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DEVELOPMENT OF A CATION EXCHANGE RESIN WITH SCINTILLATING PROPERTIES. Final Report

Technical Report ·
OSTI ID:4795042

A resin was synthesized which has the unique feature of possessing both ion exchange and scintillating properties. Cationic species of radioactive nuclides are readily adsorbed from aqueous solution in a manner similar to that of conventional ion exchange resins. Radioactive emanations from the captured nuclides result in the excitation of resin phosphors. The emitted light is of a wave length that effectively activates a photomultiplier tube of an S-11 or -13 response. Thus, radioactive isotopes can readily be counted by coupling the resin on which they are adsorbed to a photomultiplier tube and pulse counter. The resin was made by a suspension-type polymerization process as solid, spherical beads. The beads were made of polyvinyltoluene crosslinked with divinylbenzene and contained p-terphenyl and 1,4-bis-STA2-(5-phenyloxazolyl)! - benzene (POPOP) dissolved in solid solution. Ionizing sulfonic groups (-SO/sub 3/ H) were introduced on or near the surface of the beads by direct sulfonation of the aromatic nuclei. Exchange capacities in the range of 0.01 to 0.1 milliequivalents per gram of beads were obtained. Sr/sup 90/, Pu/sup 239/, and Po/sup 210/ were counted with over-all efficiencies of 50, 30, and 40% respectively, using a multichannel pulse-height analyzer. A counting efficiency of 12% was obtained for Ni/sup 63/ and 60% for Tl/sup 204/ using a liquid scintillation counter. (auth)

Research Organization:
Tracerlab. Div. of Lab. for Electronics, Inc., Richmond, Calif.
NSA Number:
NSA-16-030587
OSTI ID:
4795042
Report Number(s):
NYO-9138
Country of Publication:
United States
Language:
English