Low-pressure approach to the formation and study of exciplex systems. [For CDC 7600]
Studies on the formation and properties of new materials for high-energy, gas-phase lasers are described. Attention is directed mainly to systems having bound excited states but unbound ground states. An important class of such excimer/exciplex systems has a van der Waals dimer/oligomer as its ground state. This research attempts to probe the relative rates of electron pumping of excited-state manifolds and the preferentially pumped vibronic states within each manifold. Reactive quenching of emission, resonant self-absorption of laser emissions, and collision- and noncollision-induced intersystem crossing are also considered. Lists of personnel and facilities are included. 8 figures, 2 tables. (RWR)
- Research Organization:
- Virginia Polytechnic Inst. and State Univ., Blacksburg (USA)
- OSTI ID:
- 5058682
- Report Number(s):
- COO-2810-9
- Country of Publication:
- United States
- Language:
- English
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