonance line.
OSTI ID:
527675
Report Number(s):
CONF-960401--; ISBN 1-55899-323-1
Country of Publication:
United States
Language:
English