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A study of the effect of misfit-induced strain on the kinetics of solid phase epitaxy in the Si sub 1 minus sub x Ge sub x on l angle 001 r angle Si system

Journal Article · · Journal of Applied Physics; (United States)
DOI:https://doi.org/10.1063/1.349105· OSTI ID:5203209
 [1];  [2];  [3]
  1. Division of Engineering, Brown University, Box D, Providence, Rhode Island (USA)
  2. Oak Ridge Associated Universities, Oak Ridge National Laboratory, Bldg. 5500, MS6376 Oak Ridge, Tennessee (USA)
  3. Bellcore, Red Bank, New Jersey (USA)

In this paper we present the results of an experimental determination of the rate of solid phase epitaxical regrowth of amorphous Si{sub 1{minus}{ital x}}Ge{sub {ital x}} on {l angle}001{r angle} Si as a function of temperature and Ge concentration. Layers of chemical vapor deposited Si{sub 1{minus}{ital x}}Ge{sub {ital x}} roughly 200-nm thick containing 5.4, 11.6, and 17.0 at. % Ge were amorphized with a two-step process of 100 keV, followed by 200 keV, {sup 29}Si ion implantation. This procedure left the near surface region of the substrate, including the entire Si{sub 1{minus}{ital x}}Ge{sub {ital x}} film, amorphous to a depth of 380 nm. The epitaxical recrystallization of the alloy portion (5.4, 11.6, or 17 at. % Ge) of the amorphous layer results in the development of large lattice mismatch stresses (0.5--2 GPa). The rate of epitaxical regrowth of the amorphous material was studied with isothermal heating and {ital in} {ital situ} transmission electron microscopy observations. Isothermal annealing at temperatures between 476 and 602 {degree}C show that, compared to pure unstrained Si, the rate of regrowth is decreased in strained alloys of Si{sub 1{minus}{ital x}}Ge{sub {ital x}}. Furthermore, we report that the activation energy for strained-layer regrowth of Si{sub 1{minus}{ital x}}Ge{sub {ital x}} is not a strong function of composition and, for all three compositions, was in the range 3.2{plus minus}0.2 eV. This is significantly larger than the activation energy for the homoepitaxical regrowth of unstrained pure Si. Stress related origins of these observations are discussed.

DOE Contract Number:
AC05-84OR21400; AC05-76OR00033
OSTI ID:
5203209
Journal Information:
Journal of Applied Physics; (United States), Journal Name: Journal of Applied Physics; (United States) Vol. 70:8; ISSN 0021-8979; ISSN JAPIA
Country of Publication:
United States
Language:
English